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1.
Chemosphere ; 57(4): 273-82, 2004 Oct.
Artículo en Inglés | MEDLINE | ID: mdl-15312725

RESUMEN

A rapid and simple method for separating and determining various environmentally harmful perfluorocarboxylic acids and perfluorosulfonates was successfully developed using high- performance liquid chromatography with conductimetric detection, for product and waste management of these compounds at manufacturing and processing sites. Compounds having C(3)-C(8) perfluoroalkyl groups were separated using a Tosoh TSKgel Super-ODS column and a mobile phase consisting of a mixture of methanol and aqueous NaH(2)PO(4) at several mixing ratios. The best detection limits for the compounds ranged from 0.12 to 0.66 mg l(-1) (ppm), and linear calibration graphs were obtained up to 87-109 mg l(-1). The combination of this method with concentration of the sample by solid-phase extraction with cartridges based on styrene-divinylbenzene-copolymer enabled the determination of approximately 50 microg l(-1) (ppb) for compounds with C(4)-C(8) perfluoroalkyl groups. This method was successfully used to monitor the artificial decomposition of the perfluorocarboxylic acid n-C(4)F(9)COOH induced by a photocatalyst.


Asunto(s)
Ácidos Carboxílicos/análisis , Cromatografía Líquida de Alta Presión/métodos , Contaminantes Ambientales/análisis , Polímeros de Fluorocarbono/análisis , Fluorocarburos/análisis , Poliestirenos/química , Estándares de Referencia , Reproducibilidad de los Resultados , Sensibilidad y Especificidad
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