Independent Electrical Control of Two Quantum Dots Coupled through a Photonic-Crystal Waveguide.

Efficient light-matter interaction at the single-photon level is of fundamental importance in emerging photonic quantum technology. A fundamental challenge is addressing multiple quantum emitters at once, as intrinsic inhomogeneities of solid-state platforms require individual tuning of each emitter. We present the realization of two semiconductor quantum dot emitters that are efficiently coupled to a photonic-crystal waveguide and individually controllable by applying a local electric Stark field. We present resonant transmission and fluorescence spectra in order to probe the coupling of the two emitters to the waveguide. We exploit the single-photon stream from one quantum dot to perform spectroscopy on the second quantum dot positioned 16 µm away in the waveguide. Furthermore, power-dependent resonant transmission measurements reveal signatures of coherent coupling between the emitters. Our work provides a scalable route to realizing multiemitter collective coupling, which has inherently been missing for solid-state deterministic photon emitters.

Integrated Whispering-Gallery-Mode Resonator for Solid-State Coherent Quantum Photonics.

Tailored photonics cavities enhance light-matter interactions, ultimately enabling a fully coherent quantum interface. Here, we report an integrated microdisk cavity containing self-assembled quantum dots to coherently route photons between different access waveguides. We measure a Purcell factor of Fexp = 6.9 ± 0.9 for a cavity quality factor of about 10,000, allowing us to observe clear signatures of coherent scattering of photons by the quantum dots. We show how this integrated system can coherently reroute photons between the drop and bus ports and how this routing is controlled by detuning the quantum dot and resonator or through the strength of the excitation beam, where a critical photon number less than one photon per lifetime is required. We discuss the strengths and limitations of this approach, focusing on how the coherent scattering and single-photon nonlinearity can be used to increase the efficiency of quantum devices such as routers or Bell-state analyzers.

Experimental Reconstruction of the Few-Photon Nonlinear Scattering Matrix from a Single Quantum Dot in a Nanophotonic Waveguide.

Coherent photon-emitter interfaces offer a way to mediate efficient nonlinear photon-photon interactions, much needed for quantum information processing. Here we experimentally study the case of a two-level emitter, a quantum dot, coupled to a single optical mode in a nanophotonic waveguide. We carry out few-photon transport experiments and record the statistics of the light to reconstruct the scattering matrix elements of one- and two-photon components. This provides direct insight to the complex nonlinear photon interaction that contains rich many-body physics.

Quantum Optics with Near-Lifetime-Limited Quantum-Dot Transitions in a Nanophotonic Waveguide.

Establishing a highly efficient photon-emitter interface where the intrinsic linewidth broadening is limited solely by spontaneous emission is a key step in quantum optics. It opens a pathway to coherent light-matter interaction for, e.g., the generation of highly indistinguishable photons, few-photon optical nonlinearities, and photon-emitter quantum gates. However, residual broadening mechanisms are ubiquitous and need to be combated. For solid-state emitters charge and nuclear spin noise are of importance, and the influence of photonic nanostructures on the broadening has not been clarified. We present near-lifetime-limited linewidths for quantum dots embedded in nanophotonic waveguides through a resonant transmission experiment. It is found that the scattering of single photons from the quantum dot can be obtained with an extinction of 66 ± 4%, which is limited by the coupling of the quantum dot to the nanostructure rather than the linewidth broadening. This is obtained by embedding the quantum dot in an electrically contacted nanophotonic membrane. A clear pathway to obtaining even larger single-photon extinction is laid out; i.e., the approach enables a fully deterministic and coherent photon-emitter interface in the solid state that is operated at optical frequencies.

Chip-Based All-Optical Control of Single Molecules Coherently Coupled to a Nanoguide.

The feasibility of many proposals in nanoquantum-optics depends on the efficient coupling of photons to individual quantum emitters, the possibility to control this interaction on demand, and the scalability of the experimental platform. To address these issues, we report on chip-based systems made of one-dimensional subwavelength dielectric waveguides (nanoguides) and polycyclic aromatic hydrocarbon molecules. We discuss the design and fabrication requirements, present data on extinction spectroscopy of single molecules coupled to a nanoguide mode, and show how an external optical beam can switch the propagation of light via a nonlinear optical process. The presented architecture paves the way for the investigation of many-body phenomena and polaritonic states and can be readily extended to more complex geometries for the realization of quantum integrated photonic circuits.

Small slot waveguide rings for on-chip quantum optical circuits.

Nanophotonic interfaces between single emitters and light promise to enable new quantum optical technologies. Here, we use a combination of finite element simulations and analytic quantum theory to investigate the interaction of various quantum emitters with slot-waveguide rings. We predict that for rings with radii as small as 1.44 µm, with a Q-factor of 27,900, near-unity emitter-waveguide coupling efficiencies and emission enhancements on the order of 1300 can be achieved. By tuning the ring geometry or introducing losses, we show that realistic emitter-ring systems can be made to be either weakly or strongly coupled, so that we can observe Rabi oscillations in the decay dynamics even for micron-sized rings. Moreover, we demonstrate that slot waveguide rings can be used to directionally couple emission, again with near-unity efficiency. Our results pave the way for integrated solid-state quantum circuits involving various emitters.

Modal symmetries at the nanoscale: a route toward a complete vectorial near-field mapping.

We use symmetry considerations to understand and unravel near-field measurements, ultimately showing that we can spatially map three distinct fields using only two detectors. As an example, we create 2D field maps of the out-of-plane magnetic field and two in-plane fields for a silicon ridge waveguide. Furthermore, we are able to identify and remove polarization mixing of less than 1/30 of our experimental signals. Since symmetries are prevalent in nanophotonic structures and their near-fields, our method can have an impact on many future near-field measurements.

