Multiple quantum criticality in a two-dimensional superconductor.

The diverse phenomena associated with the two-dimensional electron gas (2DEG) that occurs at oxide interfaces include, among others, exceptional carrier mobilities, magnetism and superconductivity. Although these have mostly been the focus of interest for potential future applications, they also offer an opportunity for studying more fundamental quantum many-body effects. Here, we examine the magnetic-field-driven quantum phase transition that occurs in electrostatically gated superconducting LaTiO3/SrTiO3 interfaces. Through a finite-size scaling analysis, we show that it belongs to the (2+1)D XY model universality class. The system can be described as a disordered array of superconducting puddles coupled by a 2DEG and, depending on its conductance, the observed critical behaviour is single (corresponding to the long-range phase coherence in the whole array) or double (one related to local phase coherence, the other one to the array). A phase diagram illustrating the dependence of the critical field on the 2DEG conductance is constructed, and shown to agree with theoretical proposals. Moreover, by retrieving the coherence-length critical exponent ν, we show that the quantum critical behaviour can be clean or dirty according to the Harris criterion, depending on whether the phase-coherence length is smaller or larger than the size of the puddles.

Solar blind photoconductivity in three-terminal devices of LaAlO3/SrTiO3 heterostructures.

We report observations of photoconductivity in ultrathin films of LaAlO(3) grown on (001) SrTiO(3) at several deposition temperatures. The films show pronounced metallic behavior in the dark. The conductance of this metallic state can be enhanced by ultraviolet light (350-400 nm) of a few µW/cm(2) intensity. The decay of the photoconducting state follows stretched exponential dynamics, which can be accelerated or slowed down on the application of gate voltage, thus imparting a novel functionality to the system.

Two-dimensional superconducting phase in LaTiO3/SrTiO3 heterostructures induced by high-mobility carrier doping.

In this Letter, we show that a superconducting two-dimensional electron gas is formed at the LaTiO3/SrTiO3 interface whose transition temperature can be modulated by a back-gate voltage. The gas consists of two types of carriers: a majority of low-mobility carriers always present, and a few high-mobility ones that can be injected by electrostatic doping. The calculation of the electron spatial distribution in the confinement potential shows that the high-mobility electrons responsible for superconductivity set at the edge of the gas whose extension can be tuned by the field effect.

Simultaneous Observation of Columnar Defects and Magnetic Flux Lines in High-Temperature Bi2Sr2CaCu2O8 Superconductors.

Columnar defects generated by heavy-ion irradiation are promising structures for pinning magnetic flux lines and enhancing critical currents in superconductors with high transition temperatures. An approach that combines chemical etching and magnetic decoration was used to highlight simultaneously the distributions of columnar defects and magnetic flux lines in Bi(2)Sr(2)CaCu(2)O(8) superconductors. Analyses of images of the columnar defects and flux-line positions provide insight into flux-line pinning by elucidating (i) the occupancy of columnar defects by flux lines, (ii) the nature of topological defects in the flux-line lattice, and (iii) the translational and orientational order in this lattice.

Competition between electron pairing and phase coherence in superconducting interfaces.

In LaAlO3/SrTiO3 heterostructures, a gate tunable superconducting electron gas is confined in a quantum well at the interface between two insulating oxides. Remarkably, the gas coexists with both magnetism and strong Rashba spin-orbit coupling. However, both the origin of superconductivity and the nature of the transition to the normal state over the whole doping range remain elusive. Here we use resonant microwave transport to extract the superfluid stiffness and the superconducting gap energy of the LaAlO3/SrTiO3 interface as a function of carrier density. We show that the superconducting phase diagram of this system is controlled by the competition between electron pairing and phase coherence. The analysis of the superfluid density reveals that only a very small fraction of the electrons condenses into the superconducting state. We propose that this corresponds to the weak filling of high-energy dxz/dyz bands in the quantum well, more apt to host superconductivity.

Crossover from magnetostatic to exchange coupling in La0.67Ca0.33MnO3/YBa2Cu3O7/La0.67Ca0.33MnO3 heterostructures.

