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1.
Environ Geochem Health ; 46(8): 297, 2024 Jul 09.
Artigo em Inglês | MEDLINE | ID: mdl-38980451

RESUMO

The radiological characterization of soil contaminated with natural radionuclides enables the classification of the area under investigation, the optimization of laboratory measurements, and informed decision-making on potential site remediation. Neural networks (NN) are emerging as a new candidate for performing these tasks as an alternative to conventional geostatistical tools such as Co-Kriging. This study demonstrates the implementation of a NN for estimating radiological values such as ambient dose equivalent (H*(10)), surface activity and activity concentrations of natural radionuclides present in a waste dump of a Cu mine with a high level of natural radionuclides. The results obtained using a NN were compared with those estimated by Co-Kriging. Both models reproduced field measurements equivalently as a function of spatial coordinates. Similarly, the deviations from the reference concentration values obtained in the output layer of the NN were smaller than the deviations obtained from the multiple regression analysis (MRA), as indicated by the results of the root mean square error. Finally, the method validation showed that the estimation of radiological parameters based on their spatial coordinates faithfully reproduced the affected area. The estimation of the activity concentrations was less accurate for both the NN and MRA; however, both methods gave statistically comparable results for activity concentrations obtained by gamma spectrometry (Student's t-test and Fisher's F-test).


Assuntos
Cobre , Mineração , Redes Neurais de Computação , Monitoramento de Radiação , Poluentes Radioativos do Solo , Cobre/análise , Poluentes Radioativos do Solo/análise , Monitoramento de Radiação/métodos , Análise de Regressão
2.
Environ Monit Assess ; 196(2): 139, 2024 Jan 11.
Artigo em Inglês | MEDLINE | ID: mdl-38206400

RESUMO

Natural radioactive concentration assessment was conducted on sediment, water, and biota obtained on Vaan and Koswari islands in the Tuticorin group of islands, Tamil Nadu, India. For biotic and abiotic components, radiation profiles such as gross alpha, beta, primordial radionuclide, polonium, and lead analyses were performed. The gross α and ß range from BDL to 15.18 ± 1.7 Bq/kg and 40.43 ± 4.9 Bq/kg to 105.12 ± 11.7 Bq/kg, respectively. Primordial radionuclides were analyzed using Nal(TI)-based scintillator with PC-MCA, and the concentrations ranged from 13.43 ± 3.3 Bq/kg to 30.97 ± 9.6 Bq/kg with a mean of 21.31 ± 2.7 Bq/kg for 238U; for 232Th, the values ranged from 11.09 ± 2.6 Bq/kg to 33.55 ± 9.5 Bq/kg with an average value of 23.89 ± 3.7 Bq/kg; and for 40 K, the values are 93.33 ± 27.3 Bq/kg to 219.91 ± 39.6 Bq/kg with an average value of 148.27 ± 21.7 Bq/kg. The present study values are lesser than the world average values. 210Po and 210Pb concentrations with an average value were determined to be 33.13 Bq/L and 16.56 Bq/L, 47.55 Bq/L and 22.37 Bq/L in the water sample, and 50.437 Bq kg1 and 62.012 Bq kg1, 46.99 Bq/kg and 58.625 Bq/kg in sediments of Vaan island and Koswari island. The concentrations of 210Po and 210Pb of Pogonias cromis were 19.27 ± 1.5 Bq/kg and 8.27 ± 1.01 Bq/kg, Belonidae 28.54 ± 2.4 Bq/kg and 18.32 ± 2.3 Bq/kg, Lepisosteidae 18.68 ± 1.4 Bq/kg and 11.17 ± 1.8 Bq/kg. The committed effective dosage was determined to be 35.74-54.61 µSv/y for 210Po and 25.39-56.25 µSv/y for 210Pb, in which the 210Pb value is lower; however, the 210Po value is higher than the global average value. The annual committed effective dosage as well as the radiological hazard indices were assessed and found to be much below the global average and the recommended limit, respectively. This research provides an extensive analysis of natural background radiation and establishes a baseline report on the radiological profile of biotic and abiotic factors in the Tuticorin group of islands, namely Vaan and Koswari, in Tamil Nadu, India.


