[Current Activity Levels of Artificial Radionuclides in Water Facilities Located at the Semipalatinsk Test Site].

The current data of radioecological research within the Semipalatinsk test site (STS) are presented in the pa- per. It has been shown that almost 90% of polygon lands can be returned to the national economy. Waters of water facilities located at conditionally "background" territories of the STS do not present a radiation hazard to population. Waters of the potential water facilities located close to the radiation hazardous facilities have an increased level of the specific activity of individual radionuclides. Recommendations for the radiological assessment of the quality of waters in water facilities located near radiation hazardous facilities and adjacent territories of STS are offered in the article.

[Study on Tritium Content in Soil at Sites of Nuclear Explosions on the Territory of Semipalatinsk Test Site].

As a result of investigations carried out on the territory of Semipalatinsk Test Site, tritium was found in different environmental objects--surface and ground waters, vegetation, air environment, and snow cover. The analysis of the data obtained has shown that contamination of environmental objects at the Semipalatinsk Test Site with tritium is associated with the places where underground nuclear tests were performed. Since tritium can originate from an activation reaction and be trapped by pock particles during a test, it was decided to examine the soil in the sites where surface and excavation tests took place. It was found that the concentration of tritium in soil correlates with the concentration of europium. Probably, the concentration of tritium in the soil depends on the character and yield of the tests performed. Findings of the study have revealed that tritium can be found in soil in significant amounts not only in sites where underground nuclear tests took place but also in sites where surface and excavation nuclear tests were carried out.

Assessment of the tritium distribution in the vegetation cover in the areas of underground nuclear explosions at the Semipalatinsk test site.

This paper provides results of assessment of the tritium distribution in the vegetation cover in the areas of underground nuclear explosions at the Semipalatinsk Test Site (STS). The research was conducted at the former "Degelen" test site along the streams that are one of the main channels of tritium migration from underground nuclear explosions epicenters. The dominant plant species Carex supine and Achnatherum splendens that belong to different ecological groups in relation to humidity were selected as representatives of the vegetation cover. The TFWT (tissue free water tritium) and OBT (organically bound tritium) activity concentrations in the vegetation cover were measurement. TFWT activity concentration in the samples of both plant species had high values with an average of up to 30 kBq kg-1. The OBT activity concentration was 1-2 orders of magnitude lower than the TFWT in all plant samples. The TFWT and OBT activity concentrations in vegetation samples are closely correlated (r = 0.75, p < 0.05). No statistically significant difference was found between the content of tritium in the samples of Carex supine and those of Achnatherum splendens taken at the same locations. OBT/HTO ratios for vegetation samples of both species were close to equilibrium ratio used in environmental transfer models. In some cases, OBT/HTO ratios were significantly lower than one, which indicates that simple environmental transfer models may not accurately predict the behavior of HTO and OBT in different environmental compartments. The average OBT/HTO ratio for soil samples (0.6 ± 0.1) close to the equilibrium value indicates the equilibrium condition at the research area. The obtained [OBT]plant/[OBT]soil ratios indicate that soil organic matter accumulates tritium from year to year. However, in some locations with high tritium contamination ratios [OBT]plant/[OBT]soil were more than one due to OBT activity in soils is almost the same as OBT activity in plants. It was found that the nature of the spatial distribution of tritium in the vegetation cover in the areas of underground nuclear explosions is complex, and obviously depends on the location of the tunnels in which nuclear tests were conducted, as well as on the peculiarities of the hydrological regime of underground and surface waters, which are the main channels of tritium migration in the research area. Thus, the vegetation cover reflects the spatial distribution of tritium contamination in the sites of underground nuclear explosions and can be used as an indicator of the radiation situation when monitoring radiation-hazardous areas.

Transfer parameters of radionuclides from soil to plants at the area of craters produced by underground nuclear explosions at the Semipalatinsk test site.

A study to determine 137Cs, 90Sr, 241Am, 239+240Pu radionuclides in vegetation cover of the area of craters produced by underground nuclear explosions at the Semipalatinsk test site (STS) is summarised in this paper. Transfer factors (Tf) required for the quantitative description of the radionuclides transition from the soil to aboveground plant parts were found to be highest for sagebrush (Artemisia sublessingiana), Tf values for 90Sr were gradually decreasing with increasing distance from the dump zone. When arranging the radionuclide transferring factors in descending order, the following sequence was obtained: 90Sr Tf > 137Cs Tf > 241Am Tf > 239+240Pu Tf, which is consistent with International data. All Tf derived are much higher than those ones derived earlier for epicenters of aboveground nuclear tests and are closest to values for conventionally "background" areas at the Semipalatinsk test site.

Development of measures for limiting negative impacts of the «Atomic¼ lake on population and environment.