The influence of YBa2Cu3O7 (YBCO) superconductor layer (S-layer) with a varying thickness d YBCO = 20-50 nm on the magnetic coupling between two La0.67Ca0.33MnO3 (LCMO) ferromagnet layers (F-layer, thickness d LCMO = 50 nm) in F/S/F heterostructures (HSs) was investigated by measuring global magnetization (M) in a temperature (T) range = 2-300 K and a magnetic field (H) range = 0-10 kOe. All the HSs were superconducting with the critical temperature (T C) decreasing from = 78 to 36 K with decrease in d YBCO, whereas the ferromagnetic ordering temperature T M = 250 K did not change much. Systematically measured M-H loops of all HSs at both T > T C and T < T C show three main results (a) the two step magnetic reversal above T C converts into a four step reversal below T C in HSs with d YBCO ⩾ 30 nm, (b) the magnitude and magnetic field corresponding to the additional two switching steps show characteristic evolution with T and d YBCO; and (c) the HS with d YBCO = 20 nm shows radically different behaviour, where the two step magnetic reversal above T C continues to persist below T C and converts into a single step reversal at T [Formula: see text] T C. The first two results indicate magnetostatic coupling between the magnetic domains and the vortices across the two F/S interfaces resulting in reversal dynamics different from that deep within the LCMO layers. Whereas, the result 'c' reveals indirect exchange coupling between LCMO layers through the superconducting YBCO layer, which is a clear experimental evidence of coexistence of ferromagnetism and superconductivity in nm scale F/S/F HSs expected theoretically by Sa de Melo (2003 Physica C 387 17-25).

Magnetotransport in epitaxial films of the degenerate semiconductor Zn(1-x)Co(x)O.

Magnetotransport measurements are performed over a broad range of temperature (T) and magnetic field (H) on highly degenerate n-type Zn(1-x)Co(x)O [Formula: see text] epitaxial films. The cobalt-free samples are characterized by a metallic resistivity ρ(T) down to 2 K, a negative and predominantly isotropic magnetoresistance (MR) and optical transmission above 85% in the visible range of the electromagnetic spectrum. X-ray diffraction measurements show that while for [Formula: see text], all cobalt atoms occupy the tetrahedral sites of the wurtzite structure of ZnO, a phase separation into CoO is seen for x>0.2. In the solution phase, we do not observe any signatures of a spontaneous ordering of the cobalt spins despite a large concentration of mobile electrons (>10(20) cm(-3)). The absence of anomalous Hall resistance is consistent with this observation. The carrier concentration (n) over the entire range of x remains above the Mott limit for the insulator-to-metal transition in a doped semiconductor. However, while the Co-free samples are metallic (T>2 K), we see a resistivity (ρ) minimum followed by lnT divergence of ρ(T) at low temperatures with increasing x. The magnetoresistance of these samples is negative and predominantly isotropic. Moreover, the MR tends to follow a logH behaviour at high fields. These observations, including the Kondo-like minimum in the resistivity, suggest s-d exchange dominated transport in these dilute magnetic semiconductors.

Note: Fiber optic transport probe for Hall measurements under light and magnetic field at low temperatures: Case study of a two dimensional electron gas.

A fiber optic based probe is designed and developed for electrical transport measurements in presence of quasi-monochromatic (360-800 nm) light, varying temperature (T = 1.8-300 K), and magnetic field (B = 0-7 T). The probe is tested for the resistivity and Hall measurements performed on a LaAlO3-SrTiO3 heterointerface system with a conducting two dimensional electron gas.

Enhanced spin-orbit coupling and charge carrier density suppression in LaAl1-xCrxO3/SrTiO3 hetero-interfaces.

We report a gradual suppression of the two-dimensional electron gas (2DEG) at the LaAlO(3)/SrTiO(3) interface on substitution of chromium at the Al sites. The sheet carrier density at the interface (n□) drops monotonically from ∼2.2 × 10(14) cm(-2) to ∼2.5 × 10(13) cm(-2) on replacing ≈60% of the Al sites by Cr and the sheet resistance (R□) exceeds the quantum limit for localization (h/2e(2)) in the concentrating range 40-60% of Cr. The samples with Cr ⩽40% show a distinct minimum (T(m)) in metallic R□(T) whose position shifts to higher temperatures on increasing the substitution. Distinct signatures of Rashba spin-orbit interaction (SOI) induced magnetoresistance (MR) are seen in R□ measured in out of plane field (H⊥) geometry at T ⩽ 8 K. Analysis of these data in the framework of Maekawa-Fukuyama theory allows extraction of the SOI critical field (H(SO)) and time scale (τ(SO)) whose evolution with Cr concentration is similar as with the increasing negative gate voltage in LAO/STO interface. The MR in the temperature range 8 K ⩽ T ⩽ T(m) is quadratic in the field with a +ve sign for H⊥ and -ve sign for H∥. The behaviour of H∥ MR is consistent with Kondo theory which in the present case is renormalized by the strong Rashba SOI at T < 8 K.

Limit of the electrostatic doping in two-dimensional electron gases of LaXO3(X = Al, Ti)/SrTiO3.

