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Temporal modulation recently draws great attentions in wave manipulations, with which one can introduce the concept of temporal multilayer structure, a temporal counterpart of spatially multilayer configurations. This kind of multilayer structure holds temporal interfaces in the time domain, which provides additional flexibility in temporal operations. Here we take this opportunity and propose to simulate a non-Abelian gauge field with a temporal multilayer structure in the discrete physical system. Two basic temporal operations, i.e., the folding/unfolding operation and the phase shift operation are used to design such a temporal multilayer structure, which hence can support noncommutative operations to realize the non-Abelian Aharonov-Bohm interference in the time domain. A two-/three-dimensional non-Abelian gauge field can be built, which may be further extended to higher dimensions. Our work therefore provides a unique platform enabling generalization of non-Abelian physics to arbitrary dimensions and offers a method for wave manipulations with temporal band engineering.
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Combining microbial electrolytic cells with anaerobic digestion (MEC-AD) was considered as an important method for enhancing complex organic matter degradation. However, the magnetic biochar (MBC) addition would be an effective approach for enhancing biodegradation in MEC-AD. By designing orthogonal experiments, the optimal parameters of MBC-enhanced MEC-AD system for landfill leachate treatment were determined. The results indicated that the optimal conditions were identified as HRT of 72 h, electrode spacing of 2.5 cm, and applied voltage of 0.8 V. Under these conditions, the COD removal efficiency reached a maximum of 54.7 %. Additionally, the UV-vis, 3D-EEM, and GC-MS indicated the macromolecules 13-Docosenamide (Z), Bis(2-ethylhexyl) benzene-1,4-dicarboxylate and bis(2-ethylhexyl) phthalate were degraded. 13-Docosenamide (Z) was almost completely removed under the conditions of 0.8 V applied voltage, 2.5 cm electrode spacing and 24 h HRT, with a removal efficiency of 99.91 %. Significant differences were observed in the microbial core genera among the MEC-AD systems. The core genera in the anodic and cathodic biofilms were primarily fermentative and electroactive bacteria, including Soehngenia (2.2 % - 32.1 %, 3.2 % - 26.4 %) and Desulfomicrobium (1.1 % - 10.2 %, 2.0 % - 29.3 %). Fermentative bacteria, norank_f__Bacteroidetes_vadinHA17, established cooperative relationships with electroactive bacteria Acinetobacter. The enrichment of electrochemically active bacteria optimized microbial interactions, thereby synergistically enhancing the biotransformation of complex organic matter in landfill leachate.
Asunto(s)
Biodegradación Ambiental , Carbón Orgánico , Contaminantes Químicos del Agua , Carbón Orgánico/química , Contaminantes Químicos del Agua/metabolismo , Anaerobiosis , Electrólisis , Eliminación de Residuos Líquidos/métodos , Reactores Biológicos/microbiologíaRESUMEN
Photonic structures with Weyl points (WPs), including type I and type II, promise nontrivial surface modes and intriguing light manipulations for their three-dimensional topological bands. While previous studies mainly focus on exploring WPs in a uniform Weyl structure, here we establish Weyl heterostructures (i.e., a nonuniform Weyl lattice) with different rotational orientations in the synthetic dimension by nanostructured photonic waveguides. In this work, we unveil a transition between bound and extended modes on the interface of type-II Weyl heterostructures by tuning their rotational phases, despite the reversed topological order across the interface. This mode transition is also manifested from the total transmission to total reflection at the interface. All of these unconventional effects are attributed to the tilted dispersion of type-II Weyl band structure that can lead to mismatched bands and gaps across the interface. As a comparison, the type-I Weyl heterostructures lack the phase transition due to the untilted band structure. This work establishes a flexible scheme of artificial Weyl heterostructures that opens a new avenue toward high-dimensional topological effects and significantly enhances our capabilities in on-chip light manipulations.
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Optical vortex beams, with phase singularity characterized by a topological charge (TC), introduces a new dimension for optical communication, quantum information, and optical light manipulation. However, the evaluation of TCs after beam propagation remains a substantial challenge, impeding practical applications. Here, we introduce vortices in lateral arrays (VOILA), a novel spatial multiplexing approach that enables simultaneous transmission of a lateral array of multiple vortices. Leveraging advanced learning techniques, VOILA effectively decodes TCs, even in the presence of strong optical nonlinearities simulated experimentally. Notably, our approach achieves substantial improvements in single-shot bandwidth, surpassing single-vortex scheme by several orders of magnitude. Furthermore, our system exhibits precise fractional TC recognition in both linear and nonlinear regimes, providing possibilities for high-bandwidth communication. The capabilities of VOILA promise transformative contributions to optical information processing and structured light research, with significant potential for advancements in diverse fields.
