Single-Photon Synchronization with a Room-Temperature Atomic Quantum Memory.

Efficient synchronization of single photons that are compatible with narrow band atomic transitions is an outstanding challenge, which could prove essential for photonic quantum information processing. Here we report on the synchronization of independently generated single photons using a room-temperature atomic quantum memory. The photon source and the memory are interconnected by fibers and employ the same ladder-level atomic scheme. We store and retrieve the heralded single photons with end-to-end efficiency of η_{e2e}=25% and final antibunching of g_{h}^{(2)}=0.023. Our synchronization process results in an over tenfold increase in the photon-pair coincidence rate, reaching a rate of more than 1000 detected synchronized photon pairs per second. The indistinguishability of the synchronized photons is verified by a Hong-Ou-Mandel interference measurement.

Floquet Gauge Anomaly Inflow and Arbitrary Fractional Charge in Periodically Driven Topological-Normal Insulator Heterostructures.

Usually, when coupling in a background gauge field, topological zero modes would yield an anomalous current at the interface, culminating in the zero-mode anomaly inflow, which is ultimately conserved by extra contributions from the topological bulk. However, the anomaly inflow mechanism for guiding Floquet steady states is rarely explored in periodically driven systems. Here we synthesize a driven topological-normal insulator heterostructure and propose a Floquet gauge anomaly inflow, associated with the occurrence of arbitrary fractional charge. Through our photonic modeling, we experimentally observed a Floquet gauge anomaly as the system was driven into anomalous topological phases. Prospectively, we believe our findings could pave a novel avenue on exploring Floquet gauge anomalies in driven systems of condensed matter, photonics, and ultracold atoms.

Pulsed-pump phosphorus-doped fiber Raman amplifier around 1260 nm for applications in quantum non-linear optics.

We describe a fiber Raman amplifier for nanosecond and sub-nanosecond pulses centered around 1260 nm. The amplification takes place inside a 4.5-m-long polarization-maintaining phosphorus-doped fiber, pumped at 1080 nm by 3-ns-long pulses with a repetition rate of 200 kHz and up to 1.75 kW peak power. The input seed pulses are of sub-mW peak-power and minimal duration of 0.25 ns, carved out of a continuous-wave laser with sub-MHz linewidth. We obtain linearly polarized output pulses with peak powers of up to 1.4 kW, corresponding to peak-power conversion efficiency of over 80%. An ultrahigh small signal gain of 90 dB is achieved, and the signal-to-noise ratio 3 dB below the saturation power is above 20 dB. No significant temporal and spectral broadening is observed for output pulses up to 400 W peak power, and broadening at higher powers can be reduced by phase modulation of the seed pulse. Thus, nearly-transform-limited pulses with peak power up to 1 kW are obtained. Finally, we demonstrate the generation of pulses with controllable frequency chirp, pulses with variable width, and double pulses. This amplifier is thus suitable for coherent control of narrow atomic resonances, especially for the fast and coherent excitation of rubidium atoms to Rydberg states. These abilities open the way towards several important applications in quantum non-linear optics.

Recovering the Homogeneous Absorption of Inhomogeneous Media.

The resonant absorption of light by an ensemble of absorbers decreases when the resonance is inhomogeneously broadened. Recovering the lost absorption cross section is of great importance for various applications of light-matter interactions, particularly in quantum optics, but no recovery mechanism has yet been identified and successfully demonstrated. Here, we formulate the limit set by the inhomogeneity on the absorption, and present a mechanism able to circumvent this limit and fully recover the homogeneous absorption of the ensemble. We experimentally study this mechanism using two different level schemes in atomic vapors and demonstrate up to fivefold enhancement of the absorption above the inhomogeneous limit. Our scheme relies on light shifts induced by auxiliary fields and is thus applicable to various physical systems and inhomogeneity mechanisms.

Coherent Control and Wave Mixing in an Ensemble of Silicon-Vacancy Centers in Diamond.

Strong light-matter interactions are critical for quantum technologies based on light, such as memories or nonlinear interactions. Solid state materials will be particularly important for such applications due to the relative ease of fabrication of components. Silicon vacancy centers (SiV^{-}) in diamond feature especially narrow inhomogeneous spectral lines, which are rare in solid materials. Here, we demonstrate resonant coherent manipulation, stimulated Raman adiabatic passage, and strong light-matter interaction via the four-wave mixing of a weak signal field in an ensemble of SiV^{-} centers.

Experimental Demonstration of Quantum Effects in the Operation of Microscopic Heat Engines.

