Permittivity tensor imaging: modular label-free imaging of 3D dry mass and 3D orientation at high resolution.

The dry mass and the orientation of biomolecules can be imaged without a label by measuring their permittivity tensor (PT), which describes how biomolecules affect the phase and polarization of light. Three-dimensional (3D) imaging of PT has been challenging. We present a label-free computational microscopy technique, PT imaging (PTI), for the 3D measurement of PT. PTI encodes the invisible PT into images using oblique illumination, polarization-sensitive detection and volumetric sampling. PT is decoded from the data with a vectorial imaging model and a multi-channel inverse algorithm, assuming uniaxial symmetry in each voxel. We demonstrate high-resolution imaging of PT of isotropic beads, anisotropic glass targets, mouse brain tissue, infected cells and histology slides. PTI outperforms previous label-free imaging techniques such as vector tomography, ptychography and light-field imaging in resolving the 3D orientation and symmetry of organelles, cells and tissue. We provide open-source software and modular hardware to enable the adoption of the method.

Double-clad ytterbium-doped tapered fiber with circular birefringence as a gain medium for structured light.

Amplifying radially and azimuthally polarized beams is a significant challenge due to the instability of the complex beam shape and polarization in inhomogeneous environment. In this Letter, we demonstrated experimentally an efficient approach to directly amplify cylindrical-vector beams with axially symmetric polarization and doughnut-shaped intensity profile in a picosecond MOPA system based on a double-clad ytterbium-doped tapered fiber. To prevent polarization and beam shape distortion during amplification, for the first time to the best of our knowledge, we proposed using the spun architecture of the tapered fiber. In contrast to an isotropic fiber architecture, a spun configuration possessing nearly circular polarization eigenstates supports stable wavefront propagation. Applying this technique, we amplified the cylindrical-vector beam with 10 ps pulses up to 22 W of the average power at a central wavelength of 1030 nm and a repetition rate of 15 MHz, maintaining both mode and polarization stability.

Controlling ultrafast laser writing in silica glass by pulse temporal contrast.

We demonstrate that the temporal contrast of femtosecond light pulses is a critical parameter in laser writing inside transparent dielectrics, allowing different material modifications. In particular, anisotropic nanopores in silica glass are produced by high-contrast of 107 femtosecond Yb:KGW laser pulses rather than low-contrast of 103 Yb fiber laser pulses. The difference originates in the fiber laser storing a third of its energy in a post-pulse of up to 200 ps duration. The absorption of this low-intensity fraction of the pulse by laser-induced transient defects with relatively long lifetime and low excitation energy, such as self-trapped holes, drastically changes the kinetics of energy deposition and the type of material modification. We also demonstrate that low-contrast pulses are effective in creating lamellar birefringent structures, possibly driven by a quadrupole nonlinear current.

High damage threshold birefringent elements produced by ultrafast laser nanostructuring in silica glass.

Birefringent patterning by ultrafast laser nanostructuring in silica glass has been used for space-variant birefringent optics with high durability and high optical damage threshold. We demonstrate that the oblate-shaped birefringent modification (type X) with ultrahigh optical transmission has higher optical damage resistance, comparable to pristine silica glass. The lower damage threshold of nanogratings based modification (type 2) following thermal annealing at 900°C for an hour is improved from 0.96 J/cm2 to 1.62 J/cm2 for 300 fs laser pulses and approaches the optical damage threshold of type X (1.56 J/cm2). This opens the door to utilize these optical elements for high power laser applications where optical transmission and damage threshold are the key parameters. The lower damage threshold of type 2 modification is related to the relatively high concentration of defects, such as E' centers and oxygen-deficiency centers (ODCs).

Actively Q switched radially polarized Ho:YAG laser with an intra-cavity laser-written S-waveplate.

