Ultrafast all-optical toggle writing of magnetic bits without relying on heat.

Ultrafast excitation of matter can violate Curie's principle that the symmetry of the cause must be found in the symmetry of the effect. For instance, heating alone cannot result in a deterministic reversal of magnetization. However, if the heating is ultrafast, it facilitates toggle switching of magnetization between stable bit-states without any magnetic field. Here we show that the regime of ultrafast toggle switching can be also realized via a mechanism without relying on heat. Ultrafast laser excitation of iron-garnet with linearly polarized light modifies magnetic anisotropy and thus causes toggling magnetization between two stable bit states. This new regime of 'cold' toggle switching can be observed in ferrimagnets without a compensation point and over an exceptionally broad temperature range. The control of magnetic anisotropy required for the toggle switching exhibits reduced dissipation compared to laser-induced-heating mechanism, however the dissipation and the switching-time are shown to be competing parameters.

Dynamic complex opto-magnetic holography.

Despite recent significant progress in real-time, large-area computer-generated holography, its memory requirements and computational loads will be hard to tackle for several decades to come with the current paradigm based on a priori calculations and bit-plane writing to a spatial light modulator. Here we experimentally demonstrate a holistic approach to serial computation and repeatable writing of computer-generated dynamic holograms without Fourier transform, using minimal amounts of computer memory. We use the ultrafast opto-magnetic recording of holographic patterns in a ferrimagnetic film with femtosecond laser pulses, driven by the on-the-fly hardware computation of a single holographic point. The intensity-threshold nature of the magnetic medium allows sub-diffraction-limited, point-by-point toggling of arbitrarily localized magnetic spots on the sample, according to the proposed circular detour-phase encoding, providing complex modulation and symmetrical suppression of upper diffractive orders and conjugated terms in holographically reconstructed 3-D images.

Single-shot imaging of ultrafast all-optical magnetization dynamics with a spatiotemporal resolution.

We present a laboratory system for single-shot magneto-optical (MO) imaging of ultrafast magnetization dynamics with less than 8 fs temporal, micrometer spatial resolutions and a MO Faraday's rotation sensitivity of 4 mdeg/µm. We create a stack of MO images repeatedly employing a single pair of pump and defocused probe pulses to induce and visualize MO changes in the sample. Both laser beams are independently wavelength-tunable, allowing for a flexible, resonant adjustable two-color pump and probe scheme. To increase the MO contrast, the probe beam is spatially filtered through a 50 µm aperture. We performed the all-optical switching experiment in Co-doped yttrium iron garnet films (YIG:Co) to demonstrate the capability of the presented method. We determine the spatiotemporal distribution of the effective field of photo-induced anisotropy, driving the all-optical switching of the magnetization in the YIG:Co film without an external magnetic field. Moreover, using this imaging method, we tracked the process of the laser-induced magnetization precession.

Selection rules for all-optical magnetic recording in iron garnet.

Rapid growth of the area of ultrafast magnetism has allowed to achieve a substantial progress in all-optical magnetic recording with femtosecond laser pulses and triggered intense discussions about microscopic mechanisms responsible for this phenomenon. The typically used metallic medium nevertheless considerably limits the applications because of the unavoidable heat dissipation. In contrast, the recently demonstrated photo-magnetic recording in transparent dielectric garnet for all practical purposes is dissipation-free. This discovery raised question about selection rules, i.e. the optimal wavelength and the polarization of light, for such a recording. Here we report the computationally and experimentally identified workspace of parameters allowing photo-magnetic recording in Co-doped iron garnet using femtosecond laser pulses. The revealed selection rules indicate that the excitations responsible for the coupling of light to spins are d-d electron transitions in octahedral and tetrahedral Co-sublattices, respectively.

Spiral magnetic domain structure in cylindrically-shaped microwires.