Assuntos
Monitoramento Ambiental , Chumbo , Índia , Medição de Risco , Água
3.
Environ Monit Assess ; 196(9): 847, 2024 Aug 27.
Artigo em Inglês | MEDLINE | ID: mdl-39190160

RESUMO

This investigation quantifies the activity concentrations of natural radionuclides (226Ra, 232Th, and 40K) in the soils and certain rocks of the Koytash-Ugam Range, Uzbekistan, and assesses their radiological risks. Gamma-spectrometric analysis of soil and rock samples revealed activity concentrations ranging from 456.2 ± 56.0 to 813.9 ± 76.0 Bq kg-1 for 40K, 18.2 ± 6.3 to 70.0 ± 12.0 Bq kg-1 for 226Ra, and 30.1 ± 2.9 to 57.9 ± 10 Bq kg-1 for 232Th. This data indicates a heterogeneous distribution of radionuclides, informing radiation safety and health risk assessments on a global scale. The calculation of radiological hazard indices, including the alpha-index (ranging from 0.09 to 0.35), gamma-index (ranging from 0.40 to 0.73), and both internal (ranging from 0.40 to 0.54) and external (ranging from 0.36 to 0.54) hazard indices, was undertaken to ascertain potential health risks. The radium equivalent activity ranged from 108.4 to 199.3 Bq kg-1, and the absorbed dose rates were 51.0-93.3 nGy h-1 indoors and 96.6-178.2 nGy h-1 outdoors. These metrics underlie the estimated annual effective dose of 536.5-988.5 × 10-3 mSv y-1, highlighting the variability in radiation exposure. Additionally, the potential lifetime cancer risk was projected at 1770.4 to 3262.0 per million, with an annual gonadal dose equivalent of 361.9 to 655.5 µSv y-1, reflecting natural background radiation influence. The results underscore the importance of safe material use in construction and the necessity for routine natural radioactivity monitoring. Radon flux density (RFD) values within acceptable construction limits (26-176 mBq m-2 s-1) suggest the area's suitability for development, considering recommended safety guidelines. This study not only aids local environmental and public health frameworks but also enriches the international knowledge base, facilitating comparative studies for the advancement of global radiation protection standards. Through a detailed examination of radionuclide distribution in an under-researched area, our research highlights the critical need for integrated international approaches to natural radiological hazard assessment.


Assuntos
Monitoramento de Radiação , Rádio (Elemento) , Poluentes Radioativos do Solo , Tório , Poluentes Radioativos do Solo/análise , Uzbequistão , Rádio (Elemento)/análise , Tório/análise , Solo/química , Medição de Risco , Radioisótopos de Potássio/análise , Radiação de Fundo
4.
Environ Monit Assess ; 196(12): 1169, 2024 Nov 05.
Artigo em Inglês | MEDLINE | ID: mdl-39500760

RESUMO

The enhancement of natural radioactivity in groundwater, specifically in natural mineral water, is related to the lithological formations through which water bodies or courses pass. Although natural mineral waters are exempt from monitoring for radioactive substances according to Council Directive 2013/51/EURATOM, this study focuses on the radiological characterization of natural mineral water under Spanish Royal Decree 3/2023. The water studied was taken from Catalan aquifers with different lithological characteristics (sedimentary, metamorphic or granitic) and is sold on local markets. Moreover, radiological data on the water was correlated with its lithological origin and the health risk for different age groups was assessed. Our results showed that of the 26 natural mineral waters studied, 10 exceeded gross alpha screening value (100 mBq/L), all from granitic aquifers. Further research on natural individual radionuclides was conducted on these ten samples. 234U and 238U were at around 1100-1600 mBq/L. In addition, 210Pb was found in two samples, which also presented the highest 226Ra activity, associated with granitic bedrock and the presence of 210Po. The annual effective dose was 179.0 µSv/year and 145.9 µSv/year, exceeding 100 µSv/year mainly due to the contribution of 210Pb > 234,238U > 210Po > 226Ra, in this order. After assessing the lifetime cancer risk, these two samples were determined not to pose a health risk due to ingestion. Although no radiological monitoring is required for natural mineral water, further surveillance is recommendable.


