Scalable spin squeezing in a dipolar Rydberg atom array.

The standard quantum limit bounds the precision of measurements that can be achieved by ensembles of uncorrelated particles. Fundamentally, this limit arises from the non-commuting nature of quantum mechanics, leading to the presence of fluctuations often referred to as quantum projection noise. Quantum metrology relies on the use of non-classical states of many-body systems to enhance the precision of measurements beyond the standard quantum limit1,2. To do so, one can reshape the quantum projection noise-a strategy known as squeezing3,4. In the context of many-body spin systems, one typically uses all-to-all interactions (for example, the one-axis twisting model4) between the constituents to generate the structured entanglement characteristic of spin squeezing5. Here we explore the prediction, motivated by recent theoretical work6-10, that short-range interactions-and in particular, the two-dimensional dipolar XY model-can also enable the realization of scalable spin squeezing. Working with a dipolar Rydberg quantum simulator of up to N = 100 atoms, we demonstrate that quench dynamics from a polarized initial state lead to spin squeezing that improves with increasing system size up to a maximum of -3.5 ± 0.3 dB (before correcting for detection errors, or roughly -5 ± 0.3 dB after correction). Finally, we present two independent refinements: first, using a multistep spin-squeezing protocol allows us to further enhance the squeezing by roughly 1 dB, and second, leveraging Floquet engineering to realize Heisenberg interactions, we demonstrate the ability to extend the lifetime of the squeezed state by freezing its dynamics.

Entangling Dynamics from Effective Rotor-Spin-Wave Separation in U(1)-Symmetric Quantum Spin Models.

The nonequilibrium dynamics of quantum spin models is a most challenging topic, due to the exponentiality of Hilbert space, and it is central to the understanding of the many-body entangled states that can be generated by state-of-the-art quantum simulators. A particularly important class of evolutions is the one governed by U(1)-symmetric Hamiltonians, initialized in a state that breaks the U(1) symmetry-the paradigmatic example being the evolution of the so-called one-axis-twisting (OAT) model, featuring infinite-range interactions between spins. In this Letter, we show that the dynamics of the OAT model can be closely reproduced by systems with power-law-decaying interactions, thanks to an effective separation between the zero-momentum degrees of freedom, associated with the so-called Anderson tower of states, and reconstructing an OAT model, as well as finite-momentum ones, associated with spin-wave excitations. This mechanism explains quantitatively the recent numerical observation of spin squeezing and Schrödinger cat-state generation in the dynamics of dipolar Hamiltonians, and it paves the way for the extension of this observation to a much larger class of models of immediate relevance for quantum simulations.

Quasicrystalline Bose Glass in the Absence of Disorder and Quasidisorder.

We study the low-temperature phases of interacting bosons on a two-dimensional quasicrystalline lattice. By means of numerically exact path integral Monte Carlo simulations, we show that for sufficiently weak interactions the system is a homogeneous Bose-Einstein condensate that develops density modulations for increasing filling factor. The simultaneous occurrence of sizeable condensate fraction and density modulation can be interpreted as the analogous, in a quasicrystalline lattice, of supersolid phases occurring in conventional periodic lattices. For sufficiently large interaction strength and particle density, global condensation is lost and quantum exchanges are restricted to specific spatial regions. The emerging quantum phase is therefore a Bose glass, which here is stabilized in the absence of any source of disorder or quasidisorder, purely as a result of the interplay between quantum effects, particle interactions and quasicrystalline substrate. This finding clearly indicates that (quasi)disorder is not essential to observe Bose glass physics. Our results are of interest for ongoing experiments on (quasi)disorder-free quasicrystalline lattices.

Multipartite Entangled States in Dipolar Quantum Simulators.