In arid climate, economic activities at the territory of the "Atomic" lake is one of the topical issues for the Semipalatinsk test site (STS). Hence, the boundaries of areas with radionuclides contamination, which correspond to the level of radioactive wastes at the territory adjacent to the "Atomic" lake of STS, are to be determined. The territory around the lake is used for cattle breeding and the water of the "Atomic" lake that is the one large water source is used for livestock watering. It is important to develop measures that will limit possible negative impact on population and environment. In results of the conducted research were developed measures consisting of remediation and access limitation to the stockpile of soils with contamination level corresponding to the level of radioactive waste (RW).

Researching of tritium speciation in soils of "Balapan" site.

Speciation of tritium (3Н) in soils from the "Balapan" site in Semipalatinsk are presented in this study. Three interrelated objects were chosen for further study: "Atomic" lake, the Shagan River and an external reservoir. The main speciation forms of 3Н in soil were: 3Н in surface-adsorbed water, 3Н in interlayer water, hydroxylic 3Н, organically bound 3Н and crystalline-bound 3Н. Results will allow an estimation of contamination mechanism to be made, and will also allow the potential for migration and bioavailability of 3Н to be assessed.

Studying of tritium content in snowpack of Degelen mountain range.

The paper presents the results of investigation of tritium content in the layers of snow located in the streambeds of the "Degelen" massif contaminated with tritium. The objects of investigation were selected watercourses Karabulak, Uzynbulak, Aktybai located beyond the "Degelen" site. We studied the spatial distribution of tritium relative to the streambed of watercourses and defined the borders of the snow cover contamination. In the centre of the creek watercourses the snow contamination in the surface layer is as high as 40 000 Bq/L. The values of the background levels of tritium in areas not related to the streambed, which range from 40 to 50 Bq/L. The results of snow cover measurements in different seasonal periods were compared. The main mechanisms causing tritium transfer in snow were examined and identified. The most important mechanism of tritium transfer in the streams is tritium emanation from ice or soil surface.

Tritium as an indicator of venues for nuclear tests.

Currently, due to the Treaty on the Non-proliferation of Nuclear Weapons there is a highly topical issue of an accurate verification of nuclear explosion venues. This paper proposes to consider new method for verification by using tritium as an indicator. Detailed studies of the tritium content in the air were carried in the locations of underground nuclear tests - "Balapan" and "Degelen" testing sites located in Semipalatinsk Test Site. The paper presents data on the levels and distribution of tritium in the air where tunnels and boreholes are located - explosion epicentres, wellheads and tunnel portals, as well as in estuarine areas of the venues for the underground nuclear explosions (UNE).

Mechanisms for surface contamination of soils and bottom sediments in the Shagan River zone within former Semipalatinsk Nuclear Test Site.

The Shagan River is the only surface watercourse within the former Semipalatinsk Test Site (STS). Research in the valley of the Shagan River was carried out to study the possible migration of artificial radionuclides with surface waters over considerable distances, with the possibility these radionuclides may have entered the Irtysh River. The investigations revealed that radioactive contamination of soil was primarily caused by the first underground nuclear test with soil outburst conducted at the "Balapan" site in Borehole 1004. The surface nuclear tests carried out at the "Experimental Field" site and global fallout made insignificant contributions to contamination. The most polluted is the area in the immediate vicinity of the "Atomic" Lake crater. Contamination at the site is spatial. The total area of contamination is limited to 10-12 km from the crater piles. The ratio of plutonium isotopes was useful to determine the source of soil contamination. There was virtual absence of artificial radionuclide migration with surface waters, and possible cross-border transfer of radionuclides with the waters of Shagan and Irtysh rivers was not confirmed.

Contamination mechanisms of air basin with tritium in venues of underground nuclear explosions at the former Semipalatinsk test site.

During the period of testing from 1945 to 1962 at the territory of Semipalatinsk test site (STS) within the Degelen Mountains in tunnels, 209 underground nuclear explosions were produced. Many of the tunnels have seasonal water seepage in the form of streams, through which tritium migrates from the underground nuclear explosion (UNE) venues towards the surface. The issue of tritium contamination occupies a special place in the radioactive contamination of the environment. In this paper we assess the level and distribution of tritium in the atmospheric air of ecosystems with water seepage at tunnels № 176 and № 177, located on "Degelen" site. There has been presented general nature of tritium distribution in the atmosphere relative to surface of a watercourse which has been contaminated with tritium. The basic mechanisms were studied for tritium distribution in the air of studied ecosystems, namely, the distribution of tritium in the systems: water-atmosphere, tunnel air-atmosphere, soil water-atmosphere, vegetation-atmosphere. An analytical calculation of tritium concentration in the atmosphere by the concentration of tritium in water has been performed. There has experimentally obtained the dependence for predictive assessment of tritium concentrations in air as a function of tritium concentration in one of the inlet sources such as water, tunnel air, soil water, vegetation, etc.. The paper also describes the general nature of tritium distribution in the air in the area "Degelen".