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1.
Bioorg Med Chem Lett ; 23(9): 2495-9, 2013 May 01.
Artículo en Inglés | MEDLINE | ID: mdl-23541647

RESUMEN

Porphyrins and chlorins such as Foscan® have a natural proclivity to accumulate in cancer cells. This trait has made them good candidates for photosensitizers and as imaging agents in phototherapy. In order to improve on cellular selectivity to lower post-treatment photosensitivity bile acid porphyrin bioconjugates have been prepared and investigated in esophageal cancer cells. Bile acids which are known to selectively bind to, or be readily taken up by cancer cells were chosen as targeting moieties. Synthesis of the conjugates was achieved via selective nucleophilic monofunctionalization of 5,10,15,20-tetrahydroxyphenylporphyrins with propargyl bromide followed by Cu(I) mediated cycloaddition with bile acid azides in good yields. The compounds were readily taken up by esophageal cancer cells but showed no PDT activity.


Asunto(s)
Ácidos y Sales Biliares/química , Fármacos Fotosensibilizantes/síntesis química , Catálisis , Línea Celular Tumoral , Supervivencia Celular/efectos de los fármacos , Medios de Contraste/síntesis química , Medios de Contraste/toxicidad , Cobre/química , Reacción de Cicloadición , Neoplasias Esofágicas/tratamiento farmacológico , Neoplasias Esofágicas/patología , Humanos , Pargilina/análogos & derivados , Pargilina/química , Fotoquimioterapia , Fármacos Fotosensibilizantes/uso terapéutico , Fármacos Fotosensibilizantes/toxicidad , Porfirinas/química
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