Directly imaging spin polarons in a kinetically frustrated Hubbard system.

The emergence of quasiparticles in quantum many-body systems underlies the rich phenomenology in many strongly interacting materials. In the context of doped Mott insulators, magnetic polarons are quasiparticles that usually arise from an interplay between the kinetic energy of doped charge carriers and superexchange spin interactions1-8. However, in kinetically frustrated lattices, itinerant spin polarons-bound states of a dopant and a spin flip-have been theoretically predicted even in the absence of superexchange coupling9-14. Despite their important role in the theory of kinetic magnetism, a microscopic observation of these polarons is lacking. Here we directly image itinerant spin polarons in a triangular-lattice Hubbard system realized with ultracold atoms, revealing enhanced antiferromagnetic correlations in the local environment of a hole dopant. In contrast, around a charge dopant, we find ferromagnetic correlations, a manifestation of the elusive Nagaoka effect15,16. We study the evolution of these correlations with interactions and doping, and use higher-order correlation functions to further elucidate the relative contributions of superexchange and kinetic mechanisms. The robustness of itinerant spin polarons at high temperature paves the way for exploring potential mechanisms for hole pairing and superconductivity in frustrated systems10,11. Furthermore, our work provides microscopic insights into related phenomena in triangular-lattice moiré materials17-20.

Observation of Nagaoka polarons in a Fermi-Hubbard quantum simulator.

Quantum interference can deeply alter the nature of many-body phases of matter1. In the case of the Hubbard model, Nagaoka proved that introducing a single itinerant charge can transform a paramagnetic insulator into a ferromagnet through path interference2-4. However, a microscopic observation of this kinetic magnetism induced by individually imaged dopants has been so far elusive. Here we demonstrate the emergence of Nagaoka polarons in a Hubbard system realized with strongly interacting fermions in a triangular optical lattice5,6. Using quantum gas microscopy, we image these polarons as extended ferromagnetic bubbles around particle dopants arising from the local interplay of coherent dopant motion and spin exchange. By contrast, kinetic frustration due to the triangular geometry promotes antiferromagnetic polarons around hole dopants7. Our work augurs the exploration of exotic quantum phases driven by charge motion in strongly correlated systems and over sizes that are challenging for numerical simulation8-10.

Magnetically mediated hole pairing in fermionic ladders of ultracold atoms.

Conventional superconductivity emerges from pairing of charge carriers-electrons or holes-mediated by phonons1. In many unconventional superconductors, the pairing mechanism is conjectured to be mediated by magnetic correlations2, as captured by models of mobile charges in doped antiferromagnets3. However, a precise understanding of the underlying mechanism in real materials is still lacking and has been driving experimental and theoretical research for the past 40 years. Early theoretical studies predicted magnetic-mediated pairing of dopants in ladder systems4-8, in which idealized theoretical toy models explained how pairing can emerge despite repulsive interactions9. Here we experimentally observe this long-standing theoretical prediction, reporting hole pairing due to magnetic correlations in a quantum gas of ultracold atoms. By engineering doped antiferromagnetic ladders with mixed-dimensional couplings10, we suppress Pauli blocking of holes at short length scales. This results in a marked increase in binding energy and decrease in pair size, enabling us to observe pairs of holes predominantly occupying the same rung of the ladder. We find a hole-hole binding energy of the order of the superexchange energy and, upon increased doping, we observe spatial structures in the pair distribution, indicating repulsion between bound hole pairs. By engineering a configuration in which binding is strongly enhanced, we delineate a strategy to increase the critical temperature for superconductivity.

Signatures of Wigner crystal of electrons in a monolayer semiconductor.

When the Coulomb repulsion between electrons dominates over their kinetic energy, electrons in two-dimensional systems are predicted to spontaneously break continuous-translation symmetry and form a quantum crystal1. Efforts to observe2-12 this elusive state of matter, termed a Wigner crystal, in two-dimensional extended systems have primarily focused on conductivity measurements on electrons confined to a single Landau level at high magnetic fields. Here we use optical spectroscopy to demonstrate that electrons in a monolayer semiconductor with density lower than 3 × 1011 per centimetre squared form a Wigner crystal. The combination of a high electron effective mass and reduced dielectric screening enables us to observe electronic charge order even in the absence of a moiré potential or an external magnetic field. The interactions between a resonantly injected exciton and electrons arranged in a periodic lattice modify the exciton bandstructure so that an umklapp resonance arises in the optical reflection spectrum, heralding the presence of charge order13. Our findings demonstrate that charge-tunable transition metal dichalcogenide monolayers14 enable the investigation of previously uncharted territory for many-body physics where interaction energy dominates over kinetic energy.

