Experimental Analysis of Energy Transfers between a Quantum Emitter and Light Fields.

Energy can be transferred between two quantum systems in two forms: unitary energy-that can be used to drive another system-and correlation energy-that reflects past correlations. We propose and implement experimental protocols to access these energy transfers in interactions between a quantum emitter and light fields. Upon spontaneous emission, we measure the unitary energy transfer from the emitter to the light field and show that it never exceeds half the total energy transfer and is reduced when introducing decoherence. We then study the interference of the emitted field and a coherent laser field at a beam splitter and show that the nature of the energy transfer quantitatively depends on the quantum purity of the emitted field.

Energetics of a Single Qubit Gate.

Qubits are physical, a quantum gate thus not only acts on the information carried by the qubit but also on its energy. What is then the corresponding flow of energy between the qubit and the controller that implements the gate? Here we exploit a superconducting platform to answer this question in the case of a quantum gate realized by a resonant drive field. During the gate, the superconducting qubit becomes entangled with the microwave drive pulse so that there is a quantum superposition between energy flows. We measure the energy change in the drive field conditioned on the outcome of a projective qubit measurement. We demonstrate that the drive's energy change associated with the measurement backaction can exceed by far the energy that can be extracted by the qubit. This can be understood by considering the qubit as a weak measurement apparatus of the driving field.

Steady State Entanglement beyond Thermal Limits.

Classical engines turn thermal resources into work, which is maximized for reversible operations. The quantum realm has expanded the range of useful operations beyond energy conversion, and incoherent resources beyond thermal reservoirs. This is the case of entanglement generation in a driven-dissipative protocol, which we hereby analyze as a continuous quantum machine. We show that for such machines the more irreversible the process, the larger the concurrence. Maximal concurrence and entropy production are reached for the hot reservoir being at negative effective temperature, beating the limits set by classic thermal operations on an equivalent system.

What is quantum in quantum randomness?

It is often said that quantum and classical randomness are of different nature, the former being ontological and the latter epistemological. However, so far the question of 'What is quantum in quantum randomness?', i.e. what is the impact of quantization and discreteness on the nature of randomness, remains to be answered. In a first part, we make explicit the differences between quantum and classical randomness within a recently proposed ontology for quantum mechanics based on contextual objectivity. In this view, quantum randomness is the result of contextuality and quantization. We show that this approach strongly impacts the purposes of quantum theory as well as its areas of application. In particular, it challenges current programmes inspired by classical reductionism, aiming at the emergence of the classical world from a large number of quantum systems. In a second part, we analyse quantum physics and thermodynamics as theories of randomness, unveiling their mutual influences. We finally consider new technological applications of quantum randomness that have opened up in the emerging field of quantum thermodynamics.This article is part of a discussion meeting issue 'Foundations of quantum mechanics and their impact on contemporary society'.

Reducing Phonon-Induced Decoherence in Solid-State Single-Photon Sources with Cavity Quantum Electrodynamics.

Solid-state emitters are excellent candidates for developing integrated sources of single photons. Yet, phonons degrade the photon indistinguishability both through pure dephasing of the zero-phonon line and through phonon-assisted emission. Here, we study theoretically and experimentally the indistinguishability of photons emitted by a semiconductor quantum dot in a microcavity as a function of temperature. We show that a large coupling to a high quality factor cavity can simultaneously reduce the effect of both phonon-induced sources of decoherence. It first limits the effect of pure dephasing on the zero-phonon line with indistinguishabilities above 97% up to 18 K. Moreover, it efficiently redirects the phonon sidebands into the zero-phonon line and brings the indistinguishability of the full emission spectrum from 87% (24%) without cavity effect to more than 99% (76%) at 0K (20K). We provide guidelines for optimal cavity designs that further minimize the phonon-induced decoherence.

Strain-Gradient Position Mapping of Semiconductor Quantum Dots.

We introduce a nondestructive method to determine the position of randomly distributed semiconductor quantum dots (QDs) integrated in a solid photonic structure. By setting the structure in an oscillating motion, we generate a large stress gradient across the QDs plane. We then exploit the fact that the QDs emission frequency is highly sensitive to the local material stress to map the position of QDs deeply embedded in a photonic wire antenna with an accuracy ranging from ±35 nm down to ±1 nm. In the context of fast developing quantum technologies, this technique can be generalized to different photonic nanostructures embedding any stress-sensitive quantum emitters.

