Resource-Efficient High-Dimensional Entanglement Detection via Symmetric Projections.

We introduce two families of criteria for detecting and quantifying the entanglement of a bipartite quantum state of arbitrary local dimension. The first is based on measurements in mutually unbiased bases and the second is based on equiangular measurements. Both criteria give a qualitative result in terms of the state's entanglement dimension and a quantitative result in terms of its fidelity with the maximally entangled state. The criteria are universally applicable since no assumptions on the state are required. Moreover, the experimenter can control the trade-off between resource-efficiency and noise-tolerance by selecting the number of measurements performed. For paradigmatic noise models, we show that only a small number of measurements are necessary to achieve nearly-optimal detection in any dimension. The number of global product projections scales only linearly in the local dimension, thus paving the way for detection and quantification of very high-dimensional entanglement.

Fundamental Accuracy-Resolution Trade-Off for Timekeeping Devices.

From a thermodynamic point of view, all clocks are driven by irreversible processes. Additionally, one can use oscillatory systems to temporally modulate the thermodynamic flux towards equilibrium. Focusing on the most elementary thermalization events, this modulation can be thought of as a temporal probability concentration for these events. There are two fundamental factors limiting the performance of clocks: On the one level, the inevitable drifts of the oscillatory system, which are addressed by finding stable atomic or nuclear transitions that lead to astounding precision of today's clocks. On the other level, there is the intrinsically stochastic nature of the irreversible events upon which the clock's operation is based. This becomes relevant when seeking to maximize a clock's resolution at high accuracy, which is ultimately limited by the number of such stochastic events per reference time unit. We address this essential trade-off between clock accuracy and resolution, proving a universal bound for all clocks whose elementary thermalization events are memoryless.

Impact of Imperfect Timekeeping on Quantum Control.

In order to unitarily evolve a quantum system, an agent requires knowledge of time, a parameter that no physical clock can ever perfectly characterize. In this Letter, we study how limitations on acquiring knowledge of time impact controlled quantum operations in different paradigms. We show that the quality of timekeeping an agent has access to limits the circuit complexity they are able to achieve within circuit-based quantum computation. We do this by deriving an upper bound on the average gate fidelity achievable under imperfect timekeeping for a general class of random circuits. Another area where quantum control is relevant is quantum thermodynamics. In that context, we show that cooling a qubit can be achieved using a timer of arbitrary quality for control: timekeeping error only impacts the rate of cooling and not the achievable temperature. Our analysis combines techniques from the study of autonomous quantum clocks and the theory of quantum channels to understand the effect of imperfect timekeeping on controlled quantum dynamics.

Entanglement Detection with Imprecise Measurements.

We investigate entanglement detection when the local measurements only nearly correspond to those intended. This corresponds to a scenario in which measurement devices are not perfectly controlled, but nevertheless operate with bounded inaccuracy. We formalize this through an operational notion of inaccuracy that can be estimated directly in the lab. To demonstrate the relevance of this approach, we show that small magnitudes of inaccuracy can significantly compromise several well-known entanglement witnesses. For two arbitrary-dimensional systems, we show how to compute tight corrections to a family of standard entanglement witnesses due to any given level of measurement inaccuracy. We also develop semidefinite programming methods to bound correlations in these scenarios.

Entanglement Quantification in Atomic Ensembles.

Entanglement measures quantify nonclassical correlations present in a quantum system, but can be extremely difficult to calculate, even more so, when information on its state is limited. Here, we consider broad families of entanglement criteria that are based on variances of arbitrary operators and analytically derive the lower bounds these criteria provide for two relevant entanglement measures: the best separable approximation and the generalized robustness. This yields a practical method for quantifying entanglement in realistic experimental situations, in particular, when only few measurements of simple observables are available. As a concrete application of this method, we quantify bipartite and multipartite entanglement in spin-squeezed Bose-Einstein condensates of ∼500 atoms, by lower bounding the best separable approximation and the generalized robustness only from measurements of first and second moments of the collective spin operator.

