Parametric Amplifiers Based on Quantum Dots.

Josephson parametric amplifiers (JPAs) approaching quantum-limited noise performance have been instrumental in enabling high fidelity readout of superconducting qubits and, recently, semiconductor quantum dots (QDs). We propose that the quantum capacitance arising in electronic two-level systems (the dual of Josephson inductance) can provide an alternative dissipationless nonlinear element for parametric amplification. We experimentally demonstrate phase-sensitive parametric amplification using a QD-reservoir electron transition in a CMOS nanowire split-gate transistor embedded in a 1.8 GHz superconducting lumped-element microwave cavity, achieving parametric gains of -3 to +3 dB, limited by Sisyphus dissipation. Using a semiclassical model, we find an optimized design within current technological capabilities could achieve gains and bandwidths comparable to JPAs, while providing complementary specifications with respect to integration in semiconductor platforms or operation at higher magnetic fields.

Pure Spin Currents Driven by Colossal Spin-Orbit Coupling on Two-Dimensional Surface Conducting SrTiO3.

Spin accumulation is generated by passing a charge current through a ferromagnetic layer and sensed by other ferromagnetic layers downstream. Pure spin currents can also be generated in which spin currents flow and are detected as a nonlocal resistance in which the charge current is diverted away from the voltage measurement point. Here, we report nonlocal spin-transport on two-dimensional surface-conducting SrTiO3 (STO) without a ferromagnetic spin-injector via the spin Hall effect (and inverse spin Hall effect). By applying magnetic fields to the Hall bars at different angles to the nonlocal spin-diffusion, we demonstrate an anisotropic spin-signal that is consistent with a Hanle precession of a pure spin current. We extract key transport parameters for surface-conducting STO, including: a spin Hall angle of γ ≈ (0.25 ± 0.05), a spin lifetime of τ ∼ 49 ps, and a spin diffusion length of λs ≈ (1.23 ± 0.7) µm at 2 K.

Nanoscale Domain Wall Engineered Spin-Triplet Josephson Junctions and SQUID.

Spin-singlet Cooper pairs convert to spin-triplet Cooper pairs on passing through a magnetically noncollinear structure at a superconductor(S)/ferromagnet(F) interface. In this context, the generation of triplet supercurrents through intrinsic ferromagnetic domain walls, which are naturally occurring noncollinear magnetic features, was proposed theoretically in the past decade. However, an experimental demonstration has been lacking in the literature, particularly because of the difficulty in accessing a single domain wall, which is typically buried between two domains in a ferromagnetic material. By patterning a ferromagnetic nanoconstriction, we have been able to realize a nanoscale S/F/S planar junction, where a single domain wall (pinned at the nanoconstriction) acts as a Josephson barrier. In this geometry, we are able to show the predicted long-range triplet supercurrent across a ferromagnetic barrier exceeding 70 nm. Using this technique, we have demonstrated a ferromagnetic planar nano-SQUID device consisting of two Nb/Ni/Nb spin-triplet Josephson junctions.

Superconducting Sr2RuO4 Thin Films without Out-of-Phase Boundaries by Higher-Order Ruddlesden-Popper Intergrowth.

Ruddlesden-Popper (RP) phases (An+1BnO3n+1, n = 1, 2,···) have attracted intensive research with diverse functionalities for device applications. However, the realization of a high-quality RP-phase film is hindered by the formation of out-of-phase boundaries (OPBs) that occur at terrace edges, originating from lattice mismatch in the c-axis direction with the A'B'O3 (n = ∞) substrate. Here, using strontium ruthenate RP-phase Sr2RuO4 (n = 1) as a model system, an experimental approach for suppressing OPBs was developed. By tuning the growth parameters, the Sr3Ru2O7 (n = 2) phase was formed in a controlled manner near the film-substrate interface. This higher-order RP-phase then blocked the subsequent formation of OPBs, resulting in nearly defect-free Sr2RuO4 layer at the upper region of the film. Consequently, the Sr2RuO4 thin films exhibited superconductivity up to 1.15 K, which is the highest among Sr2RuO4 films grown by pulsed laser deposition. This work paves the way for synthesizing pristine RP-phase heterostructures and exploring their unique physical properties.