Observing interferences between past and future quantum states in resonance fluorescence.

The fluorescence of a resonantly driven superconducting qubit is measured in the time domain, providing a weak probe of the qubit dynamics. Prior preparation and final, single-shot measurement of the qubit allows us to average fluorescence records conditionally on past and future knowledge. The resulting interferences reveal purely quantum features characteristic of weak values. We demonstrate conditional averages that go beyond classical boundaries and probe directly the jump operator associated with relaxation. The experimental results are remarkably captured by a recent theory, which generalizes quantum mechanics to open quantum systems whose past and future are known.

Fabry-Perot interferometer with quantum mirrors: nonlinear light transport and rectification.

Optical transport represents a natural route towards fast communications, and it is currently used in large scale data transfer. The progressive miniaturization of devices for information processing calls for the microscopic tailoring of light transport and confinement at length scales appropriate for upcoming technologies. With this goal in mind, we present a theoretical analysis of a one-dimensional Fabry-Perot interferometer built with two highly saturable nonlinear mirrors: a pair of two-level systems. Our approach captures nonlinear and nonreciprocal effects of light transport that were not reported previously. Remarkably, we show that such an elementary device can operate as a microscopic integrated optical rectifier.

Hybrid quantum circuit with a superconducting qubit coupled to a spin ensemble.

We report the experimental realization of a hybrid quantum circuit combining a superconducting qubit and an ensemble of electronic spins. The qubit, of the transmon type, is coherently coupled to the spin ensemble consisting of nitrogen-vacancy centers in a diamond crystal via a frequency-tunable superconducting resonator acting as a quantum bus. Using this circuit, we prepare a superposition of the qubit states that we store into collective excitations of the spin ensemble and retrieve back into the qubit later on. These results constitute a proof of concept of spin-ensemble based quantum memory for superconducting qubits.

Strong coupling of a spin ensemble to a superconducting resonator.

We report the realization of a quantum circuit in which an ensemble of electronic spins is coupled to a frequency tunable superconducting resonator. The spins are nitrogen-vacancy centers in a diamond crystal. The achievement of strong coupling is manifested by the appearance of a vacuum Rabi splitting in the transmission spectrum of the resonator when its frequency is tuned through the nitrogen-vacancy center electron spin resonance.

Coherent manipulation of a solid-state artificial atom with few photons.

In a quantum network based on atoms and photons, a single atom should control the photon state and, reciprocally, a single photon should allow the coherent manipulation of the atom. Both operations require controlling the atom environment and developing efficient atom-photon interfaces, for instance by coupling the natural or artificial atom to cavities. So far, much attention has been drown on manipulating the light field with atomic transitions, recently at the few-photon limit. Here we report on the reciprocal operation and demonstrate the coherent manipulation of an artificial atom by few photons. We study a quantum dot-cavity system with a record cooperativity of 13. Incident photons interact with the atom with probability 0.95, which radiates back in the cavity mode with probability 0.96. Inversion of the atomic transition is achieved for 3.8 photons on average, showing that our artificial atom performs as if fully isolated from the solid-state environment.

Strain-mediated coupling in a quantum dot-mechanical oscillator hybrid system.

Recent progress in nanotechnology has allowed the fabrication of new hybrid systems in which a single two-level system is coupled to a mechanical nanoresonator. In such systems the quantum nature of a macroscopic degree of freedom can be revealed and manipulated. This opens up appealing perspectives for quantum information technologies, and for the exploration of the quantum-classical boundary. Here we present the experimental realization of a monolithic solid-state hybrid system governed by material strain: a quantum dot is embedded within a nanowire that features discrete mechanical resonances corresponding to flexural vibration modes. Mechanical vibrations result in a time-varying strain field that modulates the quantum dot transition energy. This approach simultaneously offers a large light-extraction efficiency and a large exciton-phonon coupling strength g0. By means of optical and mechanical spectroscopy, we find that g0/2 π is nearly as large as the mechanical frequency, a criterion that defines the ultrastrong coupling regime.

Rabi oscillations revival induced by time reversal: a test of mesoscopic quantum coherence.

