RESUMEN
The detailed shape of picosecond optical pulses from a free-electron laser (FEL) oscillator has been studied for various cavity detunings. For large values of the cavity detuning the optical pulse develops an exponential leading edge, with a time constant proportional to the applied cavity detuning and the quality factor of the resonator. This behavior has been observed at two separate FELs that have completely different resonator layouts and electron beam characteristics, and using different methods of optical pulse length measurement. The optical pulses have a full width at half maximum time-bandwidth product Deltat(FWHM)Deltaf(FWHM) of 0.2-0.3. The results presented here can be used to predict the optical pulse length and corresponding minimum spectral width that can be generated in a FEL pumped by short electron bunches. This is important for the design of new infrared free-electron laser user facilities, which need to make a balanced choice between short pulses for high temporal resolution and narrow bandwidth for linear and nonlinear spectroscopy.
RESUMEN
Using a free electron laser we have performed midinfrared transmission and reflection measurements in strongly scattering Ge powder. We have studied the wavelength dependence of the scattering properties and the optical absorption. Results indicate that our samples are close (kl(s) approximately 3) to the Anderson localization transition but still above it. This is in contrast to the recently reported strong localization of light (kl(s)<1) in a similar powder of lower refractive index particles (GaAs).
RESUMEN
A gas of Rb atoms in a static electric field has been photoexcited to just above the classical ionization threshold by a phase-locked sequence of two far infrared pulses. A single laser pulse generates a series of ejected electron packets emerging at the saddle point of the potential; each of the ejected packets is characterized by a phase and a chirp. We calculate and measure these phases and chirps using the time dependent interference of the electronic wave function controlled by the delay between the two light pulses.
RESUMEN
We present results of the first vibrational photon-echo, transient-grating, and temperature dependent transient-bleaching experiments on a-Si:H. Using these techniques, and the infrared light of a free electron laser, the vibrational population decay and phase relaxation of the Si-H stretching mode were investigated. Careful analysis of the data indicates that the vibrational energy relaxes directly into Si-H bending modes and Si phonons, with a distribution of rates determined by the amorphous host. Conversely, the pure dephasing appears to be single exponential, and can be modeled by dephasing via two-phonon interactions.
RESUMEN
We report the observation of giant quantum coherence effects in the localized modes of ionized hydrogen in synthetic fluorite. Infrared free induction decay experiments on the substitutional H- center show dramatic modulations at negative delay times due to interference between multiple vibrational levels. Spectrally resolving the degenerate four wave mixing signal allows unambiguous assignments of the participating vibrational states. The dependence of the signal intensity upon the delay path between the exciting free electron laser pulses can be accounted for in terms of the resonant third order polarization with a common dephasing time for the excited states.