Jet-Printable, Low-Melting-Temperature Ga-xSn Eutectic Composites: Application in All-Solid-State Batteries.
Materials (Basel)
; 17(5)2024 Feb 21.
Article
en En
| MEDLINE
| ID: mdl-38473469
ABSTRACT
Low-melting-point Ga-xSn eutectic composites and natural silicate mineral powders were used as the electrode and solid-state electrolyte, respectively, in all-solid-state batteries for green energy storage systems. The influences of the Sn content in the Ga-xSn composite electrode on the electrochemical performance of the batteries were evaluated, and liquid composites with a Sn concentration of up to 30 wt.% demonstrated suitability for electrode fabrication through dip coating. Sodium-enriched silicate was synthesized to serve as the solid-state electrolyte membrane because of the abundance of water molecules in its interlayer structure, enabling ion exchange. The battery capacity increased with the Sn content of the Ga-xSn anode. The formation of intermetallic compounds and oxides (CuGa2, Ga2O3, Cu6Sn5, and SnO2) resulted in a high charge-discharge capacity and stability. The Ga-Sn composite electrode for all-solid-state batteries exhibits a satisfiable capacity and stability and shows potential for jet-printed electrode applications.
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MEDLINE
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Materials (Basel)
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2024
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Article