The scalable production of multipartite entangled states in ensembles of qubits is a crucial function of quantum devices, as such states are an essential resource both for fundamental studies on entanglement, as well as for applied tasks. Here we focus on the U(1) symmetric Hamiltonians for qubits with dipolar interactions-a model realized in several state-of-the-art quantum simulation platforms for lattice spin models, including Rydberg-atom arrays with resonant interactions. Making use of exact and variational simulations, we theoretically show that the nonequilibrium dynamics generated by this Hamiltonian shares fundamental features with that of the one-axis-twisting model, namely, the simplest interacting collective-spin model with U(1) symmetry. The evolution governed by the dipolar Hamiltonian generates a cascade of multipartite entangled states-spin-squeezed states, Schrödinger's cat states, and multicomponent superpositions of coherent spin states. Investigating systems with up to N=144 qubits, we observe full scalability of the entanglement features of these states directly related to metrology, namely, scalable spin squeezing at an evolution time O(N^{1/3}) and Heisenberg scaling of sensitivity of the spin parity to global rotations for cat states reached at times O(N). Our results suggest that the native Hamiltonian dynamics of state-of-the-art quantum simulation platforms, such as Rydberg-atom arrays, can act as a robust source of multipartite entanglement.

Scalable Spin Squeezing from Spontaneous Breaking of a Continuous Symmetry.

Spontaneous symmetry breaking is a property of Hamiltonian equilibrium states which, in the thermodynamic limit, retain a finite average value of an order parameter even after a field coupled to it is adiabatically turned off. In the case of quantum spin models with continuous symmetry, we show that this adiabatic process is also accompanied by the suppression of the fluctuations of the symmetry generator-namely, the collective spin component along an axis of symmetry. In systems of S=1/2 spins or qubits, the combination of the suppression of fluctuations along one direction and of the persistence of transverse magnetization leads to spin squeezing-a much sought-after property of quantum states, both for the purpose of entanglement detection as well as for metrological uses. Focusing on the case of XXZ models spontaneously breaking a U(1) [or even SU(2)] symmetry, we show that the adiabatically prepared states have nearly minimal spin uncertainty; that the minimum phase uncertainty that one can achieve with these states scales as N^{-3/4} with the number of spins N; and that this scaling is attained after an adiabatic preparation time scaling linearly with N. Our findings open the door to the adiabatic preparation of strongly spin-squeezed states in a large variety of quantum many-body devices including, e.g., optical-lattice clocks.

Supersolid Stripe Crystal from Finite-Range Interactions on a Lattice.

Strong, long-range interactions present a unique challenge for the theoretical investigation of quantum many-body lattice models, due to the generation of large numbers of competing states at low energy. Here, we investigate a class of extended bosonic Hubbard models with off-site terms interpolating between short and infinite range, thus allowing for an exact numerical solution for all interaction strengths. We predict a novel type of stripe crystal at strong coupling. Most interestingly, for intermediate interaction strengths we demonstrate that the stripes can turn superfluid, thus leading to a self-assembled array of quasi-one-dimensional superfluids. These bosonic superstripes turn into an isotropic supersolid with decreasing the interaction strength. The mechanism for stripe formation is based on cluster self-assembling in the corresponding classical ground state, reminiscent of classical soft-matter models of polymers, different from recently proposed mechanisms for cold gases of alkali or dipolar magnetic atoms.

Phase-change switching in 2D via soft interactions.

We present a new type of phase-change behavior relevant for information storage applications, that can be observed in 2D systems with cluster-forming ability. The temperature-based control of the ordering in 2D particle systems depends on the existence of a crystal-to-glass transition. We perform molecular dynamics simulations of models with soft interactions, demonstrating that the crystalline and amorphous structures can be easily tuned by heat pulses. The physical mechanism responsible for this behavior is a self-assembled polydispersity, that depends on the cluster-forming ability of the interactions. Therefore, the range of real materials that can perform such a transition is very wide in nature, ranging from colloidal suspensions to vortex matter. The state of the art in soft matter experimental setups, controlling interactions, polydispersity and dimensionality, makes it a very fertile ground for practical applications.

Glass Transitions in Monodisperse Cluster-Forming Ensembles: Vortex Matter in Type-1.5 Superconductors.

At low enough temperatures and high densities, the equilibrium configuration of an ensemble of ultrasoft particles is a self-assembled, ordered, cluster crystal. In the present Letter, we explore the out-of-equilibrium dynamics for a two-dimensional realization, which is relevant to superconducting materials with multiscale intervortex forces. We find that, for small temperatures following a quench, the suppression of the thermally activated particle hopping hinders the ordering. This results in a glass transition for a monodispersed ensemble, for which we derive a microscopic explanation in terms of an "effective polydispersity" induced by multiscale interactions. This demonstrates that a vortex glass can form in clean systems of thin films of "type-1.5" superconductors. An additional setup to study this physics can be layered superconducting systems, where the shape of the effective vortex-vortex interactions can be engineered.