Assuntos
Água Potável , Água Subterrânea , Águas Minerais , Monitoramento de Radiação , Poluentes Radioativos da Água , Águas Minerais/análise , Medição de Risco , Poluentes Radioativos da Água/análise , Água Potável/química , Água Subterrânea/química , Espanha , Humanos , Rádio (Elemento)/análise , Radioisótopos de Chumbo/análise , Urânio/análise
5.
Environ Monit Assess ; 196(12): 1151, 2024 Nov 04.
Artigo em Inglês | MEDLINE | ID: mdl-39489820

RESUMO

To establish a radiological national reference for agricultural soil across Tunisian oases and assess the risk to human health associated with date consumption, with a focus on comparing the impact of traditional and modern fertilization, radiological parameters and activity levels of 226Ra, 232Th, and 4°K were determined for 27 oases. These oases were located in three southern Tunisian governorates. The activity concentration of 226Ra, 232Th, and 4°K was measured using a 3 × 3 inch NaI(Tl) scintillation detector, which was found to be 21.82 ± 1.0 Bq kg - 1 , 26.51 ± 1.1 Bq kg - 1 , and 559.21 ± 23.0 Bq kg - 1 , respectively, for traditional oases and 26.56 ± 1.2 Bq kg - 1 , 24.45 ± 1.1 Bq kg - 1 , and 661.28 ± 26.3 Bq kg - 1 , respectively, for modern oases. In addition, ambient dose equivalent rate was measured during sampling using a multipurpose hand-held radiation CsI(Tl) detector, which was found to be 0.075 µSv/h in traditional oases and 0.078 µSv/h in modern oases. The resulting radiological parameters and activity concentrations were then compared to results from neighboring countries and the average soil activity worldwide.


Assuntos
Agricultura , Fertilizantes , Monitoramento de Radiação , Poluentes Radioativos do Solo , Solo , Tunísia , Poluentes Radioativos do Solo/análise , Monitoramento de Radiação/métodos , Solo/química , Rádio (Elemento)/análise , Tório/análise , Radioatividade , Radioisótopos de Potássio/análise
6.
Environ Monit Assess ; 196(2): 186, 2024 Jan 23.
Artigo em Inglês | MEDLINE | ID: mdl-38253920

RESUMO

To estimate the radiation hazard due to the natural terrestrial radioactivity, 598 samples of soil covering the entire Romanian territory were collected and analyzed for the distribution of natural radionuclides 40K, 228Ac, and 226Ra. The ultra-low background Slanic-Prahova underground laboratory was used to determine the gamma-ray-specific activity of these radioactive isotopes with an uncertainty between 5 and 20%. All these data permitted to establishing a set of 2D maps illustrating the distribution of specific activity of each radionuclide as well as of the resulting air dose rate, all of them illustrating an heterogeneous distribution, increased values being displaced on the western and south-western territory. Mediated over 598 points, these determinations led to a value of annual effective dose of 0.7 ± 0.15 mSv/y and an external hazard index of 0.46 ± 0.1, both attesting to a radioecologically safe environment for human activity.


Assuntos
Monitoramento Ambiental , Laboratórios , Humanos , Romênia , Raios gama , Radioisótopos
7.
Environ Monit Assess ; 196(11): 1033, 2024 Oct 08.
Artigo em Inglês | MEDLINE | ID: mdl-39377949

RESUMO

The aim of this study was to analyze the radiological hazards and the potential for generating acid mine drainage from the fine coal waste commonly stored in tailings dams. The magnetic susceptibility, natural gamma radioactivity, and net neutralization potential of the tailings are characterized. The results show that the fine coal waste has a uranium equivalent concentration (eU) of 46-48 Bq kg-1, which is 37.14% higher than the world average, and 39-47 Bq kg-1 equivalent concentration of thorium (eTh), which is 56.66% higher than the world average. Also, the absorbed gamma radiation dose rate is higher than the world average. Acid-base balance tests indicate that the net neutralization potential ranged from 0.38 to 2.44. The physical properties indicate a possible radiological risk, while the chemical properties show that generating and non-generating acid drainage can coexist in the fine dam tailings.


Assuntos
Minas de Carvão , Urânio/análise , Monitoramento de Radiação , Carvão Mineral , Tório/análise , Mineração , Raios gama , Ácidos
8.
Environ Monit Assess ; 196(11): 1038, 2024 Oct 09.
Artigo em Inglês | MEDLINE | ID: mdl-39384632

RESUMO

Radionuclide and radon levels have been investigated in soil samples and residential environments within the Mungo and Nkam Divisions of the Littoral Region. These analyses employed gamma spectrometry facilitated by a NaI (Tl) detector for soil samples, yielding average activity concentrations of 226Ra, 232Th, and 40 K at 23.8, 72, and 105 Bq kg-1, respectively. Various radiological parameters were calculated to evaluate radiological hazards. Additionally, the indoor radon concentrations were quantified utilizing the CR-39 solid-state nuclear track detector (Radtrack), revealing an average concentration of 25 Bq m-3 and an associated inhalation dose of 0.66 mSv y-1. Risk assessments for lung cancer attributable to indoor radon exposure incorporated models such as the Harley model. An observed moderate correlation between indoor radon levels and external 226Ra concentrations implies that radon intrusion indoors might be substantially influenced by the 226Ra present in the subjacent soil, considering the construction of residential structures directly upon these terrains.