The ability of the internal states of a working fluid to be in a coherent superposition is one of the basic properties of a quantum heat engine. It was recently predicted that in the regime of small engine action, this ability can enable a quantum heat engine to produce more power than any equivalent classical heat engine. It was also predicted that in the same regime, the presence of such internal coherence causes different types of quantum heat engines to become thermodynamically equivalent. Here, we use an ensemble of nitrogen vacancy centers in diamond for implementing two types of quantum heat engines, and experimentally observe both effects.

Ultrahigh and persistent optical depths of cesium in Kagomé-type hollow-core photonic crystal fibers.

Alkali-filled hollow-core fibers are a promising medium for investigating light-matter interactions, especially at the single-photon level, due to the tight confinement of light and high optical depths achievable by light-induced atomic desorption (LIAD). However, until now these large optical depths could only be generated for seconds, at most once per day, severely limiting the practicality of the technology. Here we report the generation of the highest observed transient (>10(5) for up to a minute) and highest observed persistent (>2000 for hours) optical depths of alkali vapors in a light-guiding geometry to date, using a cesium-filled Kagomé-type hollow-core photonic crystal fiber (HC-PCF). Our results pave the way to light-matter interaction experiments in confined geometries requiring long operation times and large atomic number densities, such as generation of single-photon-level nonlinearities and development of single photon quantum memories.

Quantum vortices of strongly interacting photons.

Vortices are topologically nontrivial defects that generally originate from nonlinear field dynamics. All-optical generation of photonic vortices-phase singularities of the electromagnetic field-requires sufficiently strong nonlinearity that is typically achieved in the classical optics regime. We report on the realization of quantum vortices of photons that result from a strong photon-photon interaction in a quantum nonlinear optical medium. The interaction causes faster phase accumulation for copropagating photons, producing a quantum vortex-antivortex pair within the two-photon wave function. For three photons, the formation of vortex lines and a central vortex ring confirms the existence of a genuine three-photon interaction. The wave function topology, governed by two- and three-photon bound states, imposes a conditional phase shift of π per photon, a potential resource for deterministic quantum logic operations.

Nonlinear coherent heat machines.

We propose heat machines that are nonlinear, coherent, and closed systems composed of few field (oscillator) modes. Their thermal-state input is transformed by nonlinear Kerr interactions into nonthermal (non-Gaussian) output with controlled quantum fluctuations and the capacity to deliver work in a chosen mode. These machines can provide an output with strongly reduced phase and amplitude uncertainty that may be useful for sensing or communications in the quantum domain. They are experimentally realizable in optomechanical cavities where photonic and phononic modes are coupled by a Josephson qubit or in cold gases where interactions between photons are transformed into dipole-dipole interacting Rydberg atom polaritons. This proposed approach is a step toward the bridging of quantum and classical coherent and thermodynamic descriptions.

Two-photon path-entangled states in multimode waveguides.

We experimentally show that two-photon path-entangled states can be coherently manipulated by multimode interference in multimode waveguides. By measuring the output two-photon spatial correlation function versus the phase of the input state, we show that multimode waveguides perform as nearly ideal multiport beam splitters at the quantum level, creating a large variety of entangled and separable multipath two-photon states.

A hybrid quantum memory-enabled network at room temperature.

Quantum memory capable of storage and retrieval of flying photons on demand is crucial for developing quantum information technologies. However, the devices needed for long-distance links are different from those envisioned for local processing. We present the first hybrid quantum memory-enabled network by demonstrating the interconnection and simultaneous operation of two types of quantum memory: an atomic ensemble-based memory and an all-optical Loop memory. Interfacing the quantum memories at room temperature, we observe a well-preserved quantum correlation and a violation of Cauchy-Schwarz inequality. Furthermore, we demonstrate the creation and storage of a fully-operable heralded photon chain state that can achieve memory-built-in combining, swapping, splitting, tuning, and chopping single photons in a chain temporally. Such a quantum network allows atomic excitations to be generated, stored, and converted to broadband photons, which are then transferred to the next node, stored, and faithfully retrieved, all at high speed and in a programmable fashion.

Fast, noise-free memory for photon synchronization at room temperature.

Future quantum photonic networks require coherent optical memories for synchronizing quantum sources and gates of probabilistic nature. We demonstrate a fast ladder memory (FLAME) mapping the optical field onto the superposition between electronic orbitals of rubidium vapor. Using a ladder-level system of orbital transitions with nearly degenerate frequencies simultaneously enables high bandwidth, low noise, and long memory lifetime. We store and retrieve 1.7-ns-long pulses, containing 0.5 photons on average, and observe short-time external efficiency of 25%, memory lifetime (1/e) of 86 ns, and below 10-4 added noise photons. Consequently, coupling this memory to a probabilistic source would enhance the on-demand photon generation probability by a factor of 12, the highest number yet reported for a noise-free, room temperature memory. This paves the way toward the controlled production of large quantum states of light from probabilistic photon sources.