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The moiré lattice has recently attracted broad interest in both solid-state physics and photonics where exotic phenomena in manipulating the quantum states are explored. In this work, we study the one-dimensional (1D) analogs of "moiré" lattices in a synthetic frequency dimension constructed by coupling two resonantly modulated ring resonators with different lengths. Unique features associated with the flatband manipulation as well as the flexible control of localization position inside each unit cell in the frequency dimension have been found, which can be controlled via the choice of flatband. Our work therefore provides insight into simulating moiré physics in 1D synthetic frequency space, which holds important promise for potential applications toward optical information processing.
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Measuring topological invariants is an essential task in characterizing topological phases of matter. They are usually obtained from the number of edge states due to the bulk-edge correspondence or from interference since they are integrals of the geometric phases in the energy band. It is commonly believed that the bulk band structures could not be directly used to obtain the topological invariants. Here, we implement the experimental extraction of Zak phase from the bulk band structures of a Su-Schrieffer-Heeger (SSH) model in the synthetic frequency dimension. Such synthetic SSH lattices are constructed in the frequency axis of light, by controlling the coupling strengths between the symmetric and antisymmetric supermodes of two bichromatically driven rings. We measure the transmission spectra and obtain the projection of the time-resolved band structure on lattice sites, where a strong contrast between the non-trivial and trivial topological phases is observed. The topological Zak phase is naturally encoded in the bulk band structures of the synthetic SSH lattices, which can hence be experimentally extracted from the transmission spectra in a fiber-based modulated ring platform using a laser with telecom wavelength. Our method of extracting topological phases from the bulk band structure can be further extended to characterize topological invariants in higher dimensions, while the exhibited trivial and non-trivial transmission spectra from the topological transition may find future applications in optical communications.
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Weyl medium has triggered remarkable interest owing to its nontrivial topological edge states in 3D photonic band structures that were mainly revealed as surface modes yet. It is undoubted that the connection of two different Weyl media will give rise to more fruitful physics at their interface, while they face extreme difficulty in high-dimensional lattice matching. Here, we successfully demonstrate the non-Hermitian Weyl interface physics in complex synthetic parameter space, which is implemented in a loss-controlled silicon waveguide array. By establishing non-Hermitian Hamiltonian in the parameter space, new Weyl interfaces with distinct topological origins are predicted and experimentally observed in silicon waveguides. Significantly, our Letter exploits the non-Hermitian parameter to create the synthetic dimension by manipulating the non-Hermitian order, which successfully circumvents the difficulty in lattice matching for high-dimensional interfaces. The revealed rich topological Weyl interface states and their phase transitions in silicon waveguide platform further imply potentials in chip-scale photonics integrations.
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Topologically protected edge states based on valley photonic crystals (VPCs) have been widely studied, from theoretical verification to technical applications. However, research on integrated tuneable topological devices is still lacking. Here, we study the phase-shifting theory of topological edge modes based on a VPC structure. Benefiting from the phase vortex formed by the VPC structure, the optical path of the topological edge mode in the propagation direction is approximately two-fold that of the conventional optical mode in a strip waveguide. In experiments, we show a 1.57-fold improvement in π-phase tuning efficiency. By leveraging the high-efficiency phase-shifting properties and the sharp-turn features of the topological waveguide, we demonstrate an ultracompact 1 × 2 thermo-optic topological switch (TOTS) operating at telecommunication wavelengths. A switching power of 18.2 mW is needed with an ultracompact device footprint of 25.66 × 28.3 µm in the wavelength range of 1530-1582 nm. To the best of our knowledge, this topological photonic switch is the smallest switch of any dielectric or semiconductor 1 × 2/2 × 2 broadband optical switches, including thermo-optic and electro-optic switches. In addition, a high-speed transmission experiment employing the proposed TOTS is carried out to demonstrate the robust transmission of high-speed data. Our work reveals the phase-shifting mechanism of valley edge modes, which may enable diverse topological functional devices in many fields, such as optical communications, nanophotonics, and quantum information processing.