Assuntos
Poluição do Ar em Ambientes Fechados , Habitação , Monitoramento de Radiação , Radônio , Poluentes Radioativos do Solo , Radônio/análise , Camarões , Poluentes Radioativos do Solo/análise , Poluição do Ar em Ambientes Fechados/análise , Poluição do Ar em Ambientes Fechados/estatística & dados numéricos , Poluentes Radioativos do Ar/análise , Rádio (Elemento)/análise , Tório/análise , Solo/química
9.
Radiat Environ Biophys ; 62(2): 279-285, 2023 05.
Artigo em Inglês | MEDLINE | ID: mdl-36862217

RESUMO

The purpose of this study was to investigate the radiological quality of drinking water in Ma'an governorate, which includes the archeological city of Petra and is one of Jordan's most important tourist destinations. To the best of the authors' knowledge, this is the first study in southern Jordan that investigates radioactivity in drinking water and its potential to cause cancer. A liquid scintillation detector was used to measure gross alpha and gross beta activities in tap water samples from Ma'an governorate. A high-purity Germanium detector was used to measure the activity concentrations of 226Ra and 228Ra. Gross alpha, gross beta, 226Ra, and 228Ra activities were < 110-724 mBq/l, < 220-362 mBq/l, < 11-241 mBq/l, and < 32-49 mBq/l, respectively. The results were compared to internationally recommended levels and literature values. Annual effective doses ([Formula: see text]) from 226 and 228Ra intake were calculated for infants, children, and adults. The highest doses were found for children while the lowest were found for infants. For each water sample, the lifetime risk of radiation-induced cancer (LTR) was calculated for the whole population. All of the LTR values were lower than the value recommended by the World Heath Organisation. It is concluded that there are no significant radiation-related health risks associated with consumption of tap water from the studied region.


Assuntos
Água Potável , Neoplasias Induzidas por Radiação , Monitoramento de Radiação , Radioatividade , Rádio (Elemento) , Poluentes Radioativos da Água , Criança , Lactente , Adulto , Humanos , Água Potável/análise , Doses de Radiação , Neoplasias Induzidas por Radiação/epidemiologia , Neoplasias Induzidas por Radiação/etiologia , Jordânia/epidemiologia , Poluentes Radioativos da Água/análise , Rádio (Elemento)/análise
10.
Int J Environ Health Res ; 33(12): 1640-1651, 2023 Dec.
Artigo em Inglês | MEDLINE | ID: mdl-36041221

RESUMO

Gamma spectrometric measurement of natural radionuclides activity concentrations by HPGe detectors was conducted in 150 agricultural soil samples collected from six states of southwestern Nigeria. The overall activity concentrations of radionuclides ranged from 15.27 to 972.00 Bqkg-1 for 40K, 0.66 to 336.19 Bqkg-1 for 232Th and 1.32 to 123.01 Bqkg-1 for 238U, with mean values of 143.95, 17.02 and 22.92 Bqkg-1, respectively. The overall averages results from this study were generally lower than worldwide average value of 420, 33 and 45 Bqkg-1 for 40K, 238U and 232Th, respectively, thus minimal transfer to plant may be expected. The estimated radiation dose levels of the soil indicated acceptable limits for general public exposure. The radioactivity levels of 40K, 232Th and 238U in the investigated agricultural soil of southwestern Nigeria are within acceptable limits. Therefore, stochastic radiological health effects of radiation exposure by farmers may not be feasible at the current moment.


