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Sound attenuation in stable glasses.
Wang, Lijin; Berthier, Ludovic; Flenner, Elijah; Guan, Pengfei; Szamel, Grzegorz.
Affiliation
  • Wang L; Beijing Computational Science Research Center, Beijing 100193, P. R. China. pguan@csrc.ac.cn and Department of Chemistry, Colorado State University, Fort Collins, Colorado 80523, USA. flennere@gmail.com.
  • Berthier L; Laboratoire Charles Coulomb (L2C), University of Montpellier, CNRS, 34095 Montpellier, France.
  • Flenner E; Department of Chemistry, Colorado State University, Fort Collins, Colorado 80523, USA. flennere@gmail.com.
  • Guan P; Beijing Computational Science Research Center, Beijing 100193, P. R. China. pguan@csrc.ac.cn.
  • Szamel G; Department of Chemistry, Colorado State University, Fort Collins, Colorado 80523, USA. flennere@gmail.com.
Soft Matter ; 15(35): 7018-7025, 2019 Sep 21.
Article in En | MEDLINE | ID: mdl-31433423
ABSTRACT
Understanding the difference between the universal low-temperature properties of amorphous and crystalline solids requires an explanation for the stronger damping of long-wavelength phonons in amorphous solids. A longstanding sound attenuation scenario, resulting from a combination of experiments, theories, and simulations, leads to a quartic scaling of sound attenuation with the wavevector, which is commonly attributed to the Rayleigh scattering of sound. Modern computer simulations offer conflicting conclusions regarding the validity of this picture. We simulate glasses with an unprecedentedly broad range of stabilities to perform the first microscopic analysis of sound damping in model glass formers across a range of experimentally relevant preparation protocols. We present convincing evidence that quartic scaling is recovered for small wavevectors irrespective of the glass's stability. With increasing stability, the wavevector where the quartic scaling begins increases by approximately a factor of three and the sound attenuation decreases by over an order of magnitude. Our results uncover an intimate connection between glass stability and sound damping.

Full text: 1 Collection: 01-internacional Database: MEDLINE Type of study: Prognostic_studies Language: En Journal: Soft Matter Year: 2019 Type: Article Affiliation country: United States

Full text: 1 Collection: 01-internacional Database: MEDLINE Type of study: Prognostic_studies Language: En Journal: Soft Matter Year: 2019 Type: Article Affiliation country: United States