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1.
Proc Natl Acad Sci U S A ; 115(27): 6995-6999, 2018 07 03.
Artículo en Inglés | MEDLINE | ID: mdl-29915042

RESUMEN

A phase transition occurs when correlated regions of a new phase grow to span the system and the fluctuations within the correlated regions become long lived. Here, we present neutron scattering measurements showing that this conventional picture must be replaced in YFe2Al10, a compound that forms naturally very close to a [Formula: see text] quantum phase transition. Fully quantum mechanical fluctuations of localized moments are found to diverge at low energies and temperatures; however, the fluctuating moments are entirely without spatial correlations. Zero temperature order in YFe2Al10 is achieved by an entirely local type of quantum phase transition that may originate with the creation of the moments themselves.

2.
Phys Rev Lett ; 126(17): 179601, 2021 Apr 30.
Artículo en Inglés | MEDLINE | ID: mdl-33988444
3.
Phys Rev Lett ; 111(6): 067204, 2013 Aug 09.
Artículo en Inglés | MEDLINE | ID: mdl-23971608

RESUMEN

The S=1/2 spin chain material SrCuO2 doped with 1% S=1 Ni impurities is studied by inelastic neutron scattering. At low temperatures, the spectrum shows a pseudogap Δ≈8 meV, absent in the parent compound, and not related to any structural phase transition. The pseudogap is shown to be a generic feature of quantum spin chains with dilute defects. A simple model based on this idea quantitatively accounts for the experimental data measured in the temperature range from 2 to 300 K, and allows us to represent the momentum-integrated dynamic structure factor in a universal scaling form.

4.
Phys Rev Lett ; 105(4): 046804, 2010 Jul 23.
Artículo en Inglés | MEDLINE | ID: mdl-20867875

RESUMEN

The magnetotransport in single layer graphene has been experimentally investigated in magnetic fields up to 18 T as a function of temperature. A pronounced T dependence is observed for T≲50 K, which is either metallic, or insulating, depending on the filling factor ν. The metal-insulator transition (MIT) occurs at |ν{c}|∼0.65 and in the regime of the dissipative transport, where the longitudinal resistance Rxx>1/2R{K}. The critical resistivity (Rxx per square) is ρ{xx}(ν{c})≈1/2R{K} and is correlated with the appearance of zero plateau in Hall conductivity σ{xy}(ν) and peaks in σ{xx}(ν). This leads us to construct a universal low-T (n, B) phase diagram of this quantum phase transition.

5.
J Phys Condens Matter ; 32(37): 374003, 2019 Aug 14.
Artículo en Inglés | MEDLINE | ID: mdl-31412327

RESUMEN

Neutron scattering has played a significant role in characterizing magnetic and structural correlations in Fe1+y Te1-x Se x and their connections with superconductivity. Here we review several key aspects of the physics of iron chalcogenide superconductors where neutron studies played a key role. These topics include the phase diagram of Fe1+y Te1-x Se x , where the doping-dependence of structural transitions can be understood from a mapping to the anisotropic random field Ising model. We then discuss orbital-selective Mott physics in the Fe chalcogenide series, where temperature-dependent magnetism in the parent material provided one of the earliest cases for orbital-selective correlation effects in a Hund's metal. Finally, we elaborate on the character of local magnetic correlations revealed by neutron scattering, its dependence on temperature and composition, and the connections to nematicity and superconductivity.

6.
Nat Commun ; 10(1): 1123, 2019 03 08.
Artículo en Inglés | MEDLINE | ID: mdl-30850591

RESUMEN

The fundamental excitations in an antiferromagnetic chain of spins-1/2 are spinons, de-confined fractional quasiparticles that when combined in pairs, form a triplet excitation continuum. In an Ising-like spin chain the continuum is gapped and the ground state is Néel ordered. Here, we report high resolution neutron scattering experiments, which reveal how a magnetic field closes this gap and drives the spin chains in Yb2Pt2Pb to a critical, disordered Luttinger-liquid state. In Yb2Pt2Pb the effective spins-1/2 describe the dynamics of large, Ising-like Yb magnetic moments, ensuring that the measured excitations are exclusively longitudinal, which we find to be well described by time-dependent density matrix renormalization group calculations. The inter-chain coupling leads to the confinement of spinons, a condensed matter analog of quark confinement in quantum chromodynamics. Insensitive to transverse fluctuations, our measurements show how a gapless, dispersive longitudinal mode arises from confinement and evolves with magnetic order.

7.
Science ; 352(6290): 1206-10, 2016 Jun 03.
Artículo en Inglés | MEDLINE | ID: mdl-27257254

RESUMEN

Exotic quantum states and fractionalized magnetic excitations, such as spinons in one-dimensional chains, are generally expected to occur in 3d transition metal systems with spin 1/2. Our neutron-scattering experiments on the 4f-electron metal Yb2Pt2Pb overturn this conventional wisdom. We observe broad magnetic continuum dispersing in only one direction, which indicates that the underlying elementary excitations are spinons carrying fractional spin-1/2. These spinons are the emergent quantum dynamics of the anisotropic, orbital-dominated Yb moments. Owing to their unusual origin, only longitudinal spin fluctuations are measurable, whereas the transverse excitations such as spin waves are virtually invisible to magnetic neutron scattering. The proliferation of these orbital spinons strips the electrons of their orbital identity, resulting in charge-orbital separation.

8.
Phys Rev Lett ; 69(11): 1699-1702, 1992 Sep 14.
Artículo en Inglés | MEDLINE | ID: mdl-10046291
10.
Phys Rev Lett ; 87(1): 017202, 2001 Jul 02.
Artículo en Inglés | MEDLINE | ID: mdl-11461493

RESUMEN

The spin-excitation continuum, expected to dominate the low-energy fluctuation spectrum in the Haldane spin chain around the Brillouin zone center, q = 0, is directly observed by inelastic magnetic neutron scattering in the S = 1 quasi-1D antiferromagnet CsNiCl3. We find that the single mode approximation fails, and that a finite energy width appears in the dynamic correlation function S(q,omega) for q less, similar 0.5 pi. The width increases with decreasing q, while S(q,omega) acquires an asymmetric shape qualitatively similar to that predicted for the two-magnon continuum in the nonlinear sigma-model.

11.
Phys Rev Lett ; 93(8): 087202, 2004 Aug 20.
Artículo en Inglés | MEDLINE | ID: mdl-15447220

RESUMEN

We have investigated the spin dynamics in the strongly correlated chain copper oxide SrCuO2 for energies up to greater, similar 0.6 eV using inelastic neutron scattering. We observe a gapless continuum of magnetic excitations, which is well described by the "Müller ansatz" for the two-spinon continuum in the S=1/2 antiferromagnetic Heisenberg spin chain. The lower boundary of the continuum extends up to approximately 360 meV, which corresponds to an exchange constant J=226(12) meV.

12.
Phys Rev Lett ; 90(8): 087202, 2003 Feb 28.
Artículo en Inglés | MEDLINE | ID: mdl-12633455

RESUMEN

Inelastic neutron scattering was used to probe edge states in a quantum spin liquid. The experiment was performed on finite length antiferromagnetic spin-1 chains in Y2BaNi1-xMgxO5. At finite fields, there is a Zeeman resonance below the Haldane gap. The wave-vector dependence of its intensity provides direct evidence for staggered magnetization at chain ends, which decays exponentially towards the bulk [xi=8(1) at T=0.1 K]. Continuum contributions to the chain-end spectrum indicate interchain segment interactions. We also observe a finite size blueshift of the Haldane gap.

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