Nanosecond Q switched pulses and radial polarization are established stand-alone techniques for enhanced laser materials processing applications, but are generally challenging to achieve simultaneously at high average power levels. Here, we demonstrate a 20.6 W radially polarized Ho:YAG rod laser which has been actively Q switched in order to generate 515 µJ, 210 ns pulses at 2097 nm. By utilizing an ultra-low-loss spatially variant birefringent wave plate (S-waveplate) inside the laser cavity, the linearly polarized fundamental mode has been converted to a radially polarized donut-shaped beam with very high conversion efficiency.

Broadband fiber-based entangled photon-pair source at telecom O-band.

In this Letter, we report a polarization-entangled photon-pair source based on type-II spontaneous parametric downconversion at telecom O-band in periodically poled silica fiber (PPSF). The photon-pair source exhibits more than 130 nm (∼24THz) emission bandwidth centered at 1306.6 nm. The broad emission spectrum results in a short biphoton correlation time, and we experimentally demonstrate a Hong-Ou-Mandel interference dip with a full width of 26.6 fs at half-maximum. Owing to the low birefringence of the PPSF, the biphotons generated from type-II SPDC are polarization-entangled over the entire emission bandwidth, with a measured fidelity to a maximally entangled state greater than 95.4%. The biphoton source provides the broadest bandwidth entangled biphotons at O-band to our knowledge.

Dispersion measurement assisted by a stimulated parametric process.

Dispersion plays a major role in the behavior of light inside photonic devices. Current state-of-the-art dispersion measurement techniques utilize linear interferometers that can be applied to devices with small dispersion-length products. However, linear interferometry often requires beam alignment and phase stabilization. Recently, common-path nonlinear interferometers in the spontaneous regime have been used to demonstrate alignment-free and phase-stable dispersion measurements. However, they require single-photon detectors, resulting in high system cost and long integration times. We overcome these issues by utilizing a nonlinear interferometer in the stimulated regime and demonstrate the ability to measure the dispersion of a device with a dispersion-length product as small as 0.009 ps/nm at a precision of 0.0002 ps/nm. Moreover, this regime allows us to measure dispersion with shorter integration times (in comparison to the spontaneous regime) and conventional optical components and detectors.

Alignment-free dispersion measurement with interfering biphotons.

Measuring the dispersion of photonic devices with small dispersion-length products is challenging due to the phase-sensitive and alignment-intensive nature of conventional methods. In this Letter, we demonstrate a quantum technique to extract the second- and third-order chromatic dispersion of a short single-mode fiber using a fiber-based quantum nonlinear interferometer. The interferometer consists of two cascaded fiber-based biphoton sources, with each source acting as a nonlinear beam splitter. A fiber under test is placed between these two sources and introduces a frequency-dependent phase that is imprinted on the biphoton spectrum (interferogram) at the output of the interferometer. This interferogram contains the dispersion properties of the test fiber. Our technique has three novel features: (1) the broadband nature of the biphoton sources used in our setup allows accurate dispersion measurements on test devices with small dispersion-length products; (2) our all-fiber common-path interferometer requires no beam alignment or phase stabilization; and (3) multiple phase-matching processes supported in our biphoton sources enable dispersion measurements at different wavelengths, which yields the third-order dispersion achieved for the first time, to the best of our knowledge, using a quantum optical technique.

Ultrafast laser-induced birefringence in various porosity silica glasses: from fused silica to aerogel.

We compare a femtosecond laser induced modification in silica matrices with three different degrees of porosity. In single pulse regime, the decrease of substrate density from fused silica to high-silica porous glass and to silica aerogel glass results in tenfold increase of laser affected region with the formation of a symmetric cavity surrounded by the compressed silica shell with pearl like structures. In multi-pulse regime, if the cavity produced by the first pulse is relatively large, the subsequent pulses do not cause further modifications. If not, the transition from void to the anisotropic structure with the optical axis oriented parallel to the incident polarization is observed. The maximum retardance value achieved in porous glass is twofold higher than in fused silica, and tenfold greater than in aerogel. The polarization sensitive structuring in porous glass by two pulses of ultrafast laser irradiation is demonstrated, as well as no observable stress is generated at any conditions.

Compensation-free broadband entangled photon pair sources.