Assuntos
Monitoramento de Radiação , Poluentes Radioativos do Solo , Solo/química , Nigéria , Monitoramento de Radiação/métodos , Poluentes Radioativos do Solo/análise , Radioisótopos/análise , Doses de Radiação
11.
Int J Environ Health Res ; 33(12): 1706-1715, 2023 Dec.
Artigo em Inglês | MEDLINE | ID: mdl-36062411

RESUMO

Bentonite is a soft, porous, easily shaped, and absorbent material rich in aluminum, sodium, and potassium. Bentonite is a mineral widely utilized as drilling mud, ore pelletizing, absorbent/adsorbent, bleaching agent, water impedance, coating, and raw material in various industries. In this study, radiometric measurements of 90 bentonite samples collected from 21 quarries in Turkey were performed using gamma-ray spectrometry. The radiological hazards caused by indoor exposure to adults due to the utilization of bentonites as raw materials in the construction industry and outdoor external exposures to quarry workers were evaluated by estimating the activity concentration index, annual effective doses, and lifetime cancer risk. The average activity concentrations of 226Ra, 232Th and 40K measured in bentonite samples were found as (50 ± 5) Bq/kg, (76 ± 4) Bq/kg and (373 ± 19) Bq/kg, respectively. The evaluation results reveal that the bentonites examined could be safely utilized as raw materials.


Assuntos
Monitoramento de Radiação , Radônio , Humanos , Bentonita/análise , Monitoramento de Radiação/métodos , Radônio/análise , Radioisótopos/análise , Espectrometria gama
12.
Environ Geochem Health ; 45(12): 9825-9836, 2023 Dec.
Artigo em Inglês | MEDLINE | ID: mdl-37861806

RESUMO

In this study, the specific activities of 226Ra, 232Th and 40K in the unfired construction materials (solid card bricks, 4-hole bricks, pavement bricks) containing fly ash and bottom ash from a coal-fired thermal power plant in Vietnam were measured using the low-level gamma-ray spectrometer with HPGe detector. Also, the 222Rn concentrations in these materials were analyzed using RAD7 radon monitor and then radon mass exhalation rate and emanation fraction of these materials were calculated. The potential radiological hazards for residents living in the model room made of these materials were evaluated. The average specific activity of 226Ra, 232Th and 40K were found as 67.7, 79.3 and 703.5 Bq kg-1, respectively. The total annual effective dose (due to external gamma exposure and internal radon exposure for resident living in the CEN model room made of the unfired brick samples) was found as 0.9 mSv y-1 which is lower than the worldwide average dose of 2.4 mSv y-1. Calculations from ResRad-Build code showed that the doses due to radon exposure account for from 62.3% (at the first year) to 98.8% (at the next 30 years) of the total gamma and radon dose. Under low air exchange to the outside environment, from the 6th year onwards, the total dose may exceed the average dose value from natural radiation exposure sources.


Assuntos
Monitoramento de Radiação , Radônio , Cinza de Carvão/análise , Vietnã , Radônio/análise , Materiais de Construção
13.
J Radiol Prot ; 43(3)2023 09 22.
Artigo em Inglês | MEDLINE | ID: mdl-37699385

RESUMO

The accumulation of naturally occurring radionuclides in solid residues was investigated from groundwater treatment facilities (GTFs) in Finland. Natural radionuclides U-238, Ra-226, Pb-210 and Ra-228 were found in various precipitates, sludges and filters at concentrations exceeding the general clearance level of 1 kBq kg-1used for solid materials in the European directive 2013/59/Euratom. The accumulation of natural radionuclides in different solid residues was observed even when the activity concentrations in the untreated groundwater were relatively low, and when there was no measurable change in the concentrations between raw and treated groundwater within analytical uncertainties. Based on mass and activity balance considerations this is thought to be due to the large volumes of treated water per year. The exposure of workers to natural radiation from solid residues in the regular use of a groundwater facility was found not to be likely to exceed 0.3 mSv a-1if the activity concentrations are <10 kBq kg-1for U-238, Ra-226, Pb-210 and Ra-228. The worker exposure from solid residues is therefore likely to remain below the reference level of 1 mSv a-1, and indoor radon is more of a concern for the radiation protection of workers at GTFs. However, the natural radionuclide content in the different solid residues from groundwater treatment needs to be characterised properly to be able to ensure safety in the final use of the residues with respect to the potential exposure of the public.


