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1.
Nat Commun ; 15(1): 824, 2024 Jan 27.
Artigo em Inglês | MEDLINE | ID: mdl-38280890

RESUMO

Most superconductors have an isotropic, single component order parameter and are well described by the standard (BCS) theory for superconductivity. Unconventional, multiple-component superconductors are exceptionally rare and are much less understood. Here, we combine scanning tunneling microscopy and angle-resolved macroscopic transport for studying the candidate chiral superconductor, 4Hb-TaS2. We reveal quasi-periodic one-dimensional modulations in the tunneling conductance accompanied by two-fold symmetric superconducting critical field. The strong modulation of the in-plane critical field, Hc2, points to a nematic, unconventional order parameter. However, the imaged vortex core is isotropic at low temperatures. We suggest a model that reconciles this apparent discrepancy and takes into account previously observed spontaneous time-reversal symmetry breaking at low temperatures. The model describes a competition between a dominating chiral superconducting order parameter and a nematic one. The latter emerges close to the normal phase. Our results strongly support the existence of two-component superconductivity in 4Hb-TaS2 and can provide valuable insights into other systems with coexistent charge order and superconductivity.

2.
Phys Rev Lett ; 106(4): 047002, 2011 Jan 28.
Artigo em Inglês | MEDLINE | ID: mdl-21405348

RESUMO

The phase diagram of the superconducting high-T(c) cuprates is governed by two energy scales: T*, the temperature below which a gap is opened in the excitation spectrum, and T(c), the superconducting transition temperature. The way these two energy scales are reflected in the low-temperature energy gap is being intensively debated. Using Zn substitution and carefully controlled annealing we prepared a set of samples having the same T* but different T(c)'s, and measured their gap using angle-resolved photoemission spectroscopy (ARPES). We show that T(c) is not related to the gap shape or size, but it controls the size of the coherence peak at the gap edge.

3.
Sci Adv ; 6(13): eaax9480, 2020 Mar.
Artigo em Inglês | MEDLINE | ID: mdl-32258393

RESUMO

Van der Waals materials offer unprecedented control of electronic properties via stacking of different types of two-dimensional materials. A fascinating frontier, largely unexplored, is the stacking of strongly correlated phases of matter. We study 4Hb-TaS2, which naturally realizes an alternating stacking of 1T-TaS2 and 1H-TaS2 structures. The former is a well-known Mott insulator, which has recently been proposed to host a gapless spin-liquid ground state. The latter is a superconductor known to also host a competing charge density wave state. This raises the question of how these two components affect each other when stacked together. We find a superconductor with a T c of 2.7 Kelvin and anomalous properties, of which the most notable one is a signature of time-reversal symmetry breaking, abruptly appearing at the superconducting transition. This observation is consistent with a chiral superconducting state.

4.
Phys Rev Lett ; 101(13): 137002, 2008 Sep 26.
Artigo em Inglês | MEDLINE | ID: mdl-18851483

RESUMO

In the underdoped high temperature superconductors, instead of a complete Fermi surface above Tc, only disconnected Fermi arcs appear, separated by regions that still exhibit an energy gap. We show that in this pseudogap phase, the energy-momentum relation of electronic excitations near EF behaves like the dispersion of a normal metal on the Fermi arcs, but like that of a superconductor in the gapped regions. We argue that this dichotomy in the dispersion is difficult to reconcile with a competing order parameter, but is consistent with pairing without condensation.

5.
Phys Rev Lett ; 99(15): 157001, 2007 Oct 12.
Artigo em Inglês | MEDLINE | ID: mdl-17995204

RESUMO

Angle resolved photoemission on underdoped Bi2Sr2CaCu2O8 reveals that the magnitude and d-wave anisotropy of the superconducting state energy gap are independent of temperature all the way up to T{c}. This lack of T variation of the entire k-dependent gap is in marked contrast to mean field theory. At T{c} the point nodes of the d-wave gap abruptly expand into finite length "Fermi arcs." This change occurs within the width of the resistive transition, and thus the Fermi arcs are not simply thermally broadened nodes but rather a unique signature of the pseudogap phase.

6.
Phys Rev Lett ; 96(10): 107006, 2006 Mar 17.
Artigo em Inglês | MEDLINE | ID: mdl-16605781

RESUMO

The autocorrelation of angle resolved photoemission data from the high temperature superconductor Bi(2)Sr(2)CaCu(2)O(8+delta) shows distinct peaks in momentum space which disperse with binding energy in the superconducting state, but not in the pseudogap phase. Although it is tempting to attribute a nondispersive behavior in momentum space to charge ordering, a deconstruction of the autocorrelation reveals that the nondispersive peaks arise from the tips of the Fermi arcs, which themselves do not change with binding energy.

7.
Phys Rev Lett ; 92(25 Pt 1): 257007, 2004 Jun 25.
Artigo em Inglês | MEDLINE | ID: mdl-15245055

RESUMO

Using the transverse field muon spin relaxation technique, we measure the temperature dependence of the magnetic field penetration depth lambda, in the NaxCoO2.yH(2)O system. We find that lambda, which is determined by the superfluid density n(s) and the effective mass m*, is very small and on the edge of the TF-microSR sensitivity. Nevertheless, the results indicate that this system obeys the Uemura relation. By comparing lambda with the normal state electron density, we conclude that m* of the superconductivity carrier is 70 times larger than the mass of bare electrons. Finally, the order parameter in this system cannot be described by a complete gap over the entire Fermi surface.

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