Quantum sources that provide broadband biphotons entangled in both polarization and time-energy degrees of freedom are a rich quantum resource that finds many applications in quantum communication, sensing, and metrology. Creating such a source while maintaining high entanglement quality over a broad spectral range is a challenge, which conventionally requires various compensation steps to erase temporal, spectral, or spatial distinguishabilities. Here, we point out that in fact compensation is not always necessary. The key to generate broadband polarization-entangled biphotons via type-II spontaneous parametric downcoversion (SPDC) without compensation is to use nonlinear materials with sufficiently low group birefringence that the biphoton bandwidth becomes dispersion-limited. Most nonlinear crystals or waveguides cannot meet this condition, but it is easily met in fiber-based systems. We reveal the interplay of group birefringence and dispersion on SPDC bandwidth and polarization entanglement quality. We show that periodically poled silica fiber (PPSF) is an ideal medium to generate high-concurrence (>0.977) polarization-entangled photons over a broad spectral range (>77nm), directly and without compensation. This is the highest polarization-entanglement concurrence reported that is maintained over a broad spectral range from a compensation-free source.

Void-nanograting transition by ultrashort laser pulse irradiation in silica glass.

The structural evolution from void modification to self-assembled nanogratings in fused silica is observed for moderate (NA > 0.4) focusing conditions. Void formation, appears before the geometrical focus after the initial few pulses and after subsequent irradiation, nanogratings gradually occur at the top of the induced structures. Nonlinear Schrödinger equation based simulations are conducted to simulate the laser fluence, intensity and electron density in the regions of modification. Comparing the experiment with simulations, the voids form due to cavitation in the regions where electron density exceeds 1020 cm-3 but is below critical. In this scenario, the energy absorption is insufficient to reach the critical electron density that was once assumed to occur in the regime of void formation and nanogratings, shedding light on the potential formation mechanism of nanogratings.

Tailored surface birefringence by femtosecond laser assisted wet etching.

Surface texturing is demonstrated by the combination of wet etching and ultrafast laser nanostructuring of silica glass. Using potassium hydroxide (KOH) at room temperature as an etchant of laser modified glass, we show the polarization dependent linear increase in retardance reaching a threefold value within 25 hours. The dispersion control of birefringence by the etching procedure led to achromatic behaviour over the entire visible spectral range. The mechanism of enhanced KOH etching selectivity after femtosecond laser exposure is discussed and correlated to the formation of various laser-induced defects, such as silicon-rich oxygen deficiency and color centers.

Airy beams generated by ultrafast laser-imprinted space-variant nanostructures in glass.

We demonstrate a technique to generate accelerating Airy beams with a femtosecond laser-imprinted space variant birefringent structure in silica glass. Our approach enables the generation of dual Airy beams with polarization sensitive beam deflection. The produced beam is used for the glass scribing. After the glass-breaking process, a spontaneous self-detachment of a fiber-like structure occurs that can be exploited as an alternative way for fabricating glass cantilevers.

All-fiber frequency-doubled visible laser.

All-fiber ns-pulsed visible laser at λ=521 nm is realized by frequency doubling an Yb-doped fiber laser with a periodically poled silica fiber. A 50-mW second-harmonic (SH) output power is produced that is over 6-orders of magnitude greater than previous results obtained with poled fibers in the visible spectral range. The normalized conversion efficiency of 0.3%/W is to date the largest demonstrated with poled fiber technology. Furthermore, 21% conversion efficiency is achieved for the doubling of 8-ps pulses from a neodymium-doped yttrium vanadate solid-state laser. The advances are made possible by the precision and flexibility offered by using the continuous periodic UV erasure, as opposite to photolithographic methods, for the fabrication of over 20-cm-long χ(2)-gratings for quasi-phase matched SH generation.

Seemingly unlimited lifetime data storage in nanostructured glass.

We demonstrate recording and retrieval of the digital document with a nearly unlimited lifetime. The recording process of multiplexed digital data was implemented by femtosecond laser nanostructuring of fused quartz. The storage allows unprecedented parameters including hundreds of terabytes per disc data capacity, thermal stability up to 1000 °C, and virtually unlimited lifetime at room temperature. We anticipate that this demonstration will open a new era of eternal data archiving.