Experimental Single-Copy Entanglement Distillation.

The phenomenon of entanglement marks one of the furthest departures from classical physics and is indispensable for quantum information processing. Despite its fundamental importance, the distribution of entanglement over long distances through photons is unfortunately hindered by unavoidable decoherence effects. Entanglement distillation is a means of restoring the quality of such diluted entanglement by concentrating it into a pair of qubits. Conventionally, this would be done by distributing multiple photon pairs and distilling the entanglement into a single pair. Here, we turn around this paradigm by utilizing pairs of single photons entangled in multiple degrees of freedom. Specifically, we make use of the polarization and the energy-time domain of photons, both of which are extensively field tested. We experimentally chart the domain of distillable states and achieve relative fidelity gains up to 13.8%. Compared to the two-copy scheme, the distillation rate of our single-copy scheme is several orders of magnitude higher, paving the way towards high-capacity and noise-resilient quantum networks.

Pathways for Entanglement-Based Quantum Communication in the Face of High Noise.

Entanglement-based quantum communication offers an increased level of security in practical secret shared key distribution. One of the fundamental principles enabling this security-the fact that interfering with one photon will destroy entanglement and thus be detectable-is also the greatest obstacle. Random encounters of traveling photons, losses, and technical imperfections make noise an inevitable part of any quantum communication scheme, severely limiting distance, key rate, and environmental conditions in which quantum key distribution can be employed. Using photons entangled in their spatial degree of freedom, we show that the increased noise resistance of high-dimensional entanglement can indeed be harnessed for practical key distribution schemes. We perform quantum key distribution in eight entangled paths at various levels of environmental noise and show key rates that, even after error correction and privacy amplification, still exceed 1 bit per photon pair and furthermore certify a secure key at noise levels that would prohibit comparable qubit based schemes from working.

Efficient Generation of High-Dimensional Entanglement through Multipath Down-Conversion.

High-dimensional entanglement promises to greatly enhance the performance of quantum communication and enable quantum advantages unreachable by qubit entanglement. One of the great challenges, however, is the reliable production, distribution, and local certification of high-dimensional sources of entanglement. In this Letter, we present an optical setup capable of producing quantum states with an exceptionally high level of scalability, control, and quality that, together with novel certification techniques, achieve the highest amount of entanglement recorded so far. We showcase entanglement in 32-spatial dimensions with record fidelity to the maximally entangled state (F=0.933±0.001) and introduce measurement efficient schemes to certify entanglement of formation (E_{oF}=3.728±0.006). Combined with the existing multicore fiber technology, our results will lay a solid foundation for the construction of high-dimensional quantum networks.

Erratum: Quantifying Entanglement of Maximal Dimension in Bipartite Mixed States [Phys. Rev. Lett. 117, 190502 (2016)].

This corrects the article DOI: 10.1103/PhysRevLett.117.190502.

Unifying Paradigms of Quantum Refrigeration: A Universal and Attainable Bound on Cooling.

Cooling quantum systems is arguably one of the most important thermodynamic tasks connected to modern quantum technologies and an interesting question from a foundational perspective. It is thus of no surprise that many different theoretical cooling schemes have been proposed, differing in the assumed control paradigm and complexity, and operating either in a single cycle or in steady state limits. Working out bounds on quantum cooling has since been a highly context dependent task with multiple answers, with no general result that holds independent of assumptions. In this Letter we derive a universal bound for cooling quantum systems in the limit of infinite cycles (or steady state regimes) that is valid for any control paradigm and machine size. The bound only depends on a single parameter of the refrigerator and is theoretically attainable in all control paradigms. For qubit targets we prove that this bound is achievable in a single cycle and by autonomous machines.

Measuring azimuthal and radial modes of photons.

