High-fidelity spin qubit operation and algorithmic initialization above 1 K.

The encoding of qubits in semiconductor spin carriers has been recognized as a promising approach to a commercial quantum computer that can be lithographically produced and integrated at scale1-10. However, the operation of the large number of qubits required for advantageous quantum applications11-13 will produce a thermal load exceeding the available cooling power of cryostats at millikelvin temperatures. As the scale-up accelerates, it becomes imperative to establish fault-tolerant operation above 1 K, at which the cooling power is orders of magnitude higher14-18. Here we tune up and operate spin qubits in silicon above 1 K, with fidelities in the range required for fault-tolerant operations at these temperatures19-21. We design an algorithmic initialization protocol to prepare a pure two-qubit state even when the thermal energy is substantially above the qubit energies and incorporate radiofrequency readout to achieve fidelities up to 99.34% for both readout and initialization. We also demonstrate single-qubit Clifford gate fidelities up to 99.85% and a two-qubit gate fidelity of 98.92%. These advances overcome the fundamental limitation that the thermal energy must be well below the qubit energies for the high-fidelity operation to be possible, surmounting a main obstacle in the pathway to scalable and fault-tolerant quantum computation.

Dynamics of Hole Singlet-Triplet Qubits with Large g-Factor Differences.

The spin-orbit interaction permits to control the state of a spin qubit via electric fields. For holes it is particularly strong, allowing for fast all electrical qubit manipulation, and yet an in-depth understanding of this interaction in hole systems is missing. Here we investigate, experimentally and theoretically, the effect of the cubic Rashba spin-orbit interaction on the mixing of the spin states by studying singlet-triplet oscillations in a planar Ge hole double quantum dot. Landau-Zener sweeps at different magnetic field directions allow us to disentangle the effects of the spin-orbit induced spin-flip term from those caused by strongly site-dependent and anisotropic quantum dot g tensors. Our work, therefore, provides new insights into the hole spin-orbit interaction, necessary for optimizing future qubit experiments.

Strong Coupling of Microwave Photons to Antiferromagnetic Fluctuations in an Organic Magnet.

Coupling between a crystal of di(phenyl)-(2,4,6-trinitrophenyl)iminoazanium radicals and a superconducting microwave resonator is investigated in a circuit quantum electrodynamics (circuit QED) architecture. The crystal exhibits paramagnetic behavior above 4 K, with antiferromagnetic correlations appearing below this temperature, and we demonstrate strong coupling at base temperature. The magnetic resonance acquires a field angle dependence as the crystal is cooled down, indicating anisotropy of the exchange interactions. These results show that multispin modes in organic crystals are suitable for circuit QED, offering a platform for their coherent manipulation. They also utilize the circuit QED architecture as a way to probe spin correlations at low temperature.

Universal response of quantum systems with chaotic dynamics.

The prediction of the response of a closed system to external perturbations is one of the central problems in quantum mechanics, and in this respect, the local density of states (LDOS) provides an in-depth description of such a response. The LDOS is the distribution of the overlaps squared connecting the set of eigenfunctions with the perturbed one. Here, we show that in the case of closed systems with classically chaotic dynamics, the LDOS is a Breit-Wigner distribution under very general perturbations of arbitrary high intensity. Consequently, we derive a semiclassical expression for the width of the LDOS which is shown to be very accurate for paradigmatic systems of quantum chaos. This Letter demonstrates the universal response of quantum systems with classically chaotic dynamics.

Loschmidt echo and the local density of states.

Loschmidt echo (LE) is a measure of reversibility and sensitivity to perturbations of quantum evolutions. For weak perturbations its decay rate is given by the width of the local density of states (LDOS). When the perturbation is strong enough, it has been shown in chaotic systems that its decay is dictated by the classical Lyapunov exponent. However, several recent studies have shown an unexpected nonuniform decay rate as a function of the perturbation strength instead of that Lyapunov decay. Here we study the systematic behavior of this regime in perturbed cat maps. We show that some perturbations produce coherent oscillations in the width of LDOS that imprint clear signals of the perturbation in LE decay. We also show that if the perturbation acts in a small region of phase space (local perturbation) the effect is magnified and the decay is given by the width of the LDOS.