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We demonstrate that chirped pulse up-conversion (CPU), a method routinely used with systems based on 1-kHz Titanium:Sapphire lasers, can be extended to a repetition rate of 100 kHz with an Ytterbium diode-pumped femtosecond amplifier. Individual mid-infrared spectra can thus be measured directly in the near infrared using a fast CMOS linescan camera. After an appropriate Fourier processing, a spectral resolution of 1.1 cm-1 is reported, currently limited by our spectrometer. Additionally, we demonstrate the application of CPU to a pump-probe measurement of the vibrational relaxation in carboxy-hemoglobin, and we show that the combination of fast scanning and fast acquisition enables a straightforward removal of pump scattering interference.
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Femtosecond laser sources with high repetition rate in the ultraviolet (UV) and vacuum UV (VUV) are fundamental tools enabling tabletop time-resolved and angle-resolved photoemission spectroscopy in solids. We describe a VUV source at 114 nm (10.8 eV) based on an industrial grade ytterbium-doped ultrafast laser, a nonlinear pulse width selection stage, and two cascaded frequency tripling stages, first in crystals, second in xenon. The role of ionization in gas-based perturbative third harmonic generation phase-matching is analyzed using a simple theory, numerical simulations, and experimental data. The source features high photon flux, high repetition rate, and adjustable time resolutions. Thereby, in combination with a state-of-the-art angle-resolved photoemission spectroscopy (ARPES) apparatus it enables the study of the electronic dynamics of the whole Brillouin zone in a large number of materials.
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We report about a setup for carrier-envelope phase (CEP) control and stabilization in passive systems based on difference frequency generation (DFG). The principle of this approach relies on the amplitude to phase modulation transfer in the white-light generation process. A small modulation of the pump laser intensity is used to obtain a DFG output modulated in CEP. This technique is demonstrated in a CEP-stable system pumped by an Yb-doped fiber amplifier. It is first characterized by measuring CEP modulations produced by applying arbitrary waveforms. The CEP actuator is then used for slow drifts correction in a feedback loop. The results show the capability of this simple approach for OPA/OPCPA CEP-stabilized setups.
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We present an efficient and robust scheme to produce energetic sub-15 fs pulses centered at 515 nm with a peak power exceeding 3 GW. Combining efficient second-harmonic generation of a 135 fs, 50 W Yb-doped fiber amplifier with a low-loss capillary-based visible pulse compression stage, we reach an overall efficiency higher than >20%. The system is also designed to take advantage of the repetition rate flexibility of the fiber amplifier, leading sub-15 fs pulse generation from 166 to 500 kHz with an average power exceeding the 10 watt level. The combined reduction of the laser wavelength and pulse duration is expected to highly improve the yield of high-order harmonic generation to provide high photon flux of ultrashort extreme ultraviolet radiation.
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Starting from a femtosecond ytterbium-doped fiber amplifier, we demonstrate the generation of near Fourier transform-limited high peak power picosecond pulses through spectral compression in a nonlinear solid-state-based multipass cell. Input 260 fs pulses negatively chirped to 2.4 ps are spectrally compressed from 6 nm down to 1.1 nm, with an output energy of 13.5 µJ and near transform-limited pulses of 2.1 ps. A pulse shaper included in the femtosecond source provides some control over the output spectral shape, in particular its symmetry. The spatial quality and spatio-spectral homogeneity are conserved in this process. These results show that the use of multipass cells allows energy scaling of spectral compression setups while maintaining the spatial properties of the laser beam.
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A hybrid-system approach using a low-gain Yb:YAG single crystal booster amplifier behind a state-of-the-art industrial high-power femtosecond fiber system is studied to significantly increase the output pulse energy of the fiber amplifier. With this system, more than 60 W of average power is demonstrated at 100 kHz for pulse duration of 400 fs, corresponding to an energy per pulse of 600 µJ. Reducing the repetition rate, the energy is increased up to 2.5 mJ (before compression), which corresponds to the limitation due to laser damage threshold of the optical coatings. To scale further the energy, passive divided-pulse amplification is then implemented at the entrance of the bulk amplifier. Using this geometry, a safe nominal operating point is presented with output pulse energies of 3 mJ before and 2.3 mJ after compression and with a pulse duration of 520 fs, corresponding to a peak power of 4.4 GW.
