Anomalies in the Charge Yields of Fission Fragments from the

Fast-neutron-induced fission of ^{238}U at an energy just above the fission threshold is studied with a novel technique which involves the coupling of a high-efficiency γ-ray spectrometer (MINIBALL) to an inverse-kinematics neutron source (LICORNE) to extract charge yields of fission fragments via γ-γ coincidence spectroscopy. Experimental data and fission models are compared and found to be in reasonable agreement for many nuclei; however, significant discrepancies of up to 600% are observed, particularly for isotopes of Sn and Mo. This indicates that these models significantly overestimate the standard 1 fission mode and suggests that spherical shell effects in the nascent fission fragments are less important for low-energy fast-neutron-induced fission than for thermal neutron-induced fission. This has consequences for understanding and modeling the fission process, for experimental nuclear structure studies of the most neutron-rich nuclei, for future energy applications (e.g., Generation IV reactors which use fast-neutron spectra), and for the reactor antineutrino anomaly.

The Neutrons for Science Facility at SPIRAL-2.

The neutrons for science (NFS) facility is a component of SPIRAL-2, the new superconducting linear accelerator built at GANIL in Caen (France). The proton and deuteron beams delivered by the accelerator will allow producing intense neutron fields in the 100 keV-40 MeV energy range. Continuous and quasi-mono-kinetic energy spectra, respectively, will be available at NFS, produced by the interaction of a deuteron beam on a thick Be converter and by the 7Li(p,n) reaction on thin converter. The pulsed neutron beam, with a flux up to two orders of magnitude higher than those of other existing time-of-flight facilities, will open new opportunities of experiments in fundamental research as well as in nuclear data measurements. In addition to the neutron beam, irradiation stations for neutron-, proton- and deuteron-induced reactions will be available for cross-sections measurements and for the irradiation of electronic devices or biological cells. NFS, whose first experiment is foreseen in 2018, will be a very powerful tool for physics, fundamental research as well as applications like the transmutation of nuclear waste, design of future fission and fusion reactors, nuclear medicine or test and development of new detectors.

Identification of a shape isomer in 235U.

The shape isomer in 235U has been searched for in a neutron-induced fission experiment on 234U, which was performed at the isomer spectrometer NEPTUNE of the EC-JRC IRMM. A neutron source, with a tunable pulse frequency in the Hz to kHz range and its individually adjustable neutron pulse width in connection with an appropriate detector system turned out to be the ideal instrument to perform an isomer search, when decay half-lives above 100 micros are expected. From the delayed fission events observed for two different NEPTUNE settings and at mean incident neutron energies En=0.95 and 1.27 MeV the isomeric fission half-life could be determined to be T1/2=(3.6+/-1.8) ms. The corresponding cross section was determined to sigmaif=(10+/-8) microb. With these results an experimental confirmation for the existence of a superdeformed shape isomer in odd-uranium isotopes is given for the first time.

Volume traps--a new retrospective radon monitor.

A new method to trace back average radon concentrations in dwellings over several decades in time has been developed. This retrospective radon monitor is based on the measurement of the alpha activity of 210Po deposited in volume traps, e.g., spongy materials used for mattresses and cushions. Polyester samples with different densities have been exposed to radon-laden air. The exposures correspond to characteristic radon concentrations between 390 Bq m-3 and 3.9 kBq m-3 over a 20 y period. The precision in converting the 210Po-signal to the radon exposure has been improved by more than one order of magnitude compared to other common techniques. It is shown that this very sensitive method may be applied to almost all types of volume traps used in households.

The assessment of plutonium and americium in contaminated wounds with high energy resolution semiconductor detectors.

A simple to use method was installed for the measurement of wounds contaminated with plutonium and americium by using a semiconductor detector. This technique does not explicitly require the knowledge of the detector efficiency but uses a plant 241Am calibration source. A computer programme has also been developed for the quantification of the contamination according to the shape and the depth of the contaminant in the wound.

Multi-layer ²³5UF4-6LiF-Au targets for high-resolution fission fragment measurements.

Multi-layer (235)UF4-(6)LiF-Au targets have been produced by vacuum deposition on thin polyimide foils with an areal density, measured by spectrophotometry, of about 33µgcm(-2). The foils were first covered with an Au-layer and then, with a second layer of (6)LiF, both by vapour deposition. The (235)UF4 layer was prepared by fluoride sublimation. Each deposited mass was characterized separately by means of differential weighing for the Au and (6)LiF layers and by low-geometry alpha-particle counting for the (235)UF4 layer. The atomic abundances of the uranium base material have been measured by thermal ionization mass spectrometry. The targets were prepared for measuring fission-fragment emission yields with high mass-resolution.

Neutron-induced fission cross section of 233Pa between 1.0 and 3.0 MeV.

The energy dependent neutron-induced fission cross section of 233Pa has for the first time been measured directly with monoenergetic neutrons. This nuclide is an important intermediary in a thorium based fuel cycle, and its fission cross section is a key parameter in the modeling of future advanced fuel and reactor concepts. A first experiment resulted in four cross section values between 1.0 and 3.0 MeV, establishing a fission threshold in excess of 1 MeV. Significant discrepancies were found with a previous indirect experimental determination and with model estimates.