Assuntos
Água Subterrânea , Radioatividade , Urânio , Humanos , Finlândia
14.
J Radiol Prot ; 43(1)2023 02 22.
Artigo em Inglês | MEDLINE | ID: mdl-36731127

RESUMO

Radon-222 (222Rn) and its decay products are the primary sources of a population's exposure to background ionizing radiation. Radon decay products are the leading cause of lung cancer for non-smokers and the second leading cause of lung cancer after smoking for smokers. A community-driven long-term radon survey was completed in 232 residential homes in different subdivisions of Whitehorse, the capital of the Yukon, during the heating season from November to April in 2016-2017 and in 2017-2018. Radon concentrations were measured in living rooms and bedrooms on ground floors. The arithmetic and geometric means of indoor radon activity concentrations in different subdivisions of Whitehorse ranged from 52 ± 0.6 Bq m-3and 37 ± 2.3 Bq m-3in the Downtown area of Whitehorse to 993.0 ± 55.0 Bq m-3and 726.2 ± 2.4 Bq m-3in Wolf Creek. Underlying geology and glacial surfaces may partly explain these variations of indoor radon concentrations in subdivisions of Whitehorse. A total of 78 homes (34.0%) had radon concentrations higher than 100 Bq m-3, 47 homes (20.5%) had concentrations higher than 200 Bq m-3and 33 homes (14.4%) had concentrations higher than 300 Bq m-3. The indoor radon contribution to the annual effective inhalation dose to residents ranged from 3.0 mSv in the Downtown area to 51.0 mSv in Wolf Creek. The estimated annual average dose to adults in Whitehorse, Yukon, is higher than the world's average annual effective dose of 1.3 mSv due to the inhalation of indoor radon. The annual radon inhalation effective dose was assessed using radon measurements taken during winter; hence the assessed dose may be overestimated. Cost-efficient mitigation methods are available to reduce radon in existing buildings and to prevent radon entry into new buildings.


Assuntos
Poluentes Radioativos do Ar , Poluição do Ar em Ambientes Fechados , Monitoramento de Radiação , Radônio , Lobos , Animais , Poluição do Ar em Ambientes Fechados/análise , Radônio/análise , Poluentes Radioativos do Ar/análise , Canadá , Habitação , Monitoramento de Radiação/métodos
15.
Environ Monit Assess ; 195(12): 1523, 2023 Nov 23.
Artigo em Inglês | MEDLINE | ID: mdl-37995004

RESUMO

Surface soil samples were collected from Konya, Turkey and natural activity concentrations were determined using the ɤ-ray spectroscopy system with HPGe detector. The activity concentrations of 226Ra, 232Th and 40K were found to vary from 14.07 ± 0.71 Bq kg-1 dw to 67.27 ± 1.62 Bq kg-1 dw, 10.19 ± 2.60 Bq kg-1 dw to 46.09 ± 0.76 Bq kg-1 dw and 107.87 ± 13.32 Bq kg-1 dw to 605.95 ± 11.34 Bq kg-1 dry weight (dw), respectively. The radiological hazard parameters such as Raeq, D, AEDE, ELCR, AGDE, Hex, Hin, and Iɤ evaluated the radiological risk for the public and environment. The mean values of D, AEDE and ELCR are lower than the world average value of 57 nGy h-1, 70 µSv y-1, 0.29 × 10-3 respectively. The activity concentration distribution maps of 226Ra, 232Th and 40K and the radiological maps of the radiological hazard parameters were plotted using the Surfer programme. Cluster analysis was carried out to indicate the similarity between the variables.


Assuntos
Monitoramento de Radiação , Radioatividade , Rádio (Elemento) , Poluentes Radioativos do Solo , Monitoramento de Radiação/métodos , Poluentes Radioativos do Solo/análise , Solo/química , Turquia , Saúde Radiológica , Tório/análise , Radioisótopos de Potássio/análise , Rádio (Elemento)/análise
16.
Environ Monit Assess ; 195(5): 579, 2023 Apr 17.
Artigo em Inglês | MEDLINE | ID: mdl-37067680