Bilayer Wigner crystals in a transition metal dichalcogenide heterostructure.

One of the first theoretically predicted manifestations of strong interactions in many-electron systems was the Wigner crystal1-3, in which electrons crystallize into a regular lattice. The crystal can melt via either thermal or quantum fluctuations4. Quantum melting of the Wigner crystal is predicted to produce exotic intermediate phases5,6 and quantum magnetism7,8 because of the intricate interplay of Coulomb interactions and kinetic energy. However, studying two-dimensional Wigner crystals in the quantum regime has often required a strong magnetic field9-11 or a moiré superlattice potential12-15, thus limiting access to the full phase diagram of the interacting electron liquid. Here we report the observation of bilayer Wigner crystals without magnetic fields or moiré potentials in an atomically thin transition metal dichalcogenide heterostructure, which consists of two MoSe2 monolayers separated by hexagonal boron nitride. We observe optical signatures of robust correlated insulating states at symmetric (1:1) and asymmetric (3:1, 4:1 and 7:1) electron doping of the two MoSe2 layers at cryogenic temperatures. We attribute these features to bilayer Wigner crystals composed of two interlocked commensurate triangular electron lattices, stabilized by inter-layer interaction16. The Wigner crystal phases are remarkably stable, and undergo quantum and thermal melting transitions at electron densities of up to 6 × 1012 per square centimetre and at temperatures of up to about 40 kelvin. Our results demonstrate that an atomically thin heterostructure is a highly tunable platform for realizing many-body electronic states and probing their liquid-solid and magnetic quantum phase transitions4-8,17.

Spin transport in a tunable Heisenberg model realized with ultracold atoms.

Simple models of interacting spins have an important role in physics. They capture the properties of many magnetic materials, but also extend to other systems, such as bosons and fermions in a lattice, gauge theories, high-temperature superconductors, quantum spin liquids, and systems with exotic particles such as anyons and Majorana fermions1,2. To study and compare these models, a versatile platform is needed. Realizing such systems has been a long-standing goal in the field of ultracold atoms. So far, spin transport has only been studied in systems with isotropic spin-spin interactions3-12. Here we realize the Heisenberg model describing spins on a lattice, with fully adjustable anisotropy of the nearest-neighbour spin-spin couplings (called the XXZ model). In this model we study spin transport far from equilibrium after quantum quenches from imprinted spin-helix patterns. When spins are coupled only along two of three possible orientations (the XX model), we find ballistic behaviour of spin dynamics, whereas for isotropic interactions (the XXX model), we find diffusive behaviour. More generally, for positive anisotropies, the dynamics ranges from anomalous superdiffusion to subdiffusion, whereas for negative anisotropies, we observe a crossover in the time domain from ballistic to diffusive transport. This behaviour is in contrast with expectations from the linear-response regime and raises new questions in understanding quantum many-body dynamics far away from equilibrium.

The spontaneous symmetry breaking in Ta2NiSe5 is structural in nature.

The excitonic insulator is an electronically driven phase of matter that emerges upon the spontaneous formation and Bose condensation of excitons. Detecting this exotic order in candidate materials is a subject of paramount importance, as the size of the excitonic gap in the band structure establishes the potential of this collective state for superfluid energy transport. However, the identification of this phase in real solids is hindered by the coexistence of a structural order parameter with the same symmetry as the excitonic order. Only a few materials are currently believed to host a dominant excitonic phase, Ta2NiSe5 being the most promising. Here, we test this scenario by using an ultrashort laser pulse to quench the broken-symmetry phase of this transition metal chalcogenide. Tracking the dynamics of the material's electronic and crystal structure after light excitation reveals spectroscopic fingerprints that are compatible only with a primary order parameter of phononic nature. We rationalize our findings through state-of-the-art calculations, confirming that the structural order accounts for most of the gap opening. Our results suggest that the spontaneous symmetry breaking in Ta2NiSe5 is mostly of structural character, hampering the possibility to realize quasi-dissipationless energy transport.

Terahertz parametric amplification as a reporter of exciton condensate dynamics.

