Entanglement distribution over a 96-km-long submarine optical fiber.

Quantum entanglement is one of the most extraordinary effects in quantum physics, with many applications in the emerging field of quantum information science. In particular, it provides the foundation for quantum key distribution (QKD), which promises a conceptual leap in information security. Entanglement-based QKD holds great promise for future applications owing to the possibility of device-independent security and the potential of establishing global-scale quantum repeater networks. While other approaches to QKD have already reached the level of maturity required for operation in absence of typical laboratory infrastructure, comparable field demonstrations of entanglement-based QKD have not been performed so far. Here, we report on the successful distribution of polarization-entangled photon pairs between Malta and Sicily over 96 km of submarine optical telecommunications fiber. We observe around 257 photon pairs per second, with a polarization visibility above 90%. Our results show that QKD based on polarization entanglement is now indeed viable in long-distance fiber links. This field demonstration marks the longest-distance distribution of entanglement in a deployed telecommunications network and demonstrates an international submarine quantum communication channel. This opens up myriad possibilities for future experiments and technological applications using existing infrastructure.

Proximitized Josephson junctions in highly-doped InAs nanowires robust to optical illumination.

We have studied the effects of optical-frequency light on proximitized InAs/Al Josephson junctions based on highly n-doped InAs nanowires at varying incident photon flux and at three different photon wavelengths. The experimentally obtained IV curves were modeled using a resistively shunted junction model which takes scattering at the contact interfaces into account. Despite the fact that the InAs weak link is photosensitive, the Josephson junctions were found to be surprisingly robust, interacting with the incident radiation only through heating, whereas above the critical current our devices showed non-thermal effects resulting from photon exposure. Our work indicates that Josephson junctions based on highly-doped InAs nanowires can be integrated in close proximity to photonic circuits. The results also suggest that such junctions can be used for optical-frequency photon detection through thermal processes by measuring a shift in critical current.

Semiconductor devices for entangled photon pair generation: a review.

Entanglement is one of the most fascinating properties of quantum mechanical systems; when two particles are entangled the measurement of the properties of one of the two allows the properties of the other to be instantaneously known, whatever the distance separating them. In parallel with fundamental research on the foundations of quantum mechanics performed on complex experimental set-ups, we assist today with bourgeoning of quantum information technologies bound to exploit entanglement for a large variety of applications such as secure communications, metrology and computation. Among the different physical systems under investigation, those involving photonic components are likely to play a central role and in this context semiconductor materials exhibit a huge potential in terms of integration of several quantum components in miniature chips. In this article we review the recent progress in the development of semiconductor devices emitting entangled photons. We will present the physical processes allowing the generation of entanglement and the tools to characterize it; we will give an overview of major recent results of the last few years and highlight perspectives for future developments.

Significant-Loophole-Free Test of Bell's Theorem with Entangled Photons.

Local realism is the worldview in which physical properties of objects exist independently of measurement and where physical influences cannot travel faster than the speed of light. Bell's theorem states that this worldview is incompatible with the predictions of quantum mechanics, as is expressed in Bell's inequalities. Previous experiments convincingly supported the quantum predictions. Yet, every experiment requires assumptions that provide loopholes for a local realist explanation. Here, we report a Bell test that closes the most significant of these loopholes simultaneously. Using a well-optimized source of entangled photons, rapid setting generation, and highly efficient superconducting detectors, we observe a violation of a Bell inequality with high statistical significance. The purely statistical probability of our results to occur under local realism does not exceed 3.74×10^{-31}, corresponding to an 11.5 standard deviation effect.

Room-temperature laser emission of ZnO nanowires explained by many-body theory.

Are excitons involved in lasing in ZnO nanowires or not? Our recently developed and experimentally tested quantum many-body theory sheds new light on this question. We measured the laser thresholds and Fabry-Pérot laser modes for three radically different excitation schemes. The thresholds, photon energies, and mode spacings can all be explained by our theory, without invoking enhanced light-matter interaction, as is needed in an earlier excitonic model. Our conclusion is that lasing in ZnO nanowires at room temperature is not of excitonic nature, as is often thought, but instead is electron-hole plasma lasing.

Ultrafast all-optical shutter based on two-photon absorption.

