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Dramatic Plasmon Response to the Charge-Density-Wave Gap Development in 1T-TiSe_{2}.
Lin, Zijian; Wang, Cuixiang; Balassis, A; Echeverry, J P; Vasenko, A S; Silkin, V M; Chulkov, E V; Shi, Youguo; Zhang, Jiandi; Guo, Jiandong; Zhu, Xuetao.
Afiliación
  • Lin Z; Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
  • Wang C; School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 100049, China.
  • Balassis A; Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
  • Echeverry JP; School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 100049, China.
  • Vasenko AS; Department of Physics and Engineering Physics, Fordham University, 441 East Fordham Road, Bronx, New York 10458, USA.
  • Silkin VM; Universidad de Ibagué Carrera 22 Calle 67 B, Av. Ambalá Ibagué Tolima 730007, Colombia.
  • Chulkov EV; HSE University, 101000 Moscow, Russia.
  • Shi Y; I. E. Tamm Department of Theoretical Physics, P. N. Lebedev Physical Institute, Russian Academy of Sciences, 119991 Moscow, Russia.
  • Zhang J; Donostia International Physics Center (DIPC), 20018 San Sebastián/Donostia, Basque Country, Spain.
  • Guo J; Departamento de Polímeros y Materiales Avanzados: Física, Química y Tecnología, Facultad de Ciencias Químicas, Universidad del País Vasco UPV/EHU, Apartado 1072, 20080 San Sebastián/Donostia, Basque Country, Spain.
  • Zhu X; IKERBASQUE, Basque Foundation for Science, 48013 Bilbao, Basque Country, Spain.
Phys Rev Lett ; 129(18): 187601, 2022 Oct 28.
Article en En | MEDLINE | ID: mdl-36374677
1T-TiSe_{2} is one of the most studied charge density wave (CDW) systems, not only because of its peculiar properties related to the CDW transition, but also due to its status as a promising candidate of exciton insulator signaled by the proposed plasmon softening at the CDW wave vector. Using high-resolution electron energy loss spectroscopy, we report a systematic study of the temperature-dependent plasmon behaviors of 1T-TiSe_{2}. We unambiguously resolve the plasmon from phonon modes, revealing the existence of Landau damping to the plasmon at finite momentums, which does not support the plasmon softening picture for exciton condensation. Moreover, we discover that the plasmon lifetime at zero momentum responds dramatically to the band gap evolution associated with the CDW transition. The interband transitions near the Fermi energy in the normal phase are demonstrated to serve as a strong damping channel of plasmons, while such a channel in the CDW phase is suppressed due to the CDW gap opening, which results in the dramatic tunability of the plasmon in semimetals or small-gap semiconductors.

Texto completo: 1 Banco de datos: MEDLINE Idioma: En Revista: Phys Rev Lett Año: 2022 Tipo del documento: Article País de afiliación: China

Texto completo: 1 Banco de datos: MEDLINE Idioma: En Revista: Phys Rev Lett Año: 2022 Tipo del documento: Article País de afiliación: China