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1.
Philos Trans A Math Phys Eng Sci ; 380(2215): 20210108, 2022 Jan 24.
Article in English | MEDLINE | ID: mdl-34865528

ABSTRACT

Removing methane from the air is possible, but do the costs outweigh the benefits? This note explores the question of whether removing methane from the atmosphere is justifiable. Destruction of methane by oxidation to CO2 eliminates 97% of the warming impact on a 100-yr time scale. Methane can be oxidized by a variety of methods including thermal or ultraviolet photocatalysis and various processes of physical, chemical or biological oxidizers. Each removal method has energy costs (with the risk of causing embedded CO2 emission that cancel the global warming gain), but in specific circumstances, including settings where air with high methane is habitually present, removal may be competitive with direct efforts to cut fugitive methane leaks. In all cases however, great care must be taken to ensure that the destruction has a net positive impact on the total global warming, and that the resources required would not be better used for stopping the methane from being emitted. This article is part of a discussion meeting issue 'Rising methane: is warming feeding warming? (part 2)'.


Subject(s)
Methane , Oxidation-Reduction
2.
Environ Sci Technol ; 55(13): 8583-8591, 2021 07 06.
Article in English | MEDLINE | ID: mdl-34159780

ABSTRACT

Megacities, with their large and complex infrastructures, are significant sources of methane emissions. To develop a simple, low-cost methodology to quantify these globally important methane sources, this study focuses on mobile measurements of methane (CH4) and its isotopic composition in Paris. Data collected between September 2018 to March 2019 resulted in 17 days of measurements, which provided spatial distribution of street-level methane mixing ratios, source type identification, and emission quantification. Consequently, 90 potential leaks were detected in Paris sorted into three leak categories: natural gas distribution network emissions (63%), sewage network emissions (33%), and emissions from heating furnaces of buildings (4%). The latter category has not previously been reported in urban methane studies. Accounting for the detectable emissions from the ground, the total estimated CH4 emission rate of Paris was 5000 L/min (190 t/yr), with the largest contribution from gas leaks (56%). This ranks Paris as a city with medium CH4 emissions. Two areas of clusters were found, where 22% and 56% of the total potential emissions of Paris were observed. Our findings suggest that the natural gas distribution network, the sewage system, and furnaces of buildings are ideal targets for street-level CH4 emission reduction efforts for Paris.


Subject(s)
Air Pollutants , Methane , Air Pollutants/analysis , Cities , France , Methane/analysis , Natural Gas/analysis
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