Quantum linewidth limitation of a laser stabilized with a nonlinear microcavity.

We show that the linewidth of a laser locked to an optical cavity characterized with nonzero optical cubic nonlinearity is restricted by the value of the nonlinear frequency shift of the cavity mode per single photon localized in the mode. This effect is masked by the fundamental thermodynamic noise in monolithic microcavities. The quantum limit of the linewidth can be measured using two independent lasers separately locked to spatially overlapping modes of the nonlinear resonator.

Low threshold Kerr solitons.

Pumping a nonlinear optical cavity with continuous wave coherent light can result in generation of a stable train of short optical pulses. Pumping the cavity with a non-degenerate resonant coherent dichromatic pump usually does not produce a stable mode-locked regime due to competition of the oscillations at the pump frequencies. We show that generation of stable optical pulses is feasible in a dichromatically pumped cavity characterized with group velocity dispersion optimized in a way that the group velocity value becomes identical for the generated pulses and the beat note of the pump harmonics. The power threshold of the process drops nearly four times in this case and the produced pulses become sub-harmonically locked to the dichromatic pump harmonics. The process is useful for generation of broadband optical frequency combs and optical time crystals.

Towards chip-scale optical frequency synthesis based on optical heterodyne phase-locked loop.

An integrated heterodyne optical phase-locked loop was designed and demonstrated with an indium phosphide based photonic integrated circuit and commercial off-the-shelf electronic components. As an input reference, a stable microresonator-based optical frequency comb with a 50-dB span of 25 nm (~3 THz) around 1550 nm, having a spacing of ~26 GHz, was used. A widely-tunable on-chip sampled-grating distributed-Bragg-reflector laser is offset locked across multiple comb lines. An arbitrary frequency synthesis between the comb lines is demonstrated by tuning the RF offset source, and better than 100Hz tuning resolution with ± 5 Hz accuracy is obtained. Frequency switching of the on-chip laser to a point more than two dozen comb lines away (~5.6 nm) and simultaneous locking to the corresponding nearest comb line is also achieved in a time ~200 ns. A low residual phase noise of the optical phase-locking system is successfully achieved, as experimentally verified by the value of -80 dBc/Hz at an offset of as low as 200 Hz.

Bose-Hubbard hopping due to resonant Rayleigh scattering.

We show theoretically that dynamic behavior of light confined in the modes of a nonlinear optical ring cavity characterized by resonant Rayleigh scattering can be described using the Bose-Hubbard model. Nonlinear interaction between clockwise and counterclockwise optical modes results in instability and intermode hopping occurring at a rate defined by the frequency separation of the Rayleigh doublet harmonics. Hopping may lead to an instability and breathing behavior of a Kerr frequency comb observed in the cavity.

Microresonator-stabilized extended-cavity diode laser for supercavity frequency stabilization.

We demonstrate a simple, compact, and cost-effective laser noise reduction method for stabilizing an extended-cavity diode laser to a 3×105 finesse mirror Fabry-Perot (F-P) cavity, corresponding to a resonance linewidth of 10 kHz, by using a crystalline MgF2 whispering gallery mode microresonator. The laser linewidth is reduced to sub-kilohertz such that a stable Pound-Drever-Hall error signal is built up. The wavelength of the pre-stabilized laser is tunable within a large bandwidth covering the high-reflection mirror coating of an F-P supercavity.

On Sagnac frequency splitting in a solid-state ring Raman laser.

We report on an accurate measurement of the frequency splitting of an optical rotating ring microcavity made out of calcium fluoride. By measuring the frequencies of the clockwise and counter-clockwise coherent Raman emissions confined in the cavity modes, we show that the frequency splitting is inversely proportional to the refractive index of the cavity host material. The measurement has an accuracy of 1% and unambiguously confirms the classical theoretical prediction based on special theory of relativity. This Letter also demonstrates the usefulness of the ring Raman microlaser for rotation measurements.

Clustered frequency comb.

We show theoretically that it is feasible to generate a spectrally broad Kerr frequency comb consisting of several spectral clusters phase matched due to interplay among second- and higher-order group velocity dispersion contributions. We validate the theoretical analysis experimentally by driving a magnesium fluoride resonator, characterized with 110 GHz free spectral range, with a continuous wave light at 1.55 µm and observing two comb clusters separated by nearly two-thirds of an octave.

Ultrahigh Q whispering gallery mode electro-optic resonators on a silicon photonic chip.