Condensates are a hallmark of emergence in quantum materials such as superconductors and charge density waves. Excitonic insulators are an intriguing addition to this library, exhibiting spontaneous condensation of electron-hole pairs. However, condensate observables can be obscured through parasitic coupling to the lattice. Here we employ nonlinear terahertz spectroscopy to disentangle such obscurants through measurement of the quantum dynamics. We target Ta2NiSe5, a putative room-temperature excitonic insulator in which electron-lattice coupling dominates the structural transition (Tc = 326 K), hindering identification of excitonic correlations. A pronounced increase in the terahertz reflectivity manifests following photoexcitation and exhibits a Bose-Einstein condensation-like temperature dependence well below the Tc, suggesting an approach to monitor the exciton condensate dynamics. Nonetheless, dynamic condensate-phonon coupling remains as evidenced by peaks in the enhanced reflectivity spectrum at select infrared-active phonon frequencies, indicating that parametric reflectivity enhancement arises from phonon squeezing. Our results highlight that coherent dynamics can drive parametric stimulated emission.

Imaging magnetic polarons in the doped Fermi-Hubbard model.

Polarons-electronic charge carriers 'dressed' by a local polarization of the background environment-are among the most fundamental quasiparticles in interacting many-body systems, and emerge even at the level of a single dopant1. In the context of the two-dimensional Fermi-Hubbard model, polarons are predicted to form around charged dopants in an antiferromagnetic background in the low-doping regime, close to the Mott insulating state2-7; this prediction is supported by macroscopic transport and spectroscopy measurements in materials related to high-temperature superconductivity8. Nonetheless, a direct experimental observation of the internal structure of magnetic polarons is lacking. Here we report the microscopic real-space characterization of magnetic polarons in a doped Fermi-Hubbard system, enabled by the single-site spin and density resolution of our ultracold-atom quantum simulator. We reveal the dressing of doublons by a local reduction-and even sign reversal-of magnetic correlations, which originates from the competition between kinetic and magnetic energy in the system. The experimentally observed polaron signatures are found to be consistent with an effective string model at finite temperature7. We demonstrate that delocalization of the doublon is a necessary condition for polaron formation, by comparing this setting with a scenario in which a doublon is pinned to a lattice site. Our work could facilitate the study of interactions between polarons, which may lead to collective behaviour, such as stripe formation, as well as the microscopic exploration of the fate of polarons in the pseudogap and 'bad metal' phases.

Local Noise Spectroscopy of Wigner Crystals in Two-Dimensional Materials.

We propose local electromagnetic noise spectroscopy as a versatile and noninvasive tool to study Wigner crystal phases of strongly interacting two-dimensional electronic systems. In-plane imaging of the local noise is predicted to enable single-site resolution of the electron crystal when the sample-probe distance is less than the interelectron separation. At larger sample-probe distances, noise spectroscopy encodes information about the low-energy Wigner crystal phonons, including the dispersion of the transverse shear mode, the pinning resonance due to disorder, and optical modes emerging, for instance, in bilayer crystals. We discuss the potential utility of local noise probes in analyzing the rich set of phenomena expected to occur in the vicinity of the melting transition.

A magnon scattering platform.

Scattering experiments have revolutionized our understanding of nature. Examples include the discovery of the nucleus [R. G. Newton, Scattering Theory of Waves and Particles (1982)], crystallography [U. Pietsch, V. Holý, T. Baumback, High-Resolution X-Ray Scattering (2004)], and the discovery of the double-helix structure of DNA [J. D. Watson, F. H. C. Crick, Nature 171, 737-738]. Scattering techniques differ by the type of particles used, the interaction these particles have with target materials, and the range of wavelengths used. Here, we demonstrate a two-dimensional table-top scattering platform for exploring magnetic properties of materials on mesoscopic length scales. Long-lived, coherent magnonic excitations are generated in a thin film of yttrium iron garnet and scattered off a magnetic target deposited on its surface. The scattered waves are then recorded using a scanning nitrogen vacancy center magnetometer that allows subwavelength imaging and operation under conditions ranging from cryogenic to ambient environment. While most scattering platforms measure only the intensity of the scattered waves, our imaging method allows for spatial determination of both amplitude and phase of the scattered waves, thereby allowing for a systematic reconstruction of the target scattering potential. Our experimental results are consistent with theoretical predictions for such a geometry and reveal several unusual features of the magnetic response of the target, including suppression near the target edges and a gradient in the direction perpendicular to the direction of surface wave propagation. Our results establish magnon scattering experiments as a platform for studying correlated many-body systems.

