Excitation of a single atom with exponentially rising light pulses.

We investigate the interaction between a single atom and optical pulses in a coherent state with a controlled temporal envelope. In a comparison between a rising exponential and a square envelope, we show that the rising exponential envelope leads to a higher excitation probability for fixed low average photon numbers, in accordance with a time-reversed Weisskopf-Wigner model. We characterize the atomic transition dynamics for a wide range of the average photon numbers and are able to saturate the optical transition of a single atom with ≈50 photons in a pulse by a strong focusing technique.

Preparation of an exponentially rising optical pulse for efficient excitation of single atoms in free space.

We report on a simple method to prepare optical pulses with exponentially rising envelope on the time scale of a few ns. The scheme is based on the exponential transfer function of a fast transistor, which generates an exponentially rising envelope that is transferred first on a radio frequency carrier, and then on a coherent cw laser beam with an electro-optical phase modulator. The temporally shaped sideband is then extracted with an optical resonator and can be used to efficiently excite a single (87)Rb atom.