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The dimensionality of a physical system is one of the major parameters defining its physical properties. The recently introduced concept of synthetic dimension has made it possible to arbitrarily manipulate the system of interest and harness light propagation in different ways. It also facilitates the transformative architecture of system-on-a-chip devices enabling far reaching applications such as optical isolation. In this report, a novel architecture based on dynamically-modulated waveguide arrays with the Su-Schrieffer-Heeger configuration in the spatial dimension is proposed and investigated with an eye on a practical implementation. The propagation of light through the one-dimensional waveguide arrays mimics time evolution of the field in a synthetic two-dimensional lattice. The addition of the effective gauge potential leads to an exotic topologically protected one-way transmission along adjacent boundary. A cosine-shape isolated band, which supports the topological Bloch oscillation in the frequency dimension under the effective constant force, appears and is localized at the spatial boundary being robust against small perturbations. This work paves the way to improved light transmission capabilities under topological protections in both spatial and spectral regimes and provides a novel platform based on a technologically feasible lithium niobate platform for optical computing and communication.
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Supercontinuum (SC) light sources hold versatile applications in many fields ranging from imaging microscopic structural dynamics to achieving frequency comb metrology. Although such broadband light sources are readily accessible in the visible and near infrared regime, the ultraviolet (UV) extension of SC spectrum is still challenging. Here, we demonstrate that the joint contribution of strong field ionization and quantum resonance leads to the unexpected UV continuum radiation spanning the 100 nm bandwidth in molecular nitrogen ions. Quantum coherences in a bunch of ionic levels are found to be created by dynamic Stark-assisted multiphoton resonances following tunneling ionization. We show that the dynamical evolution of the coherence-enhanced polarization wave gives rise to laser-assisted continuum emission inside the laser field and free-induction decay after the laser field, which jointly contribute to the SC generation together with fifth harmonics. As proof of principle, we also show the application of the SC radiation in the absorption spectroscopy. This work offers an alternative scheme for constructing exotic SC sources, and opens up the territory of ionic quantum optics in the strong-field regime.
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Temporal modulations in photonics bring many exotic optical phenomena in the time dimension while metamaterials provide powerful ways in manipulating light in the spatial domain. The authors envision the connection, Floquet Metamaterials, may deliver novel opportunities in nanophotonics.
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Synthetic dimensions have garnered widespread interest for implementing high dimensional classical and quantum dynamics on low-dimensional geometries. Synthetic frequency dimensions, in particular, have been used to experimentally realize a plethora of bulk physics effects. However, in synthetic frequency dimension there has not been a demonstration of a boundary which is of paramount importance in topological physics due to the bulk-edge correspondence. Here we construct boundaries in the frequency dimension of dynamically modulated ring resonators by strongly coupling an auxiliary ring. We explore various effects associated with such boundaries, including confinement of the spectrum of light, discretization of the band structure, and the interaction of boundaries with one-way chiral modes in a quantum Hall ladder, which exhibits topologically robust spectral transport. Our demonstration of sharp boundaries fundamentally expands the capability of exploring topological physics, and has applications in classical and quantum information processing in synthetic frequency dimensions.
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We develop a background-free single-beam coherent Raman scattering technique enabling the high-sensitivity detection of greenhouse gases. In this scheme, Raman coherence prepared by a femtosecond laser is interrogated by self-generated narrowband air lasing, thus allowing single-beam measurements without complex pulse shaping. The unique temporal and spectral characteristics of air lasing are beneficial for improving the signal-to-noise ratio and spectral resolution of Raman signals. With this method, SF6 gas present at a concentration of 0.38% was detected in an SF6-air mixture. This technique provides a simple and promising route for remote detection due to the low divergence of Raman signals and the availability of high-energy pump lasers, which may broaden the potential applications of air lasing.
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The notion of topological phases extended to dynamical systems stimulates extensive studies, of which the characterization of nonequilibrium topological invariants is a central issue and usually necessitates the information of quantum dynamics in both the time and momentum dimensions. Here, we propose the topological holographic quench dynamics in synthetic dimension, and also show it provides a highly efficient scheme to characterize photonic topological phases. A pseudospin model is constructed with ring resonators in a synthetic lattice formed by frequencies of light, and the quench dynamics is induced by initializing a trivial state, which evolves under a topological Hamiltonian. Our key prediction is that the complete topological information of the Hamiltonian is encoded in quench dynamics solely in the time dimension, and is further mapped to lower-dimensional space, manifesting the holographic features of the dynamics. In particular, two fundamental time scales emerge in the dynamical evolution, with one mimicking the topological band on the momentum dimension and the other characterizing the residue time evolution of the state after the quench. For this, a universal duality between the quench dynamics and the equilibrium topological phase of the spin model is obtained in the time dimension by extracting information from the field evolution dynamics in modulated ring systems in simulations. This work also shows that the photonic synthetic frequency dimension provides an efficient and powerful way to explore the topological nonequilibrium dynamics.