Unravelling nonlinear spectral evolution using nanoscale photonic near-field point-to-point measurements.

We demonstrate nanoscale photonic point-to-point measurements characterizing a single component inside an all-optical signal-processing chip. We perform spectrally resolved near-field scanning optical microscopy on ultrashort pulses propagating inside a slow light photonic crystal waveguide, which is part of a composite sample. A power study reveals a reshaping of the pulse's spectral density, which we model using the nonlinear Schrödinger equation. With the model, we are able to identify the various physical processes governing the nonlinear pulse propagation. Finally, we contrast the near-field measurements with transmission measurements of the complete composite sample to elucidate the importance of gaining local information about the evolution of the spectral density.

Ultrafast tunable optical delay line based on indirect photonic transitions.

We introduce the concept of an indirect photonic transition and demonstrate its use in a dynamic delay line to alter the group velocity of an optical pulse. Operating on an ultrafast time scale, we show continuously tunable delays of up to 20 ps, using a slow light photonic crystal waveguide only 300 µm in length. Our approach is flexible, in that individual pulses in a pulse stream can be controlled independently, which we demonstrate by operating on pulses separated by just 30 ps. The two-step indirect transition is demonstrated here with a 30% conversion efficiency.

All-optical ultrafast control of beaming through a single sub-wavelength aperture in a metal film.

We propose an ultrafast all-optical technique to control and beam the light emerging from a sub-wavelength slit in a planar gold film by exciting a transient grating in the area around the slit. A FDTD model is used to show how excitation of surface plasmon polaritons by the grating governs the beaming process. Both the grating and the beaming effect are shown to decay on a picosecond time-scale. An on-off contrast of 5 dB is obtained for the beaming, with a divergence angle of only 2.4 degrees.

Ultrafast silicon-based active plasmonics at telecom wavelengths.

Using a gold/silicon grating coupler and modulating the silicon dielectric constant with 775 nm, 800 fs pump pulses we demonstrate an ultrafast spectral shift to a surface plasmon polariton coupling resonance for 1300-1700 nm probe pulses. With a modest pump fluence of 2.2 mJ cm(-2) the pump-induced free carriers shift the resonance by more than its width, with recovery occurring in 103 ps due to surface recombination.

Ultrafast all-optical coupling of light to surface plasmon polaritons on plain metal surfaces.

We propose and demonstrate an ultrafast all-optical method to couple light to surface plasmon polaritons on planar gold films. By interfering two 150 fs, 810 nm pulses we excite a transient grating in the temperature of the free electrons of the metal, resulting in a grating in the dielectric function, and leading to a 1 ps launch window for plasmonic excitation. We use pump-probe experiments to identify these ultrashort plasmonic excitations between 520 and 570 nm.

Core-Shell Plasmonic Nanohelices.

We introduce core-shell plasmonic nanohelices, highly tunable structures that have a different response in the visible for circularly polarized light of opposite handedness. The glass core of the helices is fabricated using electron beam induced deposition and the pure gold shell is subsequently sputter coated. Optical measurements allow us to explore the chiral nature of the nanohelices, where differences in the response to circularly polarized light of opposite handedness result in a dissymmetry factor of 0.86, more than twice of what has been previously reported. Both experiments and subsequent numerical simulations demonstrate the extreme tunability of the core-shell structures, where nanometer changes to the geometry can lead to drastic changes of the optical responses. This tunability, combined with the large differential transmission, make core-shell plasmonic nanohelices a powerful nanophotonic tool for, for example, (bio)sensing applications.

Harmonics Generation by Surface Plasmon Polaritons on Single Nanowires.

We present experimental observations of visible wavelength second- and third-harmonic generation on single plasmonic nanowires of variable widths. We identify that near-infrared surface plasmon polaritons, which are guided along the nanowire, act as the source of the harmonics generation. We discuss the underlying mechanism of this nonlinear process, using a combination of spatially resolved measurements and numerical simulations to show that the visible harmonics are generated via a combination of both local and propagating plasmonic modes. Our results provide the first demonstration of nanoscale nonlinear optics with guided, propagating plasmonic modes on a lithographically defined chip, opening up new routes toward integrated optical circuits for information processing.

Ultracompact (3 µm) silicon slow-light optical modulator.

Wavelength-scale optical modulators are essential building blocks for future on-chip optical interconnects. Any modulator design is a trade-off between bandwidth, size and fabrication complexity, size being particularly important as it determines capacitance and actuation energy. Here, we demonstrate an interesting alternative that is only 3 µm long, only uses silicon on insulator (SOI) material and accommodates several nanometres of optical bandwidth at 1550 nm. The device is based on a photonic crystal waveguide: by combining the refractive index shift with slow-light enhanced absorption induced by free-carrier injection, we achieve an operation bandwidth that significantly exceeds the shift of the bandedge. We compare a 3 µm and an 80 µm long modulator and surprisingly, the shorter device outperforms the longer one. Despite its small size, the device achieves an optical bandwidth as broad as 7 nm for an extinction ratio of 10 dB, and modulation times ranging between 500 ps and 100 ps.

Ultrafast control of grating-assisted light coupling to surface plasmons.

We demonstrate subpicosecond control over the coupling of free-space radiation to surface-plasmon polaritons using 830 and 500 nm period gold gratings. Thermal changes to the electron distribution following irradiation by 100 fs, 810 nm pulses produce a shift of the 570 nm plasmon resonance by approximately 0.75 nm with reflectivity change up to 6% and decay time of approximately 1 ps.