Fast quantum interference of a nanoparticle via optical potential control.

We introduce and theoretically analyze a scheme to prepare and detect non-Gaussian quantum states of an optically levitated particle via the interaction with light pulses that generate cubic and inverted potentials. We show that this approach allows to operate on sufficiently short time- and length scales to beat decoherence in a regime accessible in state-of-the-art experiments. Specifically, we predict the observation of single-particle interference of a nanoparticle with a mass above 108 atomic mass units delocalized by several nanometers, on timescales of milliseconds. The proposed experiment uses only optical and electrostatic control, and can be performed at about 10-10 mbar and at room temperature. We discuss the prospect of this method for coherently splitting the wavepacket of massive dielectric objects without using either projective measurements or an internal level structure.

Observation of high-order imaginary Poynting momentum optomechanics in structured light.

The imaginary Poynting momentum (IPM) of light has been captivated as an unusual origin of optical forces. However, the IPM force is predicted only for dipolar magnetoelectric particles that are hardly used in optical manipulation experiments. Here, we report a whole family of high-order IPM forces for not only magnetoelectric but also generic Mie particles, assisted with their excited higher multipoles within. Such optomechanical manifestations derive from a nonlocal contribution of the IPM to the optical force, which can be remarkable even when the incident IPM is small. We observe the high-order optomechanics in a structured light beam, which, despite carrying no angular momentum, is able to set normal microparticles into continuous rotation. Our results provide unambiguous evidence of the ponderomotive nature of the IPM, expand the classification of optical forces, and open new possibilities for levitated optomechanics and micromanipulations.

High Q-Factor Diamond Optomechanical Resonators with Silicon Vacancy Centers at Millikelvin Temperatures.

Phonons are envisioned as coherent intermediaries between different types of quantum systems. Engineered nanoscale devices, such as optomechanical crystals (OMCs), provide a platform to utilize phonons as quantum information carriers. Here we demonstrate OMCs in diamond designed for strong for interactions between phonons and a silicon vacancy (SiV) spin. Using optical measurements at millikelvin temperatures, we measure a line width of 13 kHz (Q-factor of ∼4.4 × 105) for a 6 GHz acoustic mode, a record for diamond in the GHz frequency range and within an order of magnitude of state-of-the-art line widths for OMCs in silicon. We investigate SiV optical and spin properties in these devices and outline a path toward a coherent spin-phonon interface.

Sub-ppm Nanomechanical Absorption Spectroscopy of Silicon Nitride.

Material absorption is a key limitation in nanophotonic systems; however, its characterization is often obscured by scattering and diffraction. Here we show that nanomechanical frequency spectroscopy can be used to characterize material absorption at the parts per million level and use it to characterize the extinction coefficient κ of stoichiometric silicon nitride (Si3N4). Specifically, we track the frequency shift of a high-Q Si3N4 trampoline in response to laser photothermal heating and infer κ from a model including stress relaxation and both conductive and radiative heat transfer. A key insight is the presence of two thermalization time scales: rapid radiative cooling of the Si3N4 film and slow parasitic heating of the Si chip. We infer κ ∼ 0.1-1 ppm for Si3N4 in the 532-1550 nm wavelength range, matching bounds set by waveguide resonators. Our approach is applicable to diverse photonic materials and may offer new insights into their potential.

Unveiling Efficient Acousto-Optic Modulation in Silicon Photonic Devices via Lithium Niobate Using Transfer Printing.

Piezo-optomechanics presents a promising route to convert microwave signals to the optical domain, implementing processing tasks that are challenging using conventional electronics. The surge of integrated photonics facilitates the exploitation of localized light-sound interactions toward new technological paradigms. However, efficient acousto-optic interaction has yet to be fully exploited in silicon due to the absence of piezoelectricity, despite its maturity in photonic integrated circuits. Here, we introduce a distinctive acousto-optic scheme to supplement silicon photonic devices through heterogeneous integration with lithium niobate (LN). Utilizing LN as an efficient acoustic pump to harness the inherently exceptional photoelasticity in silicon, we demonstrate efficient microwave-to-acoustic transduction, ultimately achieving a modulation figure-of-merit of VπL ∼ 0.496 V·cm. This efficient modulation scheme is further extended to implement non-reciprocal intermodal modulation. The proposed hybrid integration route opens new possibilities for tailoring photon-phonon interactions in silicon, consolidating acousto-optic technology in multifunctional integrated photonics.

Acoustic Resonance Tuning by High-Order Lorentzian Mixing.