Cavity Quantum Electrodynamics with Hyperbolic van der Waals Materials.

The ground-state properties and excitation energies of a quantum emitter can be modified in the ultrastrong coupling regime of cavity quantum electrodynamics (QED) where the light-matter interaction strength becomes comparable to the cavity resonance frequency. Recent studies have started to explore the possibility of controlling an electronic material by embedding it in a cavity that confines electromagnetic fields in deep subwavelength scales. Currently, there is a strong interest in realizing ultrastrong-coupling cavity QED in the terahertz (THz) part of the spectrum, since most of the elementary excitations of quantum materials are in this frequency range. We propose and discuss a promising platform to achieve this goal based on a two-dimensional electronic material encapsulated by a planar cavity consisting of ultrathin polar van der Waals crystals. As a concrete setup, we show that nanometer-thick hexagonal boron nitride layers should allow one to reach the ultrastrong coupling regime for single-electron cyclotron resonance in a bilayer graphene. The proposed cavity platform can be realized by a wide variety of thin dielectric materials with hyperbolic dispersions. Consequently, van der Waals heterostructures hold the promise of becoming a versatile playground for exploring the ultrastrong-coupling physics of cavity QED materials.

Generating Coherent Phonon Waves in Narrow-Band Materials: A Twisted Bilayer Graphene Phaser.

Twisted bilayer graphene (TBG) exhibits extremely low Fermi velocities for electrons, with the speed of sound surpassing the Fermi velocity. This regime enables the use of TBG for amplifying vibrational waves of the lattice through stimulated emission, following the same principles of operation of free-electron lasers. Our Letter proposes a lasing mechanism relying on the slow-electron bands to produce a coherent beam of acoustic phonons. We propose a device based on undulated electrons in TBG, which we dub the phaser. The device generates phonon beams in a terahertz (THz) frequency range, which can then be used to produce THz electromagnetic radiation. The ability to generate coherent phonons in solids breaks new ground in controlling quantum memories, probing quantum states, realizing nonequilibrium phases of matter, and designing new types of THz optical devices.

Quantum Noise Spectroscopy of Dynamical Critical Phenomena.

The transition between distinct phases of matter is characterized by the nature of fluctuations near the critical point. We demonstrate that noise spectroscopy can not only diagnose the presence of a phase transition, but can also determine fundamental properties of its criticality. In particular, by analyzing a scaling collapse of the decoherence profile, one can directly extract the critical exponents of the transition and identify its universality class. Our approach naturally captures the presence of conservation laws and distinguishes between classical and quantum phase transitions. In the context of quantum magnetism, our proposal complements existing techniques and provides a novel toolset optimized for interrogating two-dimensional magnetic materials.

Stabilizing Fluctuating Spin-Triplet Superconductivity in Graphene via Induced Spin-Orbit Coupling.

A recent experiment showed that a proximity-induced Ising spin-orbit coupling enhances the spin-triplet superconductivity in Bernal bilayer graphene. Here, we show that, due to the nearly perfect spin rotation symmetry of graphene, the fluctuations of the spin orientation of the triplet order parameter suppress the superconducting transition to nearly zero temperature. Our analysis shows that both an Ising spin-orbit coupling and an in-plane magnetic field can eliminate these low-lying fluctuations and can greatly enhance the transition temperature, consistent with the recent experiment. Our model also suggests the possible existence of a phase at small anisotropy and magnetic field which exhibits quasilong-range ordered spin-singlet charge 4e superconductivity, even while the triplet 2e superconducting order only exhibits short-ranged correlations. Finally, we discuss relevant experimental signatures.

A cold-atom Fermi-Hubbard antiferromagnet.