In LaTiO3/SrTiO3 and LaAlO3/SrTiO3 heterostructures, the bending of the SrTiO3 conduction band at the interface forms a quantum well that contains a superconducting two-dimensional electron gas (2-DEG). Its carrier density and electronic properties, such as superconductivity and Rashba spin-orbit coupling can be controlled by electrostatic gating. In this article we show that the Fermi energy lies intrinsically near the top of the quantum well. Beyond a filling threshold, electrons added by electrostatic gating escape from the well, hence limiting the possibility to reach a highly-doped regime. This leads to an irreversible doping regime where all the electronic properties of the 2-DEG, such as its resistivity and its superconducting transition temperature, saturate. The escape mechanism can be described by the simple analytical model we propose.

Effect of pressure on itinerant magnetism and spin disorder in cubic FeGe.

The results of ab initio calculations of the pressure dependence of Fe magnetism in cubic FeGe are presented. We find that when the pressure-volume scale is set by means of generalized gradient approximation total energies and magnetism is described by means of the local density approximation, the critical pressure at which the magnetic phase transition occurs is estimated at ≈18 GPa, which is in good agreement with experiments. Using the disordered local moment method we find a localized to itinerant model cross-over of Fe magnetism in cubic FeGe, as a function of volume. Moreover, our calculations also suggest subtle signatures of longitudinal spin fluctuations in cubic FeGe, and that the stiffness parameter softens with increasing pressure. We associate the retention of metallicity in FeGe under pressure with the spin-disorder scattering. The effect of spin-orbit coupling on the electronic structure is also discussed.

Dynamics of a robust photo-induced insulator-metal transition driven by coherent and broad-band light in epitaxial films of La(0.625-y)Pr(y)Ca(0.375)MnO(3).

A dramatic drop of ≈5 orders of magnitude in the resistance (R) of La(0.175)Pr(0.45)Ca(0.375)MnO(3) epitaxial films upon exposure to optical photons derived from both continuous and pulsed lasers, as well as broad-band sources at temperatures (T) < 30 K is reported. The strength of change is a sensitive function of both the incident photon flux and temperature. Under isothermal conditions the photo-generated low resistance state persists eternally after removal of light. This non-equilibrium state is metallic, as revealed by the positive dR/dT for T ≤ T(p) (≈120 K). This electrically conducting state is presumably ferromagnetic as T(p) coincides with the temperature where a weak ferromagnetism sets in on cooling the insulating film from room temperature. To rule out the possibility of photon-induced local heating of the sample as a mechanism of the observed effects, photo-illumination experiments were performed under identical conditions on thin films of two non-charge-ordered manganites deposited on substrates of similar thermal conductivity. Our model for the observed transition encompasses a global charge-ordered state in which ferromagnetic metallic clusters of fraction p much less than the critical fraction p(c) for percolation exists at low temperatures. Photo-induced melting of the charge-ordered state increases this fraction beyond p(c) in a cumulative manner as successive pulses of light fall on the sample.

Two-dimensional superconductivity at a Mott insulator/band insulator interface LaTiO3/SrTiO3.

Transition metal oxides show a great variety of quantum electronic behaviours where correlations often have an important role. The achievement of high-quality epitaxial interfaces involving such materials gives a unique opportunity to engineer artificial structures where new electronic orders take place. One of the most striking result in this area is the recent observation of a two-dimensional electron gas at the interface between a strongly correlated Mott insulator LaTiO(3) and a band insulator SrTiO(3). The mechanism responsible for such a behaviour is still under debate. In particular, the influence of the nature of the insulator has to be clarified. In this article, we show that despite the expected electronic correlations, LaTiO(3)/SrTiO(3) heterostructures undergo a superconducting transition at a critical temperature T(c)(onset)~300 mK. We have found that the superconducting electron gas is confined over a typical thickness of 12 nm and is located mostly on the SrTiO(3) substrate.

Polaronic pseudogap in the metallic phase of La(0.625)Ca(0.375)MnO(3) thin films.

The electronic density of states (DOS) of La(0.625)Ca(0.375)MnO(3) (LCMO) strain-free epitaxial thin films with an insulator-metal transition temperature (T(IM)) of 250 K was probed using variable-temperature scanning tunneling microscopy and spectroscopy. We find a depression in the DOS with a finite zero bias conductance (ZBC) signifying a pseudogap in the 78-310 K temperature range. With cooling, the ZBC is found to increase, indicating an increased DOS near E(F). We interpret the pseudogap as a signature of Jahn-Teller polarons while the ZBC change, in agreement with the bulk insulator-metal transition, optical Drude peak and photoemission experiments, indicates the presence of free carriers at the Fermi energy in the metallic phase. The free carriers are discussed in terms of correlated polaronic states.

Infrared properties of single crystal MgO, a substrate for high temperature superconducting films.

We report and analyze the infrared properties of single crystal MgO, an important substrate for high T(c), superconducting films, from 10 to 280 cm(-1) and 20-300 K.