Nanoscale mechanical resonators have attracted a great deal of attention for signal processing, sensors, and quantum applications. Recent progress in ultrahigh-Q acoustic cavities in nanostructures allows strong interactions with various physical systems and advanced functional devices. Those acoustic cavities are highly sensitive to external perturbations, and it is hard to control those resonance properties since those responses are determined by the geometry and material. In this paper, we demonstrate a novel acoustic resonance tuning method by mixing high-order Lorentzian responses in an optomechanical system. Using weakly coupled phononic-crystal acoustic cavities, we achieve coherent mixing of second- and third-order Lorentzian responses, which is capable of the fine-tunability of the bandwidth and peak frequency of the resonance with a tuning range comparable to the acoustic dissipation rate of the device. This novel resonance tuning method can be widely applied to Lorentzian-response systems and optomechanics, especially active compensation for environmental fluctuation and fabrication errors.

Synthesis and Raman Detection of 5-Amino-2-mercaptobenzimidazole Self-Assembled Monolayers in Nanoparticle-on-a-Mirror Plasmonic Cavity Driven by Dielectric Waveguides.

Functionalization of metallic surfaces by molecular monolayers is a key process in fields such as nanophotonics or biotechnology. To strongly enhance light-matter interaction in such monolayers, nanoparticle-on-a-mirror (NPoM) cavities can be formed by placing metal nanoparticles on such chemically functionalized metallic monolayers. In this work, we present a novel functionalization process of gold surfaces using 5-amino-2-mercaptobenzimidazole (5-A-2MBI) molecules, which can be used for upconversion from THz to visible frequencies. The synthesized surfaces and NPoM cavities are characterized by Raman spectroscopy, atomic force microscopy (AFM), and advancing-receding contact angle measurements. Moreover, we show that NPoM cavities can be efficiently integrated on a silicon-based photonic chip performing pump injection and Raman-signal extraction via silicon nitride waveguides. Our results open the way for the use of 5-A-2MBI monolayers in different applications, showing that NPoM cavities can be effectively integrated with photonic waveguides, enabling on-chip enhanced Raman spectroscopy or detection of infrared and THz radiation.

Anomalous thermodynamic cost of clock synchronization.

Clock synchronization is critically important in positioning, navigation and timing systems. While its performance has been intensively studied in a wide range of disciplines, much less is known for the fundamental thermodynamics of clock synchronization‒what limits the precision and how to optimize the energy cost for clock synchronization. Here, we report the first experimental investigation of two stochastic autonomous clocks synchronization, unveiling the thermodynamic relation between the entropy cost and clock synchronization in an open cavity optomechanical system. Two interacting clocks are synchronized spontaneously owing to the disparate decay rates of hybrid modes by engineering the controllable cavity-mediated dissipative coupling. The measured dependence of the degree of synchronization on the overall entropy cost exhibits an unexpected non-monotonic characteristic, while the relation between the degree of synchronization and the entropy cost for the synchronization is monotonically decreasing. The investigation of transient dynamics of clock synchronization exposes a trade-off between energy and time consumption. Our results demonstrate the possibility of clock synchronization in an effective linear system, reveal the fundamental relation between clock synchronization and thermodynamics, and have a great potential for precision measurements, distributed quantum networks, and biological science.

1/f Noise Mitigation in an Opto-Mechanical Sensor with a Fabry-Pérot Interferometer.

Low-frequency and 1/f noise are common measurement limitations that arise in a variety of physical processes. Mitigation methods for these noises are dependent on their source. Here, we present a method for removing 1/f noise of optical origin using a micro-cavity Fabry-Pérot (FP) interferometer. A mechanical modulation of the FP cavity length was applied to a previously studied opto-mechanical sensor. It effectively mimics an up-conversion of the laser frequency, shifting signals to a region where lower white-noise sources dominate and 1/f noise is not present. Demodulation of this signal shifts the results back to the desired frequency range of observation with the reduced noise floor of the higher frequencies. This method was found to improve sensitivities by nearly two orders of magnitude at 1 Hz and eliminated 1/f noise in the range from 1 Hz to 4 kHz. A mathematical model for low-finesse FP cavities is presented to support these results. This study suggests a relatively simple and efficient method for 1/f noise suppression and improving the device sensitivity of systems with an FP interferometer readout.

Molecular Optomechanics Induced Hybrid Properties in Soft Materials Filled Plasmonic Nanocavities.

The optomechanical interaction between nanocavity plasmons and molecular vibrations can result in interfacial phenomena that can be tailored for sensing and photocatalytic applications. Here, we report for the first time that plasmon-vibration interaction can induce laser-plasmon detuning dependent plasmon resonance linewidth broadening, indicating energy transfer from the plasmon field to collective vibrational modes. The linewidth broadening accompanied by the large enhancement of the Raman scattering signal is observed as the laser-plasmon blue-detuning approaches the CH vibrational frequency of the molecular systems integrated in gold nanorod-on-mirror nanocavities. The experimental observations can be explained based on the molecular optomechanics theory that predicts dynamical backaction amplification of the vibrational modes and high sensitivity of Raman scattering when the plasmon resonance overlaps with the Raman emission frequency. The results presented here suggest that molecular optomechanics coupling may be manipulated for creating hybrid properties based on interactions between molecular oscillators and nanocavity electromagnetic optical modes.