Superglass Phase of Interaction-Blockaded Gases on a Triangular Lattice.

We investigate the quantum phases of monodispersed bosonic gases confined to a triangular lattice and interacting via a class of soft-shoulder potentials. The latter correspond to soft-core potentials with an additional hard-core onsite interaction. Using exact quantum Monte Carlo simulations, we show that the low temperature phases for weak and strong interactions following a temperature quench are a homogeneous superfluid and a glass, respectively. The latter is an insulating phase characterized by inhomogeneity in the density distribution and structural disorder. Remarkably, we find that for intermediate interaction strengths a superglass occurs in an extended region of the phase diagram, where glassy behavior coexists with a sizable finite superfluid fraction. This glass phase is obtained in the absence of geometrical frustration or external disorder and is a result of the competition of quantum fluctuations and cluster formation in the corresponding classical ground state. For high enough temperature, the glass and superglass turn into a floating stripe solid and a supersolid, respectively. Given the simplicity and generality of the model, these phases should be directly relevant for state-of-the-art experiments with Rydberg-dressed atoms in optical lattices.

On the possible "supersolid" character of parahydrogen clusters.

We present results of a theoretical study of structural and superfluid properties of parahydrogen (p-H(2)) clusters comprising 25, 26, and 27 molecules at low temperature. The microscopic model utilized here is based on the Silvera-Goldman pair potential. Numerical results are obtained by means of quantum Monte Carlo simulations, making use of the continuous-space worm algorithm. The clusters are superfluid in the low temperature limit, but display markedly different physical behaviors. For N = 25 and 27, superfluidity at low temperature arises as clusters melt, that is, become progressively liquid-like as a result of quantum effects. On the other hand, for N = 26, the cluster remains rigid and solid-like. We argue that the cluster (p-H(2))(26) can be regarded as a mesoscopic "supersolid". This physical picture is supported by results of simulations in which a single p-H(2) molecule in the cluster is isotopically substituted.

Classical and quantum physics of hydrogen clusters.

We present results of a comprehensive theoretical investigation of the low temperature (T) properties of clusters of para-hydrogen (p-H(2)), both pristine as well as doped with isotopic impurities (i.e., ortho-deuterium, o-D(2)). We study clusters comprising up to N = 40 molecules, by means of quantum simulations based on the continuous-space Worm algorithm. Pristine p-H(2) clusters are liquid-like and superfluid in the [Formula: see text] limit. The superfluid signal is uniform throughout these clusters; it is underlain by long cycles of permutation of molecules. Clusters with more than 22 molecules display solid-like, essentially classical behavior at temperatures down to T∼1 K; some of them are seen to turn liquid-like at sufficiently low T (quantum melting).

Monodisperse cluster crystals: Classical and quantum dynamics.

We study the phases and dynamics of a gas of monodisperse particles interacting via soft-core potentials in two spatial dimensions, which is of interest for soft-matter colloidal systems and quantum atomic gases. Using exact theoretical methods, we demonstrate that the equilibrium low-temperature classical phase simultaneously breaks continuous translational symmetry and dynamic space-time homogeneity, whose absence is usually associated with out-of-equilibrium glassy phenomena. This results in an exotic self-assembled cluster crystal with coexisting liquidlike long-time dynamical properties, which corresponds to a classical analog of supersolid behavior. We demonstrate that the effects of quantum fluctuations and bosonic statistics on cluster-glassy crystals are separate and competing: Zero-point motion tends to destabilize crystalline order, which can be restored by bosonic statistics.

Local superfluidity of parahydrogen clusters.

We study by quantum Monte Carlo simulations the local superfluid response of small (up to 27 molecules) parahydrogen clusters, down to temperatures as low as 0.05 K. We show that at low temperature superfluidity is not confined at the surface of the clusters, as recently claimed by Khairallah et al. [Phys. Rev. Lett. 98, 183401 (2007)10.1103/PhysRevLett.98.183401]. Rather, even clusters with a pronounced shell structure are essentially uniformly superfluid. Superfluidity occurs as a result of long exchange cycles involving all molecules.

Superfluidity and quantum melting of p-H2 clusters.

Structural and superfluid properties of p-H2 clusters of size up to N=40 molecules, are studied at low temperature (0.5 K