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1.
Nat Commun ; 15(1): 5376, 2024 Jun 25.
Artículo en Inglés | MEDLINE | ID: mdl-38918409

RESUMEN

Kagome lattice has been actively studied for the possible realization of frustration-induced two-dimensional flat bands and a number of correlation-induced phases. Currently, the search for kagome systems with a nearly dispersionless flat band close to the Fermi level is ongoing. Here, by combining theoretical and experimental tools, we present Sc3Mn3Al7Si5 as a novel realization of correlation-induced almost-flat bands in the kagome lattice in the vicinity of the Fermi level. Our magnetic susceptibility, 27Al nuclear magnetic resonance, transport, and optical conductivity measurements provide signatures of a correlated metallic phase with tantalizing ferromagnetic instability. Our dynamical mean-field calculations suggest that such ferromagnetic instability observed originates from the formation of nearly flat dispersions close to the Fermi level, where electron correlations induce strong orbital-selective renormalization and manifestation of the kagome-frustrated bands. In addition, a significant negative magnetoresistance signal is observed, which can be attributed to the suppression of flat-band-induced ferromagnetic fluctuation, which further supports the formation of flat bands in this compound. These findings broaden a new prospect to harness correlated topological phases via multiorbital correlations in 3d-based kagome systems.

2.
Sci Rep ; 14(1): 9042, 2024 Apr 19.
Artículo en Inglés | MEDLINE | ID: mdl-38641702

RESUMEN

We propose the regularized recurrent inference machine (rRIM), a novel machine-learning approach to solve the challenging problem of deriving the pairing glue function from measured optical spectra. The rRIM incorporates physical principles into both training and inference and affords noise robustness, flexibility with out-of-distribution data, and reduced data requirements. It effectively obtains reliable pairing glue functions from experimental optical spectra and yields promising solutions for similar inverse problems of the Fredholm integral equation of the first kind.

3.
Heliyon ; 10(7): e28056, 2024 Apr 15.
Artículo en Inglés | MEDLINE | ID: mdl-38571631

RESUMEN

Planckian behavior has been recently observed in La1·76Sr0·24CuO4 at the pseudogap critical point. The Planckian behavior takes place in an intriguing quantum metallic state at a quantum critical point. Here, the Planckian behavior was simulated with an energy-independent (or flat) and weakly temperature-dependent electron-boson spectral density (EBSD) function by using a generalized Allen's (Shulga's) formula. We obtained various optical quantities from the flat EBSD function, such as the optical scattering rate, the optical effective mass, and the optical conductivity. These quantities are well fitted with the recently observed Planckian behavior. Fermi-liquid behavior was also simulated with an energy-linear and temperature-independent EBSD function. The EBSD functions agree well with the overall doping- and temperature-dependent trends of the EBSD function obtained from the optically measured spectra of cuprate systems, which can be crucial for understanding the microscopic electron-pairing mechanism for high-Tc superconductivity in cuprates.

4.
Sci Rep ; 13(1): 2527, 2023 Feb 13.
Artículo en Inglés | MEDLINE | ID: mdl-36782013

RESUMEN

We investigated the temperature- and frequency-dependent optical scattering rates in the pseudogap phase of cuprates using model pseudogap and electron-boson spectral density (EBSD) functions. We obtained the scattering rates at various temperatures below and above a given pseudogap temperature using a generalized Allen's (or Sharapov's) formula, which has been used to analyse the measured optical spectra of correlated electron systems with a non-constant density of states at finite temperatures. The pseudogap and EBSD functions should be temperature dependent to simulate the Fermi liquid-like behaviour of underdoped cuprate systems observed in optical studies. Therefore, the observed Fermi liquid-like behaviour can be understood by considering the combined contribution from the T-dependent EBSD function and the T-dependent pseudogap. We also obtained the optical conductivity spectra from the optical scattering rates and analyzed them to investigate intriguing electronic properties. We expect that our results will aid in understanding the Fermi liquid-like optical response in the pseudogap phase and in revealing the microscopic pairing mechanism for superconductivity in cuprates.

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