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Molecular-Modified Photocathodes for Applications in Artificial Photosynthesis and Solar-to-Fuel Technologies.
Reyes Cruz, Edgar A; Nishiori, Daiki; Wadsworth, Brian L; Nguyen, Nghi P; Hensleigh, Lillian K; Khusnutdinova, Diana; Beiler, Anna M; Moore, G F.
Afiliación
  • Reyes Cruz EA; School of Molecular Sciences and the Biodesign Institute Center for Applied Structural Discovery (CASD), Arizona State University, Tempe, Arizona 85287-1604, United States.
  • Nishiori D; School of Molecular Sciences and the Biodesign Institute Center for Applied Structural Discovery (CASD), Arizona State University, Tempe, Arizona 85287-1604, United States.
  • Wadsworth BL; School of Molecular Sciences and the Biodesign Institute Center for Applied Structural Discovery (CASD), Arizona State University, Tempe, Arizona 85287-1604, United States.
  • Nguyen NP; School of Molecular Sciences and the Biodesign Institute Center for Applied Structural Discovery (CASD), Arizona State University, Tempe, Arizona 85287-1604, United States.
  • Hensleigh LK; School of Molecular Sciences and the Biodesign Institute Center for Applied Structural Discovery (CASD), Arizona State University, Tempe, Arizona 85287-1604, United States.
  • Khusnutdinova D; School of Molecular Sciences and the Biodesign Institute Center for Applied Structural Discovery (CASD), Arizona State University, Tempe, Arizona 85287-1604, United States.
  • Beiler AM; School of Molecular Sciences and the Biodesign Institute Center for Applied Structural Discovery (CASD), Arizona State University, Tempe, Arizona 85287-1604, United States.
  • Moore GF; School of Molecular Sciences and the Biodesign Institute Center for Applied Structural Discovery (CASD), Arizona State University, Tempe, Arizona 85287-1604, United States.
Chem Rev ; 122(21): 16051-16109, 2022 11 09.
Article en En | MEDLINE | ID: mdl-36173689
Nature offers inspiration for developing technologies that integrate the capture, conversion, and storage of solar energy. In this review article, we highlight principles of natural photosynthesis and artificial photosynthesis, drawing comparisons between solar energy transduction in biology and emerging solar-to-fuel technologies. Key features of the biological approach include use of earth-abundant elements and molecular interfaces for driving photoinduced charge separation reactions that power chemical transformations at global scales. For the artificial systems described in this review, emphasis is placed on advancements involving hybrid photocathodes that power fuel-forming reactions using molecular catalysts interfaced with visible-light-absorbing semiconductors.
Asunto(s)

Texto completo: 1 Colección: 01-internacional Banco de datos: MEDLINE Asunto principal: Fotosíntesis / Energía Solar Idioma: En Revista: Chem Rev Año: 2022 Tipo del documento: Article País de afiliación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Banco de datos: MEDLINE Asunto principal: Fotosíntesis / Energía Solar Idioma: En Revista: Chem Rev Año: 2022 Tipo del documento: Article País de afiliación: Estados Unidos