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Flat bands play an important role in diffraction-free photonics and attract fundamental interest in many-body physics. Here we report the engineering of flat-band localization of collective excited states of atoms in Creutz superradiance lattices with tunable synthetic gauge fields. Magnitudes and phases of the lattice hopping coefficients can be independently tuned to control the state components of the flat band and the Aharonov-Bohm phases. We can selectively excite the flat band and control the flat-band localization with the synthetic gauge field. Our study provides a room-temperature platform for flat bands of atoms and holds promising applications in exploring correlated topological materials.
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Band structure theory plays an essential role in exploring physics in both solid-state systems and photonics. Here, we demonstrate a direct experimental measurement of the dynamic band structure in a synthetic space including the frequency axis of light, realized in a ring resonator under near-resonant dynamic modulation. This synthetic lattice exhibits the physical picture of the evolution of the wave vector reciprocal to the frequency axis in the band structure, analogous to a one-dimensional lattice under an external force. We experimentally measure the trajectories of the dynamic band structure by selectively exciting the band with a continuous wave source with its frequency scanning across the entire energy regime of the band. Our results not only provide a new perspective for exploring the dynamics in fundamental physics of solid-state and photonic systems with the concept of the synthetic dimension but also enable great capability in band structure engineering in photonics.
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Quantum coherence in quantum optics is an essential part of optical information processing and light manipulation. Alkali metal vapors, despite the numerous shortcomings, are traditionally used in quantum optics as a working medium due to convenient near-infrared excitation, strong dipole transitions and long-lived coherence. Here, we proposed and experimentally demonstrated photon retention and subsequent re-emittance with the quantum coherence in a system of coherently excited molecular nitrogen ions (N2+) which are produced using a strong 800 nm femtosecond laser pulse. Such photon retention, facilitated by quantum coherence, keeps releasing directly-unmeasurable coherent photons for tens of picoseconds, but is able to be read out by a time-delayed femtosecond pulse centered at 1580 nm via two-photon resonant absorption, resulting in a strong radiation at 329.3 nm. We reveal a pivotal role of the excited-state population to transmit such extremely weak re-emitted photons in this system. This new finding unveils the nature of the coherent quantum control in N2+ for the potential platform for optical information storage in the remote atmosphere, and facilitates further exploration of fundamental interactions in the quantum optical platform with strong-field ionized molecules..
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We show that a momentum-space meron spin texture for electromagnetic fields in free space can be generated by controlling the interaction of light with a photonic crystal slab having a nonzero Berry curvature. These spin textures in momentum space have not been previously noted either in electronic or photonic systems. Breaking the inversion symmetry of a honeycomb photonic crystal gaps out the Dirac cones at the corners of Brillouin zone. The pseudospin textures of photonic bands near the gaps exhibit a meron or antimeron. Unlike the electronic systems, the pseudospin texture of the photonic modes manifests directly in the spin (polarization) texture of the leakage radiation, as the Dirac points can be above the light line. Such a spin texture provides a direct approach to visualize the local Berry curvature. Our work highlights the significant opportunities of using photonic structures for the exploration of topological spin textures, with potential applications towards topologically robust ways to manipulate polarizations and other modal characteristics of light.
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We report an experiment showing the submillimeter Imbert-Fedorov shift from the ultrastrong spin-orbital angular momentum coupling, which is a photonic version of the spin Hall effect, by measuring the reflection of light from the surface of a birefringent symmetrical metal cladding planar waveguide. The light incidents at a near-normal incident angle and excites resonant ultrahigh-order modes inside the waveguide. A 0.16-mm displacement of separated reflected light spots corresponding to two polarization states is distinguishable by human eyes. In our experiment, we demonstrate the control of polarizations of light and the direct observation of the spin Hall effect of light, which opens an important avenue towards potential applications for optical sensing and quantum information processing, where the spin nature of photons exhibits key features.
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The concept of synthetic dimensions has generated interest in many branches of science, ranging from ultracold atomic physics to photonics, as it provides a versatile platform for realizing effective gauge potentials and topological physics. Previous experiments have augmented the real-space dimensionality by one additional physical synthetic dimension. In this study, we endow a single ring resonator with two independent physical synthetic dimensions. Our system consists of a temporally modulated ring resonator with spatial coupling between the clockwise and counterclockwise modes, creating a synthetic Hall ladder along the frequency and pseudospin degrees of freedom for photons propagating in the ring. We observe a wide variety of physics, including effective spin-orbit coupling, magnetic fields, spin-momentum locking, a Meissner-to-vortex phase transition, and signatures of topological chiral one-way edge currents, completely in synthetic dimensions. Our experiments demonstrate that higher-dimensional physics can be studied in simple systems by leveraging the concept of multiple simultaneous synthetic dimensions.