An ultrafast all-optical shutter is presented, based on a simple two-color, two-photon absorption technique. For time-resolved luminescence measurements, this shutter is an interesting alternative to the optical Kerr gate. The rejection efficiency is 99%; the switching-off and switching-on speeds are limited by the pulse length only; the rejection time is determined by the crystal slab thickness; and the bandwidth spans the entire visible spectrum. We show that our shutter can also be used for accurate measurement of group velocity inside a transparent material.

Exciton Fine Structure and Lattice Dynamics in InP/ZnSe Core/Shell Quantum Dots.

Nanocrystalline InP quantum dots (QDs) hold promise for heavy-metal-free optoelectronic applications due to their bright and size-tunable emission in the visible range. Photochemical stability and high photoluminescence (PL) quantum yield are obtained by a diversity of epitaxial shells around the InP core. To understand and optimize the emission line shapes, the exciton fine structure of InP core/shell QD systems needs be investigated. Here, we study the exciton fine structure of InP/ZnSe core/shell QDs with core diameters ranging from 2.9 to 3.6 nm (PL peak from 2.3 to 1.95 eV at 4 K). PL decay measurements as a function of temperature in the 10 mK to 300 K range show that the lowest exciton fine structure state is a dark state, from which radiative recombination is assisted by coupling to confined acoustic phonons with energies ranging from 4 to 7 meV, depending on the core diameter. Circularly polarized fluorescence line-narrowing (FLN) spectroscopy at 4 K under high magnetic fields (up to 30 T) demonstrates that radiative recombination from the dark F = ±2 state involves acoustic and optical phonons, from both the InP core and the ZnSe shell. Our data indicate that the highest intensity FLN peak is an acoustic phonon replica rather than a zero-phonon line, implying that the energy separation observed between the F = ±1 state and the highest intensity peak in the FLN spectra (6 to 16 meV, depending on the InP core size) is larger than the splitting between the dark and bright fine structure exciton states.

Erratum: Bright nanoscale source of deterministic entangled photon pairs violating Bell's inequality.

A correction to this article has been published and is linked from the HTML version of this paper. The error has been fixed in the paper.

Bright nanoscale source of deterministic entangled photon pairs violating Bell's inequality.

Global, secure quantum channels will require efficient distribution of entangled photons. Long distance, low-loss interconnects can only be realized using photons as quantum information carriers. However, a quantum light source combining both high qubit fidelity and on-demand bright emission has proven elusive. Here, we show a bright photonic nanostructure generating polarization-entangled photon pairs that strongly violates Bell's inequality. A highly symmetric InAsP quantum dot generating entangled photons is encapsulated in a tapered nanowire waveguide to ensure directional emission and efficient light extraction. We collect ~200 kHz entangled photon pairs at the first lens under 80 MHz pulsed excitation, which is a 20 times enhancement as compared to a bare quantum dot without a photonic nanostructure. The performed Bell test using the Clauser-Horne-Shimony-Holt inequality reveals a clear violation (S CHSH > 2) by up to 9.3 standard deviations. By using a novel quasi-resonant excitation scheme at the wurtzite InP nanowire resonance to reduce multi-photon emission, the entanglement fidelity (F = 0.817 ± 0.002) is further enhanced without temporal post-selection, allowing for the violation of Bell's inequality in the rectilinear-circular basis by 25 standard deviations. Our results on nanowire-based quantum light sources highlight their potential application in secure data communication utilizing measurement-device-independent quantum key distribution and quantum repeater protocols.

Observation of strongly entangled photon pairs from a nanowire quantum dot.

A bright photon source that combines high-fidelity entanglement, on-demand generation, high extraction efficiency, directional and coherent emission, as well as position control at the nanoscale is required for implementing ambitious schemes in quantum information processing, such as that of a quantum repeater. Still, all of these properties have not yet been achieved in a single device. Semiconductor quantum dots embedded in nanowire waveguides potentially satisfy all of these requirements; however, although theoretically predicted, entanglement has not yet been demonstrated for a nanowire quantum dot. Here, we demonstrate a bright and coherent source of strongly entangled photon pairs from a position-controlled nanowire quantum dot with a fidelity as high as 0.859±0.006 and concurrence of 0.80±0.02. The two-photon quantum state is modified via the nanowire shape. Our new nanoscale entangled photon source can be integrated at desired positions in a quantum photonic circuit, single-electron devices and light-emitting diodes.