Crystalline whispering gallery mode (WGM) electro-optic resonators made of LiNbO3 and LiTaO3 are critical for a wide range of applications in nonlinear and quantum optics, as well as RF photonics, due to their remarkably ultrahigh Q(>108) and large electro-optic coefficient. Achieving efficient coupling of these resonators to planar on-chip optical waveguides is essential for any high-yield and robust practical applications. However, it has been very challenging to demonstrate such coupling while preserving the ultrahigh Q properties of the resonators. Here, we show how the silicon photonic platform can overcome this long-standing challenge. Silicon waveguides with appropriate designs enable efficient and strong coupling to these WGM electro-optic resonators. We discuss various integration architectures of these resonators onto a silicon chip and experimentally demonstrate critical coupling of a planar Si waveguide and an ultrahigh QLiTaO3 resonator (Q∼108). Our results show a promising path for widespread and practical applications of these resonators on a silicon photonic platform.

Optical Cherenkov radiation in overmoded microresonators.

We show that an optical analog of Cherenkov radiation (dispersive wave) is observable in a nonlinear microring resonator generating Kerr frequency comb and containing linearly interacting families of equidistant modes. The radiation results from disruptions in the frequency dependent group velocity dispersion of the pumped cavity modes and is emitted into different mode families of the resonator. This effect reveals itself as a dispersive shaped structure in the spectral envelope of the frequency comb. We found that the dips in the comb spectrum correspond to peaks of the emission of the power in the other mode families of the resonator. The spectrum of the combs that includes both mode families does not have any dips, but peaks and resembles the Cherenkov radiation spectra frequently observed in Kerr comb systems. This Letter shows that a correct description of the Kerr comb in presence of mode anti-crossings should take into account not only the pumped mode family with modified dispersion parameter, but also the modes of the interacting families.

Microresonator stabilized 2 µm distributed-feedback GaSb-based diode laser.

We report on the stabilization of a high-power distributed feedback (DFB) semiconductor laser operating at 2.05 µm wavelength, using a crystalline whispering gallery mode microresonator. The laser's frequency noise is measured to be below 100 Hz/Hz1/2 at Fourier frequencies ranging from 10 Hz to 1 MHz. The instantaneous linewidth of the laser is improved by four orders of magnitude compared with the free-running DFB laser, and is measured to be 15 Hz at 0.1 ms measurement time. The integral linewidth approaches 100 Hz. The stabilized DFB laser is integrated with a polarization maintaining output fiber and an integrated optical isolator.

Stabilized chip-scale Kerr frequency comb via a high-Q reference photonic microresonator.

We stabilize a chip-scale Si3N4 phase-locked Kerr frequency comb via locking the pump laser to an independent stable high-Q reference microresonator and locking the comb spacing to an external microwave oscillator. In this comb, the pump laser shift induces negligible impact on the comb spacing change. This scheme is a step toward miniaturization of the stabilized Kerr comb system as the microresonator reference can potentially be integrated on-chip. Fractional instability of the optical harmonics of the stabilized comb is limited by the microwave oscillator used for a comb spacing lock below 1 s averaging time and coincides with the pump laser drift in the long term.

Tunable Microcavity-Stabilized Quantum Cascade Laser for Mid-IR High-Resolution Spectroscopy and Sensing.

The need for highly performing and stable methods for mid-IR molecular sensing and metrology pushes towards the development of more and more compact and robust systems. Among the innovative solutions aimed at answering the need for stable mid-IR references are crystalline microresonators, which have recently shown excellent capabilities for frequency stabilization and linewidth narrowing of quantum cascade lasers with compact setups. In this work, we report on the first system for mid-IR high-resolution spectroscopy based on a quantum cascade laser locked to a CaF2 microresonator. Electronic locking narrows the laser linewidth by one order of magnitude and guarantees good stability over long timescales, allowing, at the same time, an easy way for finely tuning the laser frequency over the molecular absorption line. Improvements in terms of resolution and frequency stability of the source are demonstrated by direct sub-Doppler recording of a molecular line.

Extended ultrahigh-Q-cavity diode laser.

We report on a study of a 698 nm extended cavity semiconductor laser with intracavity narrowband optical feedback from a whispering gallery mode resonator. This laser comprises an ultrahigh-Q (>10(10)) resonator supporting stimulated Rayleigh scattering, a diffraction grating wavelength preselector, and a reflective semiconductor amplifier. Single longitudinal mode lasing is characterized with sub-kilohertz linewidth and a 9 nm coarse tuning range. The laser has a potential application for integration with the 1S0-3P0 strontium transition to create compact precision atomic clocks.

