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Controlling Monomer Feeding Rate to Achieve Highly Crystalline Covalent Triazine Frameworks.
Liu, Manying; Jiang, Kai; Ding, Xing; Wang, Shaolei; Zhang, Chengxin; Liu, Jing; Zhan, Zhen; Cheng, Guang; Li, Buyi; Chen, Hao; Jin, Shangbin; Tan, Bien.
Afiliación
  • Liu M; Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Luoyu Road No. 1037, 430074, Wuhan, P. R. China.
  • Jiang K; College of Science, Huazhong Agricultural University, Wuhan, 430070, P. R. China.
  • Ding X; College of Science, Huazhong Agricultural University, Wuhan, 430070, P. R. China.
  • Wang S; Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Luoyu Road No. 1037, 430074, Wuhan, P. R. China.
  • Zhang C; Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Luoyu Road No. 1037, 430074, Wuhan, P. R. China.
  • Liu J; Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Luoyu Road No. 1037, 430074, Wuhan, P. R. China.
  • Zhan Z; Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Luoyu Road No. 1037, 430074, Wuhan, P. R. China.
  • Cheng G; Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Luoyu Road No. 1037, 430074, Wuhan, P. R. China.
  • Li B; Department of Chemistry and Materials Innovation Factory, University of Liverpool, Crown Street, L69 7ZD, Liverpool, UK.
  • Chen H; College of Science, Huazhong Agricultural University, Wuhan, 430070, P. R. China.
  • Jin S; Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Luoyu Road No. 1037, 430074, Wuhan, P. R. China.
  • Tan B; Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Luoyu Road No. 1037, 430074, Wuhan, P. R. China.
Adv Mater ; 31(19): e1807865, 2019 May.
Article en En | MEDLINE | ID: mdl-30920709
ABSTRACT
The synthesis of highly crystalline covalent triazine frameworks (CTFs) with ultrastrong covalent bonds (aromatic CN) from the triazine linkage presents a great challenge to synthetic chemists. Herein, the synthesis of highly crystalline CTFs via directly controlling the monomer feeding rate is reported. By tuning the feeding rate of monomers, the crystallization process can be readily governed in a controlled manner in an open system. The sample of CTF-HUST-HC1 with abundant exposed {001} crystal facets has the better crystallinity and thus is selected to study the effect of high crystallinity on photoelectric properties. Owing to the better separation of photogenerated electron-hole pairs and charge transfer, the obtained highly ordered CTF-HUST-HC1 has superior performance in the photocatalytic removal of nitric oxide (NO) than its lesser crystalline counterparts and g-C3 N4 .
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Texto completo: 1 Banco de datos: MEDLINE Idioma: En Año: 2019 Tipo del documento: Article
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Texto completo: 1 Banco de datos: MEDLINE Idioma: En Año: 2019 Tipo del documento: Article