Ultrathin Tunable Optomechanical Metalens.

Reconfigurable metasurfaces offer great promises to enhance photonics technology by combining integration with improved functionalities. Recently, reconfigurability in otherwise static metasurfaces has been achieved by modifying the electric permittivity of the meta-atoms themselves or their immediate surrounding. Yet, it remains challenging to achieve significant and fast tunability without increasing bulkiness. Here, we demonstrate an ultrathin tunable metalens whose focal distance can be changed through optomechanical control with moderate continuous wave intensities. We achieve fast focal length changes of more than 5% with response time of the order of 10 µs.

High-Q Trampoline Resonators from Strained Crystalline InGaP for Integrated Free-Space Optomechanics.

Nanomechanical resonators realized from tensile-strained materials reach ultralow mechanical dissipation in the kHz to MHz frequency range. Tensile-strained crystalline materials that are compatible with epitaxial growth of heterostructures would thereby at the same time allow realizing monolithic free-space optomechanical devices, which benefit from stability, ultrasmall mode volumes, and scalability. In our work, we demonstrate nanomechanical string and trampoline resonators made from tensile-strained InGaP, which is a crystalline material that is epitaxially grown on an AlGaAs heterostructure. We characterize the mechanical properties of suspended InGaP nanostrings, such as anisotropic stress, yield strength, and intrinsic quality factor. We find that the latter degrades over time. We reach mechanical quality factors surpassing 107 at room temperature with a Q·f product as high as 7 × 1011Hz with trampoline-shaped resonators. The trampoline is patterned with a photonic crystal to engineer its out-of-plane reflectivity, desired for efficient signal transduction of mechanical motion to light.

Near-Field GHz Rotation and Sensing with an Optically Levitated Nanodumbbell.

A levitated nonspherical nanoparticle in a vacuum is ideal for studying quantum rotations and is an ultrasensitive torque detector for probing fundamental particle-surface interactions. Here, we optically levitate a silica nanodumbbell in a vacuum at 430 nm away from a sapphire surface and drive it to rotate at GHz frequencies. The relative linear speed between the tip of the nanodumbbell and the surface reaches 1.4 km s-1 at a submicrometer separation. The rotating nanodumbbell near the surface demonstrates a torque sensitivity of (5.0 ± 1.1) × 10-26 N m Hz-1/2 at room temperature. Moreover, we probed the near-field laser intensity distribution beyond the optical diffraction limit with a nanodumbbell levitated near a nanograting. Our numerical simulations show that the system can measure the Casimir torque and will improve the detection limit of non-Newtonian gravity by several orders of magnitude.

Radiation Pressure Backaction on a Hexagonal Boron Nitride Nanomechanical Resonator.

Hexagonal boron nitride (hBN) is a van der Waals material with excellent mechanical properties hosting quantum emitters and optically active spin defects, with several of them being sensitive to strain. Establishing optomechanical control of hBN will enable hybrid quantum devices that combine the spin degree of freedom with the cavity optomechanical toolbox. In this Letter, we report the first observation of radiation pressure backaction at telecom wavelengths with a hBN drum-head mechanical resonator. The thermomechanical motion of the resonator is coupled to the optical mode of a high finesse fiber-based Fabry-Pérot microcavity in a membrane-in-the-middle configuration. We are able to resolve the optical spring effect and optomechanical damping with a single photon coupling strength of g0/2π = 1200 Hz. Our results pave the way for tailoring the mechanical properties of hBN resonators with light.

Coupling of light and mechanics in a photonic crystal waveguide.

Observations of thermally driven transverse vibration of a photonic crystal waveguide (PCW) are reported. The PCW consists of two parallel nanobeams whose width is modulated symmetrically with a spatial period of 370 nm about a 240-nm vacuum gap between the beams. The resulting dielectric structure has a band gap (i.e., a photonic crystal stop band) with band edges in the near infrared that provide a regime for transduction of nanobeam motion to phase and amplitude modulation of an optical guided mode. This regime is in contrast to more conventional optomechanical coupling by way of moving end mirrors in resonant optical cavities. Models are developed and validated for this optomechanical mechanism in a PCW for probe frequencies far from and near to the dielectric band edge (i.e., stop band edge). The large optomechanical coupling strength predicted should make possible measurements with an imprecision below that at the standard quantum limit and well into the backaction-dominated regime. Since our PCW has been designed for near-field atom trapping, this research provides a foundation for evaluating possible deleterious effects of thermal motion on optical atomic traps near the surfaces of PCWs. Longer-term goals are to achieve strong atom-mediated links between individual phonons of vibration and single photons propagating in the guided modes (GMs) of the PCW, thereby enabling optomechanics at the quantum level with atoms, photons, and phonons. The experiments and models reported here provide a basis for assessing such goals.