With the emergence of the field of quantum communications, the appropriate choice of photonic degrees of freedom used for encoding information is of paramount importance. Highly precise techniques for measuring the polarisation, frequency, and arrival time of a photon have been developed. However, the transverse spatial degree of freedom still lacks a measurement scheme that allows the reconstruction of its full transverse structure with a simple implementation and a high level of accuracy. Here we show a method to measure the azimuthal and radial modes of Laguerre-Gaussian beams with a greater than 99 % accuracy, using a single phase screen. We compare our technique with previous commonly used methods and demonstrate the significant improvements it presents for quantum key distribution and state tomography of high-dimensional quantum states of light. Moreover, our technique can be readily extended to any arbitrary family of spatial modes, such as mutually unbiased bases, Hermite-Gauss, and Ince-Gauss. Our scheme will significantly enhance existing quantum and classical communication protocols that use the spatial structure of light, as well as enable fundamental experiments on spatial-mode entanglement to reach their full potential.

Eigenstate Thermalization for Degenerate Observables.

Under unitary time evolution, expectation values of physically reasonable observables often evolve towards the predictions of equilibrium statistical mechanics. The eigenstate thermalization hypothesis (ETH) states that this is also true already for individual energy eigenstates. Here we aim at elucidating the emergence of the ETH for observables that can realistically be measured due to their high degeneracy, such as local, extensive, or macroscopic observables. We bisect this problem into two parts, a condition on the relative overlaps and one on the relative phases between the eigenbases of the observable and Hamiltonian. We show that the relative overlaps are unbiased for highly degenerate observables and demonstrate that unless relative phases conspire to cumulative effects, this makes such observables verify the ETH. Through this we elucidate potential pathways towards proofs of thermalization.

High-Dimensional Entanglement in States with Positive Partial Transposition.

Genuine high-dimensional entanglement, i.e., the property of having a high Schmidt number, constitutes an instrumental resource in quantum communication, overcoming limitations of low-dimensional systems. States with a positive partial transpose (PPT) are generally considered weakly entangled, as they can never be distilled into pure entangled states. This naturally raises the question of whether high Schmidt numbers are possible for PPT states. Volume estimates suggest that optimal, i.e., linear, scaling in the local dimension should be possible, albeit without providing insight into the possible slope. We provide the first explicit construction of a family of PPT states that achieves linear scaling in the local dimension and we prove that random PPT states typically share this feature. Our construction also allows us to prove a recent conjecture of Chen et al. on the existence of PPT states whose Schmidt number increases by an arbitrarily large amount upon partial transposition. Finally, we link the Schmidt number to entangled sub-block matrices of a quantum state. We use this connection to prove that quantum states that are either (i) invariant under partial transposition on the smallest of their two subsystems, or (ii) absolutely PPT cannot have a maximal Schmidt number. Overall, our findings shed new light on some fundamental problems in entanglement theory.

Characterizing Genuine Multilevel Entanglement.

Entanglement of high-dimensional quantum systems has become increasingly important for quantum communication and experimental tests of nonlocality. However, many effects of high-dimensional entanglement can be simulated by using multiple copies of low-dimensional systems. We present a general theory to characterize those high-dimensional quantum states for which the correlations cannot simply be simulated by low-dimensional systems. Our approach leads to general criteria for detecting multilevel entanglement in multiparticle quantum states, which can be used to verify these phenomena experimentally.

No-Go Theorem for the Characterization of Work Fluctuations in Coherent Quantum Systems.

An open question of fundamental importance in thermodynamics is how to describe the fluctuations of work for quantum coherent processes. In the standard approach, based on a projective energy measurement both at the beginning and at the end of the process, the first measurement destroys any initial coherence in the energy basis. Here we seek extensions of this approach which can possibly account for initially coherent states. We consider all measurement schemes to estimate work and require that (i) the difference of average energy corresponds to average work for closed quantum systems and that (ii) the work statistics agree with the standard two-measurement scheme for states with no coherence in the energy basis. We first show that such a scheme cannot exist. Next, we consider the possibility of performing collective measurements on several copies of the state and prove that it is still impossible to simultaneously satisfy requirements (i) and (ii). Nevertheless, improvements do appear, and in particular, we develop a measurement scheme that acts simultaneously on two copies of the state and allows us to describe a whole class of coherent transformations.