RESUMO

Bangladesh is a rapidly developing country, which is vulnerable to various types of pollution due to the large-scale industrial and associated human activities that might potentially affect the locally harvested foodstuffs. Therefore, the transfer factor is an essential tool to assess the safety of foodstuffs due to the presence of natural radioactivity in environmental matrix and/or strata. This is a first study of its kind conducted in a well-known region for mango farming in Bangladesh, measuring the uptake of naturally occurring radioactive materials (NORMs) by grass and mango from soil to assess the ingestion doses to humans. The HPGe gamma-ray detector was used to determine the concentrations of NORMs in samples of soil (20), grass (10), and mango (10), which were then used to calculate the transfer factors of soil to grass and soil to mango. Average activity concentrations of 226Ra, 232Th, and 40K in associated soil samples (47.27 ± 4.10, 64.49 ± 4.32, 421.60 ± 28.85) of mango and 226Ra and 232Th in associated soil samples (45.07 ± 3.93, 52.17 ± 3.95) of grass were found to exceed the world average values. The average transfer factors (TFs) for mango were obtained in the order of 40K(0.80) > 226Ra (0.61) > 232Th (0.31), and for grass, it shows the order of 40K (0.78) > 232Th (0.64) > 226Ra (0.56). However, a few values (3 mango samples and 3 grass samples) of the estimated TFs exceeded the recommended limits. Moreover, Bangladesh lacks the transfer factors for most of the food crops; therefore, calculation of TFs in the major agricultural products is required all over Bangladesh, especially the foodstuffs produced near the Rooppur Nuclear Power Plant, which is scheduled to be commissioned in 2023.


Assuntos
Mangifera , Monitoramento de Radiação , Poluentes Radioativos do Solo , Humanos , Solo , Fator de Transferência , Bangladesh , Poaceae , Poluentes Radioativos do Solo/análise , Radioisótopos/análise
17.
Environ Monit Assess ; 195(11): 1307, 2023 Oct 13.
Artigo em Inglês | MEDLINE | ID: mdl-37831213

RESUMO

Radioactive elements and their impact on the environment and the food chain, including humans, are a matter of major concern, for which appropriate investigations should be performed. The priority is to examine the concentration of radioactive substances in mineral and bottled spring water. This task aims to analyze the quality of 12 conditioned mineral waters by determining their main radionuclides concentrations, such as 238U, 232Th, and 40K. The identification and the quantification of these radionuclides are carried out by their progeny (except the 40K) by using a NaI(Tl) detector coupled with a multichannel analyzer (MCA) and connected to a computer. The activity measured in all samples varied from 0.95 to 3.38 mBq.L-1 with an average of 1.94 mBq.L-1; from 1.55 to 3.56 mBq.L-1 with an average of 2.46 mBq.L-1; and from 200.68 to 269.19 mBq.L-1 with an average of 236.6 mBq.L-1, for 238U, 232Th, and 40K, respectively. To compare the combined radiological effects of radionuclides present in water, a particular factor Ra(eq) is used. This study showed that the maximum value of Ra(eq) is 27.54 mBq.L-1, which is far below the activity limit of 370 mBq.year-1 set by the Organization of Economics and Development (OECD). Concerning the effective annual dose, the following maximums were measured: 1.61 µSv.year-1, 1.133 µSv.year-1, and 0.925 µSv.year-1 for infants, children, and adults, respectively. These values are even smaller than the dose recommended by the WHO which is 100 µSv.year-1. Regarding the excess lifetime cancer risk index, a maximum of 5.63 × 10-6 is found. This index value is still less than that proposed by James, namely 2.5 × 10-3. Thus, the quality of the studied samples respects the radiological international safety and health limits.


Assuntos
Água Potável , Monitoramento de Radiação , Radioatividade , Poluentes Radioativos da Água , Lactente , Criança , Adulto , Humanos , Água Potável/química , Poluentes Radioativos da Água/análise , Espectrometria gama , Monitoramento de Radiação/métodos , Radioisótopos/análise
18.
Environ Monit Assess ; 195(9): 1028, 2023 Aug 10.
Artigo em Inglês | MEDLINE | ID: mdl-37558890

RESUMO

This study marks the first-ever assessment of radiological hazards linked to the sands and rocks of Patuartek Sea Beach, situated along one of the world's longest sea beaches in Cox' Bazar of Bangladesh. Through the utilization of an HPGe detector, a comprehensive analysis of the activity concentrations of 226Ra, 232Th, and 40 K was conducted, and their activity ranged from 7 to 23 Bq/kg, 9-58 Bq/kg, and 172-340 Bq/kg, respectively, in soils, and 19-24 Bq/kg, 27-39 Bq/kg, and 340-410 Bq/kg, respectively, in rocks. Some sand samples exhibited elevated levels of 232Th, while the rock samples displayed higher levels of 40 K compared to the global average. The radiological hazard parameters were assessed, and no values surpassed the recommended limits set by several international organizations. Hence, the sands and rocks of Patuartek sea beach pose no significant radiological risk to the residents or tourists. The findings of this study provide crucial insights for the development of a radiological baseline map in the country, which is important due to the commissioning of the country's first nuclear power plant Rooppur Nuclear Power Plant. The data may also stimulate interest in the rare-earth minerals present in the area, which is important for the electronics industry, thorium-based nuclear fuel cycles.