All-Optical, Air-Coupled Ultrasonic Detection of Low-Pressure Gas Leaks and Observation of Jet Tones in the MHz Range.

We used an ultrasensitive, broadband optomechanical ultrasound sensor to study the acoustic signals produced by pressurized nitrogen escaping from a variety of small syringes. Harmonically related jet tones extending into the MHz region were observed for a certain range of flow (i.e., Reynolds number), which is in qualitative agreement with historical studies on gas jets emitted from pipes and orifices of much larger dimensions. For higher turbulent flow rates, we observed broadband ultrasonic emission in the ~0-5 MHz range, which was likely limited on the upper end due to attenuation in air. These observations are made possible by the broadband, ultrasensitive response (for air-coupled ultrasound) of our optomechanical devices. Aside from being of theoretical interest, our results could have practical implications for the non-contact monitoring and detection of early-stage leaks in pressured fluid systems.

Real-Time Sensing with Multiplexed Optomechanical Resonators.

Nanoelectromechanical resonators have been successfully used for a variety of sensing applications. Their extreme resolution comes from their small size, which strongly limits their capture area. This leads to a long analysis time and the requirement for large sample quantity. Moreover, the efficiency of the electrical transductions commonly used for silicon resonators degrades with increasing frequency, limiting the achievable mechanical bandwidth and throughput. Multiplexing a large number of high-frequency resonators appears to be a solution, but this is complex with electrical transductions. We propose here a route to solve these issues, with a multiplexing scheme for very high-frequency optomechanical resonators. We demonstrate the simultaneous frequency measurement of three silicon microdisks fabricated with a 200 mm wafer large-scale process. The readout architecture is simple and does not degrade the sensing resolutions. This paves the way toward the realization of sensors for multiparametric analysis with an extremely low limit of detection and response time.

Geometric Tuning of Stress in Predisplaced Silicon Nitride Resonators.

We introduce a novel method to geometrically tune the tension in prestrained resonators by making Si3N4 strings with a designed predisplacement. This enables us, for example, to study their dissipation mechanisms, which are strongly dependent on the stress. After release of the resonators from the substrate, their static displacement is extracted using scanning electron microscopy. The results match finite-element simulations, which allows a quantitative determination of the resulting stress. The in- and out-of-plane eigenmodes are sensed using on-chip Mach-Zehnder interferometers, and the resonance frequencies and quality factors are extracted. The geometrically controlled stress enables tuning not only of the frequencies but also of the damping rate. We develop a model that quantitatively captures the stress dependence of the dissipation in the same SiN film. We show that the predisplacement shape provides additional flexibility, including control over the frequency ratio and the quality factor for a targeted frequency.

Superconducting Vortex-Charge Measurement Using Cavity Electromechanics.

As the magnetic field penetrates the surface of a superconductor, it results in the formation of flux vortices. It has been predicted that the flux vortices will have a charged vortex core and create a dipolelike electric field. Such a charge trapping in vortices is particularly enhanced in high-Tc superconductors (HTS). Here, we integrate a mechanical resonator made of a thin flake of HTS Bi2Sr2CaCu2O8+δ into a microwave circuit to realize a cavity-electromechanical device. Due to the exquisite sensitivity of cavity-based devices to the external forces, we directly detect the charges in the flux vortices by measuring the electromechanical response of the mechanical resonator. Our measurements reveal the strength of surface electric dipole moment due to a single vortex core to be approximately 30 |e|aB, equivalent to a vortex charge per CuO2 layer of 3.7 × 10-2|e|, where aB is the Bohr radius and e is the electronic charge.

Low Noise Opto-Electro-Mechanical Modulator for RF-to-Optical Transduction in Quantum Communications.

In this work, we present an Opto-Electro-Mechanical Modulator (OEMM) for RF-to-optical transduction realized via an ultra-coherent nanomembrane resonator capacitively coupled to an rf injection circuit made of a microfabricated read-out able to improve the electro-optomechanical interaction. This device configuration can be embedded in a Fabry-Perot cavity for electromagnetic cooling of the LC circuit in a dilution refrigerator exploiting the opto-electro-mechanical interaction. To this aim, an optically measured steady-state frequency shift of 380 Hz was seen with a polarization voltage of 30 V and a Q-factor of the assembled device above 106 at room temperature. The rf-sputtered titanium nitride layer can be made superconductive to develop efficient quantum transducers.