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Small ; 20(19): e2307045, 2024 May.
Artículo en Inglés | MEDLINE | ID: mdl-38100142

RESUMEN

Since WHO has declared the COVID-19 outbreak a global pandemic, nearly seven million deaths have been reported. This efficient spread of Severe Acute Respiratory Syndrome Coronavirus-2 (SARS-CoV-2) is facilitated by the ability of the spike glycoprotein to bind multiple cell membrane receptors. Although ACE2 is identified as the main receptor for SARS-CoV-2, other receptors could play a role in viral entry. Among others, C-type lectins such as DC-SIGN are identified as efficient trans-receptor for SARS-CoV-2 infection, so the use of glycomimetics to inhibit the infection through the DC-SIGN blockade is an encouraging approach. In this regard, multivalent nanostructures based on glycosylated [60]fullerenes linked to a central porphyrin scaffold have been designed and tested against DC-SIGN-mediated SARS-CoV-2 infection. First results show an outstanding inhibition of the trans-infection up to 90%. In addition, a deeper understanding of nanostructure-receptor binding is achieved through microscopy techniques, high-resolution NMR experiments, Quartz Crystal Microbalance experiments, and molecular dynamic simulations.


Asunto(s)
Moléculas de Adhesión Celular , Fulerenos , Lectinas Tipo C , Porfirinas , Receptores de Superficie Celular , SARS-CoV-2 , Humanos , Moléculas de Adhesión Celular/metabolismo , Moléculas de Adhesión Celular/antagonistas & inhibidores , COVID-19/virología , Tratamiento Farmacológico de COVID-19 , Fulerenos/química , Fulerenos/farmacología , Lectinas Tipo C/metabolismo , Lectinas Tipo C/antagonistas & inhibidores , Simulación de Dinámica Molecular , Porfirinas/química , Porfirinas/farmacología , Unión Proteica , Receptores de Superficie Celular/metabolismo , Receptores de Superficie Celular/antagonistas & inhibidores , SARS-CoV-2/efectos de los fármacos , SARS-CoV-2/metabolismo , Glicoproteína de la Espiga del Coronavirus/metabolismo , Glicoproteína de la Espiga del Coronavirus/química
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