Quantifying Photonic High-Dimensional Entanglement.

High-dimensional entanglement offers promising perspectives in quantum information science. In practice, however, the main challenge is to devise efficient methods to characterize high-dimensional entanglement, based on the available experimental data which is usually rather limited. Here we report the characterization and certification of high-dimensional entanglement in photon pairs, encoded in temporal modes. Building upon recently developed theoretical methods, we certify an entanglement of formation of 2.09(7) ebits in a time-bin implementation, and 4.1(1) ebits in an energy-time implementation. These results are based on very limited sets of local measurements, which illustrates the practical relevance of these methods.

Generation and confirmation of a (100 x 100)-dimensional entangled quantum system.

Entangled quantum systems have properties that have fundamentally overthrown the classical worldview. Increasing the complexity of entangled states by expanding their dimensionality allows the implementation of novel fundamental tests of nature, and moreover also enables genuinely new protocols for quantum information processing. Here we present the creation of a (100 × 100)-dimensional entangled quantum system, using spatial modes of photons. For its verification we develop a novel nonlinear criterion which infers entanglement dimensionality of a global state by using only information about its subspace correlations. This allows very practical experimental implementation as well as highly efficient extraction of entanglement dimensionality information. Applications in quantum cryptography and other protocols are very promising.

Steering Maps and Their Application to Dimension-Bounded Steering.

The existence of quantum correlations that allow one party to steer the quantum state of another party is a counterintuitive quantum effect that was described at the beginning of the past century. Steering occurs if entanglement can be proven even though the description of the measurements on one party is not known, while the other side is characterized. We introduce the concept of steering maps, which allow us to unlock sophisticated techniques that were developed in regular entanglement detection and to use them for certifying steerability. As an application, we show that this allows us to go beyond even the canonical steering scenario; it enables a generalized dimension-bounded steering where one only assumes the Hilbert space dimension on the characterized side, with no description of the measurements. Surprisingly, this does not weaken the detection strength of very symmetric scenarios that have recently been carried out in experiments.

Quantifying Entanglement of Maximal Dimension in Bipartite Mixed States.

The Schmidt coefficients capture all entanglement properties of a pure bipartite state and therefore determine its usefulness for quantum information processing. While the quantification of the corresponding properties in mixed states is important both from a theoretical and a practical point of view, it is considerably more difficult, and methods beyond estimates for the concurrence are elusive. In particular this holds for a quantitative assessment of the most valuable resource, the forms of entanglement that can only exist in high-dimensional systems. We derive a framework for lower bounding the appropriate measure of entanglement, the so-called G-concurrence, through few local measurements. Moreover, we show that these bounds have relevant applications also for multipartite states.

Should Entanglement Measures be Monogamous or Faithful?

"Is entanglement monogamous?" asks the title of a popular article [B. Terhal, IBM J. Res. Dev. 48, 71 (2004)], celebrating C. H. Bennett's legacy on quantum information theory. While the answer is affirmative in the qualitative sense, the situation is less clear if monogamy is intended as a quantitative limitation on the distribution of bipartite entanglement in a multipartite system, given some particular measure of entanglement. Here, we formalize what it takes for a bipartite measure of entanglement to obey a general quantitative monogamy relation on all quantum states. We then prove that an important class of entanglement measures fail to be monogamous in this general sense of the term, with monogamy violations becoming generic with increasing dimension. In particular, we show that every additive and suitably normalized entanglement measure cannot satisfy any nontrivial general monogamy relation while at the same time faithfully capturing the geometric entanglement structure of the fully antisymmetric state in arbitrary dimension. Nevertheless, monogamy of such entanglement measures can be recovered if one allows for dimension-dependent relations, as we show explicitly with relevant examples.