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We propose and demonstrate an OPCPA architecture emitting few-cycle pulses at 3070 nm and 1550 nm based on a high-energy femtosecond ytterbium-doped fiber amplifier pump. The short pump pulse duration allows direct seeding by a supercontinuum in the 1.4 - 1.7 µm signal range, generated in bulk YAG. It also allows a simplified dispersion management along the system and broad optical gain bandwidth. The dual output system delivers 20 µJ, 49 fs signal pulses at 1550 nm and 10 µJ, 72 fs idler pulses at 3070 nm. Power scaling limitations due to beam distortion in the last MgO:PPLN-based OPCPA stage are discussed and investigated.
RESUMO
We report on the generation of 34 fs and 50 µJ pulses from a high energy fiber amplifier system with nonlinear compression in an air-filled hypocycloid-core Kagome fiber. The unique properties of such fibers allow bridging the gap between solid core fibers-based and hollow capillary-based post-compression setups, thereby operating with pulse energies obtained with current state-of-the-art fiber systems. The overall transmission of the compression setup is over 70%. Together with Yb-doped fiber amplifier technologies, Kagome fibers therefore appear as a promising tool for efficient generation of pulses with durations below 50 fs, energies ranging from 10 to several hundreds of µJ, and high average powers.
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Active coherent beam combination using a 7-non-coupled core, polarization maintaining, air-clad, Yb-doped fiber is demonstrated as a monolithic and compact power-scaling concept for ultrafast fiber lasers. A microlens array matched to the multicore fiber and an active phase controller composed of a spatial light modulator applying a stochastic parallel gradient descent algorithm are utilized to perform coherent combining in the tiled aperture geometry. The mitigation of nonlinear effects at a pulse energy of 8.9 µJ and duration of 860 fs is experimentally verified at a repetition rate of 100 kHz. The experimental combining efficiency results in a far field central lobe carrying 49% of the total power, compared to an ideal value of 76%. This efficiency is primarily limited by group delay differences between cores which is identified as the main drawback of the system. Minimizing these group delay issues, e.g. by using short and straight rod-type multicore fibers, should allow a practical power scaling solution for femtosecond fiber systems.
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We report on the generation of 1.1-mJ, 300-fs pulses at 50 kHz by implementing an amplifier architecture whereby four stretched pulse replicas are created in the temporal and spatial domains, allowing pulse energy scaling by the same factor. The whole spatiotemporal coherent combining geometry is passive, avoiding the need for active electronic stabilization loop systems. The combining efficiency remains above 90% at all power levels.
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We report the measurement of spectral and spatial correlations in supercontinua generated by focusing microjoule pulses from a femtosecond ytterbium-doped fiber amplifier laser in bulk YAG. The measurement is full-bandwidth at a repetition rate of 1 MHz owing to the use of time-stretch dispersive Fourier transform technique. In contrast with fiber-based supercontinuum generation, our results show an excellent stability of the spectral and spatial properties of the output supercontinuum, with an essentially correlated behavior in the 1.4-1.7 µm wavelength range. These results provide strong ground for the development of supercontinuum-seeded ultrafast optical parametric amplifier systems in the mid-infrared using ytterbium lasers as pump sources.
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A hybrid ytterbium-doped fiber-bulk laser source allowing the generation of 3 ps, 350 µJ, 116 MW peak power Fourier transform-limited pulses at 50 kHz repetition rate and 1030 nm wavelength is described. Pulse duration tunability is provided by an adjustable spectral compression-based seeder system. Energy scaling capabilities of the architecture by use of the divided-pulse amplification method are investigated. This source provides a robust, compact, and versatile solution for applications such as RF photocathode guns, x- and γ-ray generation by inverse Compton scattering, and optical parametric chirped-pulse amplification pumping.