Generation of Kerr combs centered at 4.5 µm in crystalline microresonators pumped with quantum-cascade lasers.

We report on the generation of mid-infrared Kerr frequency combs in high-finesse CaF2 and MgF2 whispering-gallery-mode resonators pumped with continuous-wave room-temperature quantum cascade lasers. The combs were centered at 4.5 µm, the longest wavelength to date. A frequency comb wider than one half of an octave was demonstrated when approximately 20 mW of pump power was coupled to an MgF2 resonator characterized with quality factor exceeding 10(8).

Compact stabilized semiconductor laser for frequency metrology.

We report on the development of a frequency modulatable 795 nm semiconductor laser based on self-injection locking to a high-quality-factor whispering-gallery-mode microresonator. The laser is characterized by residual amplitude modulation below -80 dB and frequency noise better than 300 Hz/Hz(1/2) at offset frequencies ranging from 100 Hz to 10 MHz. The frequency modulation speed and span of the laser exceed 1 MHz and 4 GHz, respectively. Locking of the laser to the Doppler-free saturated absorption resonance of the (87)Rb D1 line is demonstrated and relative frequency stability better than 10(-12) is measured for integration time spanning from 1 s to 1 day. The architecture demonstrated in this study is suitable for the realization of frequency modulatable lasers at any wavelength.

Generation of a coherent near-infrared Kerr frequency comb in a monolithic microresonator with normal GVD.

We demonstrate experimentally, and describe theoretically, generation of a wide, fundamentally phase-locked Kerr frequency comb in a nonlinear resonator with a normal group velocity dispersion (GVD). A magnesium fluoride whispering-gallery mode resonator characterized with 10 GHz free spectral range and pumped either at 780 or 795 nm is used in the experiment. The envelope of the observed frequency comb differs significantly from the Kerr frequency comb spectra reported previously. We show via numerical simulation that, while the frequency comb does not correspond to generation of short optical pulses, the relative phase of the generated harmonics are fixed.

Nonlinear conversion efficiency in Kerr frequency comb generation.

We analytically and numerically investigate the nonlinear conversion efficiency in ring microresonator-based mode-locked frequency combs under different dispersion conditions. Efficiency is defined as the ratio of the average round trip energy values for the generated pulse(s) to the input pump light. We find that the efficiency degrades with growth of the comb spectral width and is inversely proportional to the number of comb lines. It depends on the cold-cavity properties of a microresonator only and can be improved by increasing the coupling coefficient. Also, it can be increased in the multi-soliton state.

On timing jitter of mode locked Kerr frequency combs.

We study fundamental timing jitter in repetition rate of a mode locked Kerr frequency comb generated in an externally pumped nonlinear ring resonator. We show that the increase in the integrated power of the comb harmonics, and the corresponding decrease of the duration of the associated pulse, results in the increase of low frequency noise, and a decrease in high frequency noise.

All-optical dissipative discrete time crystals.

Time crystals are periodic states exhibiting spontaneous symmetry breaking in either time-independent or periodically-driven quantum many-body systems. Spontaneous modification of discrete time-translation symmetry in periodically-forced physical systems can create a discrete time crystal (DTC) constituting a state of matter possessing properties like temporal rigid long-range order and coherence, which are inherently desirable for quantum computing and information processing. Despite their appeal, experimental demonstrations of DTCs are scarce and significant aspects of their behavior remain unexplored. Here, we report the experimental observation and theoretical investigation of DTCs in a Kerr-nonlinear optical microcavity. Empowered by the self-injection locking of two independent lasers with arbitrarily large frequency separation simultaneously to two same-family cavity modes and a dissipative Kerr soliton, this versatile platform enables realizing long-awaited phenomena such as defect-carrying DTCs and phase transitions. Combined with monolithic microfabrication, this room-temperature system paves the way for chip-scale time crystals supporting real-world applications outside sophisticated laboratories.

Optical resonant sensors: a method to reduce the effect of thermal drift.

The use of a whispering gallery mode (WGM) resonator with an ultrahigh quality factor Q is promising in highly sensitive, label-free, lab-on-a-chip sensor applications. We investigated a novel method of using the differential frequency of TE and TM modes to reduce the thermal noise baseline, which commonly limits the sensitivity of WGM sensors. We studied the temperature dependence of WGM based sensors and experimentally demonstrated the reduction of temperature fluctuation and thus a significant improvement in the practical sensor detection limit.