Exotic phenomena in systems with strongly correlated electrons emerge from the interplay between spin and motional degrees of freedom. For example, doping an antiferromagnet is expected to give rise to pseudogap states and high-temperature superconductors. Quantum simulation using ultracold fermions in optical lattices could help to answer open questions about the doped Hubbard Hamiltonian, and has recently been advanced by quantum gas microscopy. Here we report the realization of an antiferromagnet in a repulsively interacting Fermi gas on a two-dimensional square lattice of about 80 sites at a temperature of 0.25 times the tunnelling energy. The antiferromagnetic long-range order manifests through the divergence of the correlation length, which reaches the size of the system, the development of a peak in the spin structure factor and a staggered magnetization that is close to the ground-state value. We hole-dope the system away from half-filling, towards a regime in which complex many-body states are expected, and find that strong magnetic correlations persist at the antiferromagnetic ordering vector up to dopings of about 15 per cent. In this regime, numerical simulations are challenging and so experiments provide a valuable benchmark. Our results demonstrate that microscopy of cold atoms in optical lattices can help us to understand the low-temperature Fermi-Hubbard model.

Observation of discrete time-crystalline order in a disordered dipolar many-body system.

Understanding quantum dynamics away from equilibrium is an outstanding challenge in the modern physical sciences. Out-of-equilibrium systems can display a rich variety of phenomena, including self-organized synchronization and dynamical phase transitions. More recently, advances in the controlled manipulation of isolated many-body systems have enabled detailed studies of non-equilibrium phases in strongly interacting quantum matter; for example, the interplay between periodic driving, disorder and strong interactions has been predicted to result in exotic 'time-crystalline' phases, in which a system exhibits temporal correlations at integer multiples of the fundamental driving period, breaking the discrete time-translational symmetry of the underlying drive. Here we report the experimental observation of such discrete time-crystalline order in a driven, disordered ensemble of about one million dipolar spin impurities in diamond at room temperature. We observe long-lived temporal correlations, experimentally identify the phase boundary and find that the temporal order is protected by strong interactions. This order is remarkably stable to perturbations, even in the presence of slow thermalization. Our work opens the door to exploring dynamical phases of matter and controlling interacting, disordered many-body systems.

Variational Ansatz for the Ground State of the Quantum Sherrington-Kirkpatrick Model.

We present an Ansatz for the ground states of the quantum Sherrington-Kirkpatrick model, a paradigmatic model for quantum spin glasses. Our Ansatz, based on the concept of generalized coherent states, very well captures the fundamental aspects of the model, including the ground state energy and the position of the spin glass phase transition. It further enables us to study some previously unexplored features, such as the nonvanishing longitudinal field regime and the entanglement structure of the ground states. We find that the ground state entanglement can be captured by a simple ensemble of weighted graph states with normally distributed phase gates, leading to a volume law entanglement, contrasting with predictions based on entanglement monogamy.

Surface Cooper-Pair Spin Waves in Triplet Superconductors.

We study the electrodynamics of spin triplet superconductors including dipolar interactions, which give rise to an interplay between the collective spin dynamics of the condensate and orbital Meissner screening currents. Within this theory, we identify a class of spin waves that originate from the coupled dynamics of the spin-symmetry breaking triplet order parameter and the electromagnetic field. In particular, we study magnetostatic spin wave modes that are localized to the sample surface. We show that these surface modes can be excited and detected using experimental techniques such as microwave spin wave resonance spectroscopy or nitrogen-vacancy magnetometry, and propose that the detection of these modes offers a means for the identification of spin triplet superconductivity.

Resonantly enhanced polariton wave mixing and parametric instability in a Floquet medium.

We introduce a new theoretical approach for analyzing pump and probe experiments in non-linear systems of optical phonons. In our approach, the effect of coherently pumped polaritons is modeled as providing time-periodic modulation of the system parameters. Within this framework, propagation of the probe pulse is described by the Floquet version of Maxwell's equations and leads to phenomena such as frequency mixing and resonant parametric production of polariton pairs. We analyze light reflection from a slab of insulating material with a strongly excited phonon-polariton mode and obtain analytic expressions for the frequency-dependent reflection coefficient for the probe pulse. Our results are in agreement with recent experiments by Cartella et al. [Proc. Natl. Acad. Sci. U. S. A. 115, 12148 (2018)], which demonstrated light amplification in a resonantly excited SiC insulator. We show that, beyond a critical pumping strength, such systems should exhibit Floquet parametric instability, which corresponds to resonant scattering of pump polaritons into pairs of finite momentum polaritons. We find that the parametric instability should be achievable in SiC using current experimental techniques and discuss its signatures, including the non-analytic frequency dependence of the reflection coefficient and the probe pulse afterglow. We discuss possible applications of the parametric instability phenomenon and suggest that similar types of instabilities can be present in other photoexcited non-linear systems.