Extending the Propagation Distance of a Silver Nanowire Plasmonic Waveguide with a Dielectric Multilayer Substrate.

Chemical-synthesized silver nanowires have been proven as an efficient architecture for plasmonic waveguides, but the high propagation loss prevents their widely applications. Here, we demonstrate that the propagation distance of the plasmons along a silver nanowire can be extended if this nanowire was placed on a dielectric multilayer substrate containing a photonic band gap but not placed on a commonly used glass substrate. The propagation distance at 630 nm wavelength can reach 16 µm, even when the silver nanowire is as thin as 90 nm in diameter. Experimental and simulation results further show that the polarization of this propagating plasmon mode was nearly parallel to the surface of the dielectric multilayer, so it can be excited by a transverse-electric polarized Bloch surface wave propagating along a polymer nanowire with diameter at only about 170 nm on the same dielectric multilayer. Numerical simulations were also carried out and are consistent with the experiment results. Our work provides a platform with which to extend the propagation distance of the plasmonic waveguide and also for the integration between photonic and plasmonic waveguides on the nanometer scale.

Dark-field imaging by active polymer slab waveguide.

A dark-field imaging technique taking advantage of the active polymer slab waveguide (APSW) is experimentally investigated. The dye molecules (Rhodamine 6G, Rh6G) are doped in the polymer film for the launching of surface waves on the APSW, such as the surface plasmon polaritons on the Ag-polymer-air interface, evanescent fields at the polymer-air interface by the total internal reflection, or the guided modes. The localized surface waves will not radiate into the far-field space directly. When the specimens are placed on the surface of the APSW, these surface waves will be scattered to the far-field region, which forms the dark-field image of the specimen. Experimental results show that usage of APSW leads to high-contrast dark-field images with the conventional optical microscope system. The polymer film involved in the proposed dark-field microscopy brings about the merits of reduced roughness, good stability, bio-compatibility, and shorter wavelength of the illumination light source.

Phase modulation of surface plasmon polaritons by surface relief dielectric structures.

Phase modulation of surface plasmon polaritons (SPPs) is studied as a function of geometric length and thickness of surface relief dielectric structures on a metal film. The results indicate that the SPPs are analogous to conventional free-space light waves in terms of phase modulation by geometric sizes and refractive indices. An SPP Fresnel zoneplate is considered as an example to employ the phase modulation method for focusing enhancement at the focal point. It is found that the phase modulation optimized zoneplate has obtained 130% higher electric field intensity at the focal point than that of an amplitude-modulated zoneplate.

Selective and sensitive detection of MiRNA-21 based on gold-nanorod functionalized polydiacetylene microtube waveguide.

Development of rapid, highly selective and sensitive miRNA detection in a complex biological environment has attracted considerable attention. Herein, we describe a novel two step method to construct gold-nanorod functionalized polydiacetylene (PDA) microtube for miRNA detection. In PDA microtube, with a one-dimensional (1D) waveguide nature, the excitation position and emission out-coupling position are far apart, thus helpful in reducing contribution of auto-fluorescence from biological sample. The use of specially designed toehold-mediated strand displacement reaction enables the reliable and selective discrimination of miRNA sequences with high sequence homology. Based on the condensing enrichment effect, the detection limit of the proposed PDA microtube system is as low as 0.01nM, and it can be applied directly to detect disease-specific miRNA targets in human serum. This PDA microtube waveguide system can be further integrated into the chip for the potential applications in minimally invasive, portable clinical diagnostic equipment.

Enantioselective synthesis of helical polydiacetylenes in the visible light region.

Herein, we demonstrate for the first time that the enantio-selective polymerization of DA monomers could be realized upon irradiation with circularly polarized visible light (CPVL), which could effectively provide chiral order in the propagating step of a polymerization reaction.