Using an echo technique proposed by Morigi et al., we have time-reversed the atom-field interaction in a cavity quantum electrodynamics experiment. The collapse of the atomic Rabi oscillation in a coherent field is reversed, resulting in an induced revival signal. The amplitude of this "echo" is sensitive to nonunitary decoherence processes. Its observation demonstrates the existence of a mesoscopic quantum superposition of field states in the cavity between the collapse and the revival times.

Nondestructive Rydberg atom counting with mesoscopic fields in a cavity.

We present an efficient, state-selective, nondemolition atom-counting procedure based on the dispersive interaction of a sample of circular Rydberg atoms with a mesoscopic field contained in a high-quality superconducting cavity. The state-dependent atomic index of refraction, proportional to the atom number, shifts the classical field phase. A homodyne procedure translates the information from the phase to the intensity. The final field intensity is readout by a mesoscopic atomic sample. This method opens promising routes for quantum information processing and nonclassical state generation with Rydberg atoms.

Direct measurement of the Wigner function of a one-photon Fock state in a cavity.

We have measured the complete Wigner function W of the vacuum and of a single-photon state for a field stored in a high-Q cavity. This experiment implements the direct Lutterbach and Davidovich method [L. G. Lutterbach and L. Davidovich, Phys. Rev. Lett. 78, 2547 (1997)]] and is based on the dispersive interaction of a single circular Rydberg atom with the cavity field. The nonclassical nature of the single-photon field is exhibited by a region of negative W values. Extensions to other nonclassical cavity field states are discussed.

Generating and probing a two-photon fock state with a single atom in a cavity.

A two-photon Fock state is prepared in a cavity sustaining a "source mode" and a "target mode," with a single circular Rydberg atom. In a third-order Raman process, the atom emits a photon in the target while scattering one photon from the source into the target. The final two-photon state is probed by measuring by Ramsey interferometry the cavity light shifts induced by the target field on the same atom. Extensions to other multiphoton processes and to a new type of micromaser are briefly discussed.

Coherent control of an atomic collision in a cavity.

Following a recent proposal by S. B. Zheng and G. C. Guo [Phys. Rev. Lett. 85, 2392 (2000)], we report an experiment in which two Rydberg atoms crossing a nonresonant cavity are entangled by coherent energy exchange. The process, mediated by the virtual emission and absorption of a microwave photon, is characterized by a collision mixing angle 4 orders of magnitude larger than for atoms colliding in free space with the same impact parameter. The final entangled state is controlled by adjusting the atom-cavity detuning. This procedure, essentially insensitive to thermal fields and to photon decay, opens promising perspectives for complex entanglement manipulations.

A complementarity experiment with an interferometer at the quantum-classical boundary.

To illustrate the quantum mechanical principle of complementarity, Bohr described an interferometer with a microscopic slit that records the particle's path. Recoil of the quantum slit causes it to become entangled with the particle, resulting in a kind of Einstein-Podolsky-Rosen pair. As the motion of the slit can be observed, the ambiguity of the particle's trajectory is lifted, suppressing interference effects. In contrast, the state of a sufficiently massive slit does not depend on the particle's path; hence, interference fringes are visible. Although many experiments illustrating various aspects of complementarity have been proposed and realized, none has addressed the quantum-classical limit in the design of the interferometer. Here we report an experimental investigation of complementarity using an interferometer in which the properties of one of the beam-splitting elements can be tuned continuously from being effectively microscopic to macroscopic. Following a recent proposal, we use an atomic double-pulse Ramsey interferometer, in which microwave pulses act as beam-splitters for the quantum states of the atoms. One of the pulses is a coherent field stored in a cavity, comprising a small, adjustable mean photon number. The visibility of the interference fringes in the final atomic state probability increases with this photon number, illustrating the quantum to classical transition.

Entanglement of a mesoscopic field with an atom induced by photon graininess in a cavity.

We observe that a mesoscopic field made of several tens of microwave photons exhibits quantum features when interacting with a single Rydberg atom in a high-Q cavity. The field is split into two components whose phases differ by an angle inversely proportional to the square root of the average photon number. The field and the atomic dipole are phase entangled. These manifestations of photon graininess vanish at the classical limit. This experiment opens the way to studies of large quantum state superpositions at the quantum-classical boundary.