Controllable Enhancement of p-Wave Superconductivity via Magnetic Coupling to a Conventional Superconductor.

Unconventional superconductors are of high interest due to their rich physics, a topical example being topological edge states associated with p-wave superconductivity. A practical obstacle in studying such systems is the very low critical temperature T_{c} that is required to realize a p-wave superconducting phase in a material. We predict that the T_{c} of an intrinsic p-wave superconductor can be significantly enhanced by coupling to a conventional s-wave or d-wave superconductor with a higher critical temperature via an atomically thin ferromagnetic (F) layer. We show that this T_{c} boost is tunable via the direction of the magnetization in F. Moreover, we show that the enhancement in T_{c} can also be achieved using the Zeeman effect of an external magnetic field. Our findings provide a way to increase T_{c} in p-wave superconductors in a controllable way and make the exotic physics associated with such materials more easily accessible experimentally.

Enhanced spin pumping into superconductors provides evidence for superconducting pure spin currents.

Unlike conventional spin-singlet Cooper pairs, spin-triplet pairs can carry spin1,2. Triplet supercurrents were discovered in Josephson junctions with metallic ferromagnet spacers, where spin transport can occur only within the ferromagnet and in conjunction with a charge current. Ferromagnetic resonance injects a pure spin current from a precessing ferromagnet into adjacent non-magnetic materials3,4. For spin-singlet pairing, the ferromagnetic resonance spin pumping efficiency decreases below the critical temperature (Tc) of a coupled superconductor5,6. Here we present ferromagnetic resonance experiments in which spin sink layers with strong spin-orbit coupling are added to the superconductor. Our results show that the induced spin currents, rather than being suppressed, are substantially larger in the superconducting state compared with the normal state; although further work is required to establish the details of the spin transport process, we show that this cannot be mediated by quasiparticles and is most likely a triplet pure spin supercurrent.

Electric-field control of ferromagnetism in a nanocomposite via a ZnO phase.

La2CoMnO6 (LcmO)-ZnO nanocomposite thin films grown on SrTiO3 and Nb-SrTiO3 (001) are investigated. The films grow in the form of self-assembled epitaxial vertically aligned structures. We show that, at 120 K, an electric field applied across the nanocomposite reversibly alters magnetic properties of LcmO. The effect is consistent with charge-mediated coupling between magnetism and an electric field that can be induced by changes in ion valences.

Direct observation of a superconducting vortex diode.

The interplay between magnetism and superconductivity can lead to unconventional proximity and Josephson effects. A related phenomenon that has recently attracted considerable attention is the superconducting diode effect, in which a nonreciprocal critical current emerges. Although superconducting diodes based on superconductor/ferromagnet (S/F) bilayers were demonstrated more than a decade ago, the precise underlying mechanism remains unclear. While not formally linked to this effect, the Fulde-Ferrell-Larkin-Ovchinikov (FFLO) state is a plausible mechanism due to the twofold rotational symmetry breaking caused by the finite center-of-mass-momentum of the Cooper pairs. Here, we directly observe asymmetric vortex dynamics that uncover the mechanism behind the superconducting vortex diode effect in Nb/EuS (S/F) bilayers. Based on our nanoscale SQUID-on-tip (SOT) microscope and supported by in-situ transport measurements, we propose a theoretical model that captures our key results. The key conclusion of our model is that screening currents induced by the stray fields from the F layer are responsible for the measured nonreciprocal critical current. Thus, we determine the origin of the vortex diode effect, which builds a foundation for new device concepts.

Modification of Weak Localization in Metallic Thin Films Due to the Adsorption of Chiral Molecules.

We perform low-temperature magneto-conductance measurements on Cu and Au thin films with adsorbed chiral molecules and investigate their phase-coherent transport properties. Upon adsorption of chiral molecules, the spin-orbit coupling strength in Cu decreases and the Au films become ferromagnetic as evident from weak localization and antilocalization data. A theoretical model indicates that anisotropy in the molecular tilt angles, provided that the chiral molecules act as magnetic moments, induces a nonvanishing magnetic exchange interaction, causing changes in the spin-orbit coupling strength in Cu and Au. Our work adds a new viewpoint to the plethora of unique phenomena emerging from chiral molecule adsorption on materials.