Femtosecond versus picosecond laser machining of nano-gratings and micro-channels in silica glass.

The ability of 8 picosecond pulse lasers for three dimensional direct-writing in the bulk of transparent dielectrics is assessed through a comparative study with a femtosecond laser delivering 600 fs pulses. The comparison addresses two main applications: the fabrication of birefringent optical elements and two-step machining by laser exposure and post-processing by chemical etching. Formation of self-organized nano-gratings in glass by ps-pulses is demonstrated. Differential etching between ps-laser exposed regions and unexposed silica is observed. Despite attaining values of retardance (>100 nm) and etching rate (2 µm/min) similar to fs pulses, ps pulses are found unsuitable for bulk machining in silica glass primarily due to the build-up of a stress field causing scattering, cracks and non-homogeneous etching. Additionally, we show that the so-called "quill-effect", that is the dependence of the laser damage from the direction of writing, occurs also for ps-pulse laser machining. Finally, an opposite dependence of the retardance from the intra-pulse distance is observed for fs- and ps-laser direct writing.

Extraordinary anisotropy of ultrafast laser writing in glass.

The unusual dependence of femtosecond laser writing on the light polarization and direction of raster scanning is demonstrated in silica and chalcogenide glasses. Two different mechanisms contributing to the observed anisotropy are identified: the chevron-shaped stress induced by the sample movement and the pulse front tilt of ultrashort light pulse. Control of anisotropies associated with the spatio-temporal asymmetry of an ultrashort pulse beam and scanning geometry is crucial in the ultrafast laser machining of transparent materials.

Polarization sensitive camera by femtosecond laser nanostructuring.

A polarization imaging device based on a femtosecond laser nanostructured birefringent array is demonstrated. The device enables instant measurement of the distribution of the Stokes vectors in the visible spectrum. Polarimetric measurements with radially and circularly polarized light distributions are demonstrated.

3D Imprinting of Voxel-Level Structural Colors in Lithium Niobate Crystal.

Advanced coloration methods are of pivotal importance in science, technology, and engineering. However, 3D structural colors that are critical for emerging multidimensional information representation and recording are rarely achievable. Here, a facile voxel-level programmable 3D structural coloration in the bulk lithium niobate (LiNbO3 ) crystal is reported. This is achieved by engineering wavelength-selective interference between ordinary (O) and extraordinary (E) light in the crystal matrix. To induce effective phase contrast between O and E light for establishing the highly localized interference across the visible band, the presence of a pulse-internal-coupling effect is revealed in the single-pulse ultrafast laser-crystal interaction and an ultrafast-laser-induced micro-amorphization (MA) strategy is thus developed to manipulate local matrix structure. Consequently, micro-nanoscale colorful voxels can be fast inscribed into any spatial position of the crystal matrix in one step. It is demonstrated that the colors can be flexibly manipulated and quickly extracted in 3D space. Multidimensional MA-color data storage with large capacity, high writing and readout speed, long lifetime, and excellent stability under harsh conditions is achieved. The present principle enables multifunctional 3D structural coloration devices inside high-refractive-index transparent dielectrics and can serve as a general platform to innovate next-generation information optics.

Efficient ultrafast laser writing with elliptical polarization.

Photosensitivity in nature is commonly associated with stronger light absorption. It is also believed that artificial optical anisotropy to be the strongest when created by light with linear polarization. Contrary to intuition, ultrafast laser direct writing with elliptical polarization in silica glass, while nonlinear absorption is about 2.5 times weaker, results in form birefringence about twice that of linearly polarized light. Moreover, a larger concentration of anisotropic nanopores created by elliptically polarized light pulses is observed. The phenomenon is interpreted in terms of enhanced interaction of circularly polarized light with a network of randomly oriented bonds and hole polarons in silica glass, as well as efficient tunneling ionization produced by circular polarization. Applications to multiplexed optical data storage and birefringence patterning in silica glass are demonstrated.