RESUMO
Passive spatial and temporal coherent combining schemes are implemented to scale the output energy of a nonlinear temporal compression setup. By generating 32 replicas of the incident femtosecond pulses, the output of a high-energy fiber chirped-pulse amplifier can be compressed using self-phase modulation in a large-mode-area rod-type fiber at peak-power levels well beyond the self-focusing power. We demonstrate the generation of 71 fs 7.5 µJ pulses at 100 kHz repetition rate, corresponding to a peak power of 86 MW.
RESUMO
We report on the first diode-pumped Yb:CaGdAlO4 regenerative amplifier in the sub-100-fs regime. It generates pulses at a central wavelength of 1047 nm with up to 24 µJ energy (after compression) at a repetition rate of 50 kHz. The measured pulse duration is 97 fs, with a spectral bandwidth of 19 nm. We describe in detail how nonlinear effects are optimally used to compensate gain narrowing in order to overcome the 100 fs barrier.
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We demonstrate spectral coherent beam combining of two femtosecond fiber chirped-pulse amplifiers seeded by a common oscillator. Using active phase stabilization based on an electro-optic phase modulator, an average power of 10 W before compression and a high gain factor of 30 dB are obtained. At this gain value, 130 fs pulses with a spectral width of 19 nm can be generated, highlighting the strong potential of pulse synthesis for the reduction of the minimum duration of ultrashort pulses in fiber chirped-pulse amplifiers.
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We implement both chirped pulse amplification and divided pulse amplification in the same femtosecond fiber amplifier setup. This scheme allows an equivalent stretched pulse duration of 2.4 ns in a compact tabletop system. The generation of 77 W of compressed average power at 4.8 MHz, together with 320 fs and 430 µJ pulses at a repetition rate of 96 kHz, is demonstrated using a distributed mode-filtering, rod-type, ytterbium-doped fiber. Limitations in the temporal recombining efficiency due to gain saturation inside the fiber amplifier are identified.
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We demonstrate a versatile femtosecond power amplifier using a Yb:YAG single crystal fiber operating from 10 kHz to 10 MHz. For a total pump power of 75 W, up to 30 W is generated from the double-pass power amplifier. At a repetition rate of 10 kHz, an output energy of 1 mJ is obtained after recompression. In this configuration, the pulse duration is 380 fs, corresponding to a peak power of 2.2 GW. The M2 beam quality factor is better than 1.1 for investigated parameters.
RESUMO
We propose and demonstrate an architecture that achieves passive coherent combination of two femtosecond fiber chirped-pulse amplifiers. The setup consists in the use of a well-balanced amplifying Sagnac interferometer. The experiment shows that the temporal, spectral, and spatial qualities of each beam are retained, with the generation of 250 fs pulses at 35 MHz repetition rate, an uncompressed average power of 10 W, and a combining efficiency of 96%. The behavior of this architecture in the presence of high accumulated nonlinear phase is investigated.
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We demonstrated that Yb:YAG single crystal fibers have a strong potential for the amplification of femtosecond pulses. Seeded by 230 fs pulses with an average power of 400 mW at 30 MHz delivered by a passively mode-locked Yb:KYW oscillator, the system produced 330 fs pulses with an average power of 12 W. This is the shortest pulse duration ever produced by an Yb:YAG amplifier. The gain in the single crystal fiber reached a value as high as 30 in a simple double-pass configuration.
RESUMO
We report the use of cross-polarized wave generation to perform both pulse shortening and temporal cleaning of a high-energy ytterbium-doped fiber-based femtosecond laser system. The nonlinear processes allow both a highly efficient nonlinear conversion of 20% and a large compression ratio of 3.5, with inherently improved coherent and incoherent contrasts. This results in the generation of 37 µJ, 115 fs pulses at a repetition rate of 100 kHz with high temporal quality.