Ferroelectric switching of a two-dimensional metal.

A ferroelectric is a material with a polar structure whose polarity can be reversed (switched) by applying an electric field1,2. In metals, itinerant electrons screen electrostatic forces between ions, which explains in part why polar metals are very rare3-7. Screening also excludes external electric fields, apparently ruling out the possibility of ferroelectric switching. However, in principle, a thin enough polar metal could be sufficiently penetrated by an electric field to have its polarity switched. Here we show that the topological semimetal WTe2 provides an embodiment of this principle. Although monolayer WTe2 is centro-symmetric and thus non-polar, the stacked bulk structure is polar. We find that two- or three-layer WTe2 exhibits spontaneous out-of-plane electric polarization that can be switched using gate electrodes. We directly detect and quantify the polarization using graphene as an electric-field sensor8. Moreover, the polarization states can be differentiated by conductivity and the carrier density can be varied to modify the properties. The temperature at which polarization vanishes is above 350 kelvin, and even when WTe2 is sandwiched between graphene layers it retains its switching capability at room temperature, demonstrating a robustness suitable for applications in combination with other two-dimensional materials9-12.

Magnetic proximity and nonreciprocal current switching in a monolayer WTe2 helical edge.

The integration of diverse electronic phenomena, such as magnetism and nontrivial topology, into a single system is normally studied either by seeking materials that contain both ingredients, or by layered growth of contrasting materials1-9. The ability to simply stack very different two-dimensional van der Waals materials in intimate contact permits a different approach10,11. Here we use this approach to couple the helical edges states in a two-dimensional topological insulator, monolayer WTe2 (refs. 12-16), to a two-dimensional layered antiferromagnet, CrI3 (ref. 17). We find that the edge conductance is sensitive to the magnetization state of the CrI3, and the coupling can be understood in terms of an exchange field from the nearest and next-nearest CrI3 layers that produces a gap in the helical edge. We also find that the nonlinear edge conductance depends on the magnetization of the nearest CrI3 layer relative to the current direction. At low temperatures this produces an extraordinarily large nonreciprocal current that is switched by changing the antiferromagnetic state of the CrI3.

Giant cross-Kerr effect for propagating microwaves induced by an artificial atom.

We investigate the effective interaction between two microwave fields, mediated by a transmon-type superconducting artificial atom which is strongly coupled to a coplanar transmission line. The interaction between the fields and atom produces an effective cross-Kerr coupling. We demonstrate average cross-Kerr phase shifts of up to 20 degrees per photon with both coherent microwave fields at the single-photon level. Our results provide an important step toward quantum applications with propagating microwave photons.

Generation of nonclassical microwave states using an artificial atom in 1D open space.

We have embedded an artificial atom, a superconducting transmon qubit, in a 1D open space and investigated the scattering properties of an incident microwave coherent state. By studying the statistics of the reflected and transmitted fields, we demonstrate that the scattered states can be nonclassical. In particular, by measuring the second-order correlation function, g((2)), we show photon antibunching in the reflected field and superbunching in the transmitted field. We also compare the elastically and inelastically scattered fields using both phase-sensitive and phase-insensitive measurements.

Demonstration of a single-photon router in the microwave regime.

We have embedded an artificial atom, a superconducting transmon qubit, in an open transmission line and investigated the strong scattering of incident microwave photons (∼6 GHz). When an input coherent state, with an average photon number N≪1 is on resonance with the artificial atom, we observe extinction of up to 99.6% in the forward propagating field. We use two-tone spectroscopy to study scattering from excited states and we observe electromagnetically induced transparency (EIT). We then use EIT to make a single-photon router, where we can control to what output port an incoming signal is delivered. The maximum on-off ratio is around 99% with a rise and fall time on the order of nanoseconds, consistent with theoretical expectations. The router can easily be extended to have multiple output ports and it can be viewed as a rudimentary quantum node, an important step towards building quantum information networks.

Gate-induced superconductivity in a monolayer topological insulator.

The layered semimetal tungsten ditelluride (WTe2) has recently been found to be a two-dimensional topological insulator (2D TI) when thinned down to a single monolayer, with conducting helical edge channels. We found that intrinsic superconductivity can be induced in this monolayer 2D TI by mild electrostatic doping at temperatures below 1 kelvin. The 2D TI-superconductor transition can be driven by applying a small gate voltage. This discovery offers possibilities for gate-controlled devices combining superconductivity and nontrivial topological properties, and could provide a basis for quantum information schemes based on topological protection.