Assuntos
Monitoramento de Radiação , Radioatividade , Rádio (Elemento) , Poluentes Radioativos do Solo , Radioisótopos de Potássio/análise , Dióxido de Silício/análise , Solo , Areia , Bangladesh , Poluentes Radioativos do Solo/análise , Praias , Tório/análise , Rádio (Elemento)/análise
19.
Molecules ; 27(7)2022 Mar 25.
Artigo em Inglês | MEDLINE | ID: mdl-35408510

RESUMO

The exploitation of mineral resources may cause the environmental release of radionuclides and their introduction in the human trophic chain, affecting public health in the short and long term. A case study of the environmental radiation impact from coal mining and germanium processing was carried out in southwest China. The coal mines contain germanium and uranium and have been exploited for more than 40 years. The farmlands around the site of the coal mining and germanium processing have been contaminated by the solid waste and mine water to some extent since then. Samples of crops were collected from contaminated farmlands in the research area. The research area covers a radius of 5 km, in which there are two coal mines. 210Pb and 210Po were analyzed as the key radionuclides during the monitoring program. The average activity concentrations of 210Pb and 210Po in the crops were 1.38 and 1.32 Bq/kg in cereals, 4.07 and 2.19 Bq/kg in leafy vegetables and 1.63 and 1.32 Bq/kg in root vegetables. The annual effective doses due to the ingestion of 210Pb and 210Po in consumed crops were estimated for adult residents living in the research area. The average annual effective dose was 0.336 mSv/a, the minimum was 0.171 mSv/a and the maximum was 0.948 mSv/a. The results show that the crops grown on contaminated farmland contained an enhanced level of radioactivity concentration. The ingestion doses of local residents in the research area were significantly higher than the average level of 0.112 mSv/a in China, and the world average level of 0.042 mSv/a through 210Pb and 210Po in crop intake, respectively.


Assuntos
Minas de Carvão , Germânio , Adulto , Carvão Mineral , Produtos Agrícolas , Ingestão de Alimentos , Humanos , Chumbo , Polônio , Radioisótopos/análise
20.
J Radiol Prot ; 42(1)2022 Jan 12.
Artigo em Inglês | MEDLINE | ID: mdl-34814129

RESUMO

In the 2019-20 reporting period, 19 mining operations in Western Australia were identified as having workers who were likely to be exposed to ionising radiation stemming from naturally occurring radioactive materials, 17 of which, known hereinafter as reporting entities (REs), were required to submit an annual report of the dose estimates of their workforce to the mining regulatory authority. In 2018 the International Commission for Radiological Protection published the revision of the dose coefficients (DCs) for occupational intakes of radionuclides of the uranium-238 and thorium-232 decay series, in ICRP-137 and ICRP-141. The 2019-20 annual reports are the first to apply the revised DCs to estimate worker doses. The mean effective dose (ED) reported by the 17 REs increased by 32.4% to 0.94 mSv in 2019-20 from 0.71 mSv reported in 2018-19, indicating that the mean ED is approaching the 1 mSv annual dose estimate at which regulatory intervention should be considered. The mean committed effective dose (CED) from inhalation of dusts containing long-lived alpha-emitting (LLα) nuclides has increased by 35% from 0.40 mSv in 2018-19 to 0.54 mSv in 2019-20. The maximum CED from LLαincreased by 16.3% from 3.20 mSv in 2018-19 to 3.72 mSv in 2019-20. The authors consider that, in the absence of other explanations provided by the REs, the increase is largely attributable to the revised DC's published in ICRP-137 and ICRP-141, but highlight that there are significant variations between REs that make a generalised conclusion problematic. The maximum reported ED in 2019-20 was 6.0 mSv, an increase of 36.4% from 2018 to 2019 (4.4 mSv). The 2019-20 reporting period is the first time in a decade in which mine worker EDs have been elevated to the point that EDs have exceeded 5 mSv, a level at which personal monitoring and additional institutional controls are required.


Assuntos
Exposição Ocupacional , Monitoramento de Radiação , Proteção Radiológica , Austrália , Humanos , Exposição Ocupacional/análise , Doses de Radiação
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