Identification and characterisation of novel and unusual magnetization states remains a topic of research in modern magnetism. Recently, control of the magnetization state between the surface and volume in cylindrical microwires with the giant magneto-impedance effect has been demonstrated. Herein, the phenomenon of spatial migration of spiral magnetic domains inside a microwire is demonstrated using the magneto-optical Kerr effect. The main properties of the inclined spiral structure were determined, where the surface domain structure possessed a length limited only by actual sample length. Transformation of the structure from a spiral to an elliptical structure could be controlled by external torsion stress. Hysteresis and magnetic images were simulated based on a model assuming a spatial distribution of the internal stress inside the microwire, whose results were consistent with the experimental results. A consistent interpretation of the results in terms of the formation and transformation of the spiral magnetic domain structure is proposed.

Ultrafast nonthermal photo-magnetic recording in a transparent medium.

Discovering ways to control the magnetic state of media with the lowest possible production of heat and at the fastest possible speeds is important in the study of fundamental magnetism, with clear practical potential. In metals, it is possible to switch the magnetization between two stable states (and thus to record magnetic bits) using femtosecond circularly polarized laser pulses. However, the switching mechanisms in these materials are directly related to laser-induced heating close to the Curie temperature. Although several possible routes for achieving all-optical switching in magnetic dielectrics have been discussed, no recording has hitherto been demonstrated. Here we describe ultrafast all-optical photo-magnetic recording in transparent films of the dielectric cobalt-substituted garnet. A single linearly polarized femtosecond laser pulse resonantly pumps specific d-d transitions in the cobalt ions, breaking the degeneracy between metastable magnetic states. By changing the polarization of the laser pulse, we deterministically steer the net magnetization in the garnet, thus writing '0' and '1' magnetic bits at will. This mechanism outperforms existing alternatives in terms of the speed of the write-read magnetic recording event (less than 20 picoseconds) and the unprecedentedly low heat load (less than 6 joules per cubic centimetre).

Direct imaging of the magnetization reversal in microwires using all-MOKE microscopy.

We report a method of imaging of the magnetization reversal process using analysis of real-time images of magnetic domain structures in cylindrically shaped microwires. This method uses wide-field polarizing optical microscopy and is based on the magneto-optical Kerr effect (MOKE). The aperture diaphragm in MOKE microscope was used to control the incident angles of the light rays that reached the non-planar surface of the microwire and also determined the MOKE geometries. The movement of the non-central position of the hole in this diaphragm leads to a change in the orientation of the plane of incidence of the light along the perpendicular or the parallel direction to the axial direction of the wire. The visualization of the surface magnetic domain structures is obtained using polar and longitudinal MOKE geometries. The hysteresis loops were obtained by plotting the averaged image contrast as a function of the external magnetic field. The separation of the all-magnetization components is performed using different MOKE geometries in a microscope. We demonstrate the use of vector magnetometry to analyze the orientation of the magnetization in a cylindrically shaped microwire under the influence of an external magnetic field.

Atomic-level control of the domain wall velocity in ultrathin magnets by tuning of exchange interactions.

We demonstrate that the propagation velocity of field driven magnetic domain walls in ultrathin Au/Co/Au films with perpendicular anisotropy on vicinal substrates is anisotropic and strongly depends on the step density of the substrate. The velocity of walls oriented perpendicular to the steps drastically increases with increasing local step density while being unchanged or only weakly decreased for the walls oriented parallel to the steps. We develop an analytical model revealing the step-modified exchange interactions as the main driving force for this anisotropic behavior. The enhancement of the domain wall velocity at low magnetic fields far below the Walker instability threshold makes this phenomenon interesting for magnetic nanodevices.

Tailoring of the perpendicular magnetization component in ferromagnetic films on a vicinal substrate.

We have engineered the magnetic properties of 1-8 nm Co films epitaxially grown on an Au-buffered bifacial W(110)/W(540) single crystal. The surface of Au/W(110) was atomically flat, whereas the Au/W(540) followed the morphology of the vicinal W surface, showing a regular array of monoatomic steps. For Co grown on Au/W(540), the existence of the out-of-plane magnetization component extended strongly to a thickness d of about 8 nm, which was accompanied by an anomalous increase of the out-of-plane switching field with increasing d. In addition, the process of up-down magnetization switching could be realized with both a perpendicular and in-plane external magnetic field.