Spin-orbit coupling suppression and singlet-state blocking of spin-triplet Cooper pairs.

An inhomogeneous magnetic exchange field at a superconductor/ferromagnet interface converts spin-singlet Cooper pairs to a spin-polarized triplet state. Although the decay envelope of triplet pairs within ferromagnetic materials is well studied, little is known about their decay in nonmagnetic metals and superconductors and, in particular, in the presence of spin-orbit coupling (SOC). Here, we investigate devices in which singlet and triplet supercurrents propagate into the s-wave superconductor Nb. In the normal state of Nb, triplet supercurrents decay over a distance of 5 nm, which is an order of magnitude smaller than the decay of spin-singlet pairs due to the SOC. In the superconducting state of Nb, triplet supercurrents are not able to couple with the singlet wave function and are thus blocked by the absence of available equilibrium states in the singlet gap. The results offer insight into the dynamics between s-wave singlet and s-wave triplet states.

Magnetotransport and magnetic properties of amorphous [Formula: see text] thin films.

[Formula: see text] is an intermetallic compound with a bulk Curie temperature ([Formula: see text]) of 6-13 K. While existing studies have focused on [Formula: see text] crystals, amorphous thin-films of [Formula: see text] are potentially important since they would be magnetically soft without magnetocrystalline anisotropy, meaning that small external magnetic fields could reverse the direction of their magnetization. Here, we report [Formula: see text] thin-films with a thickness in the 5-200 nm range, deposited by DC magnetron sputtering onto Si(100). Films are amorphous with a weak temperature-dependent resistivity with values ranging between 150 and 300 [Formula: see text] cm. By means of noise spectroscopy, by analyzing the time-dependence of fluctuation-induced voltages, it is found that at low temperatures the resistance fluctuations are due to the Kondo effect. Volume magnetometry indicates [Formula: see text] K with a magnetic coercive field of 30 mT at 5 K for a 125-nm-thick film. The results are promising for the development of Ferromagnet(F)/Superconductor(S)/Ferromagnet(F) pseudo spin-valve devices based on amorphous [Formula: see text] thin films.

Controlling spin supercurrents via nonequilibrium spin injection.

We propose a mechanism whereby spin supercurrents can be manipulated in superconductor/ferromagnet proximity systems via nonequilibrium spin injection. We find that if a spin supercurrent exists in equilibrium, a nonequilibrium spin accumulation will exert a torque on the spins transported by this current. This interaction causes a new spin supercurrent contribution to manifest out of equilibrium, which is proportional to and polarized perpendicularly to both the injected spins and the equilibrium spin current. This is interesting for several reasons: as a fundamental physical effect; due to possible applications as a way to control spin supercurrents; and timeliness in light of recent experiments on spin injection in proximitized superconductors.

Electric control of superconducting transition through a spin-orbit coupled interface.

We demonstrate theoretically all-electric control of the superconducting transition temperature using a device comprised of a conventional superconductor, a ferromagnetic insulator, and semiconducting layers with intrinsic spin-orbit coupling. By using analytical calculations and numerical simulations, we show that the transition temperature of such a device can be controlled by electric gating which alters the ratio of Rashba to Dresselhaus spin-orbit coupling. The results offer a new pathway to control superconductivity in spintronic devices.

Strong odd-frequency correlations in fully gapped Zeeman-split superconductors.

It is now well established that at a superconductor/ferromagnet (S/F) interface an unconventional superconducting state arises in which the pairing is odd-frequency. The hallmark signature of this superconducting state is generally understood to be an enhancement of the electronic density of states (DoS) at subgap energies close to the S/F interface. However, here we show that an odd frequency state can be present even if the DoS is fully gapped. As an example, we show that this is the case in the pioneering S/FI (where FI is a insulating ferromagnet) tunneling experiments of Meservey and Tedrow, and we derive a generalized analytical criterium to describe the effect of odd-frequency pairing on the DoS. Finally, we propose a simple experiment in which odd-frequency pairing in a Zeeman-split superconductor can be unambiguously detected via the application of an external magnetic field.