Fast simulation for interacting four-level Rydberg atoms: electromagnetically induced transparency and Autler-Townes splitting.

Quantum sensing using Rydberg atoms is an emerging technology for precise measurement of electric fields. However, most existing computational methods are all based on a single-particle model and neglect Rydberg-Rydberg interaction between atoms. In this study, we introduce the interaction term into the conventional four-level optical Bloch equations. By incorporating fast iterations and solving for the steady-state solution efficiently, we avoid the computation of a massive 4N × 4N dimensional matrix. Additionally, we apply the Doppler frequency shift to each atom used in the calculation, eliminating the requirement for an additional Doppler iteration. These schemes allow for the calculation of the interaction between 7000 atoms around one minute. Based on the many-body model, we investigate the Rydberg-Rydberg interaction of Rydberg atoms under different atomic densities. Furthermore, we compare our results with the literature data of a three-level system and the experimental results of our own four-level system. The results demonstrate the validity of our model, with an effective error of 4.59% compared to the experimental data. Finally, we discover that the many-body model better predicts the linear range for measuring electric fields than the single-particle model, making it highly applicable in precise electric field measurements.

Wavelength division multiplexing based on the coupling effect of helical edge states in two-dimensional dielectric photonic crystals.

Photonic topological insulators with topologically protected edge states featuring one-way, robustness and backscattering-immunity possess extraordinary abilities to steer and manipulate light. In this work, we construct a topological heterostructure (TH) consisting of a domain of nontrivial pseudospin-type topological photonic crystals (PCs) sandwiched between two domains of trivial PCs based on two-dimensional all-dielectric core-shell PCs in triangle lattice. We consider three THs with different number of layers in the middle nontrivial domain (i.e., one-layer, two-layer, three-layer) and demonstrate that the projected band diagrams of the three THs host interesting topological waveguide states (TWSs) with properties of one-way, large-area, broad-bandwidth and robustness due to coupling effect of the helical edge states associated with the two domain-wall interfaces. Moreover, taking advantage of the tunable bandgap between the TWSs by the layer number of the middle domain due to the coupling effect, a topological Y-splitter with functionality of wavelength division multiplexing is explicitly demonstrated exploiting the unique feature of the dispersion curves of TWSs in the three THs. Our work not only offers a new method to realize pseudospin-polarized large-area TWSs with tunable mode-width, but also could provide new opportunities for practical applications in on-chip multifunctional (i.e., wavelength division multiplexing) photonic devices with topological protection and information processing with pseudospin-dependent transport.

High-Q metasurface signal isolator for 1.5T surface coil magnetic resonance imaging on the go.

The combination of surface coils and metamaterials remarkably enhance magnetic resonance imaging (MRI) performance for significant local staging flexibility. However, due to the coupling in between, impeded signal-to-noise ratio (SNR) and low-contrast resolution, further hamper the future growth in clinical MRI. In this paper, we propose a high-Q metasurface decoupling isolator fueled by topological LC loops for 1.5T surface coil MRI system, increasing the magnetic field up to fivefold at 63.8 MHz. We have employed a polarization conversion mechanism to effectively eliminate the coupling between the MRI metamaterial and the radio frequency (RF) surface transmitter-receiver coils. Furthermore, a high-Q metasurface isolator was achieved by taking advantage of bound states in the continuum (BIC) for extremely high-resolution MRI and spectroscopy. An equivalent physical model of the miniaturized metasurface design was put forward through LC circuit analysis. This study opens up a promising route for the easy-to-use and portable surface coil MRI scanners.

Accurate optical optimization of light-emitting diodes with consideration of coupling between Purcell factor and transmittance coefficient.

The calculation method for light emission efficiency splits external quantum efficiency (EQE) into internal quantum efficiency (IQE) and light extraction efficiency (LEE) independently. Consequently, the IQE connected to Purcell factor and the LEE are calculated separately. This traditional method ignores the interplays between the Purcell factor and transmittance coefficient in spectral domain, which all strongly depend on emitting directions. In this work, we propose a new figure of merit to describe the light emission process accurately by using the direction-dependent Purcell factor and transmittance coefficient simultaneously. We use a specific LED structure as a numerical example to illustrate the calculation method and optimization procedure.

Bound valley edge states in the continuum.

Topological valley photonics provides a unique way to manipulate the flow of light. In general, valley edge states that exhibit unidirectional propagation and are immune to defects and disorders could be realized at the interface between two valley photonic crystals with opposite valley Chern numbers. Herein, by merging the physics of valley edge states and bound states in the continuum, we propose and numerically demonstrate a novel, to the best of our knowledge, concept of edge states termed bound valley edge states in the continuum, which enjoys the topological features of valley edge states, such as, unidirectional propagation and immunity to disorders, but are formed at the interface between air and a single valley photonic crystal. Our results not only provide an effective way to reduce the size of valley photonic structures but also facilitate new applications where the proposed concept of bound valley edge states in the continuum could be exploited for optical sensing and unidirectional waveguiding.

Integrated Terahertz Generator-Manipulators Using Epsilon-near-Zero-Hybrid Nonlinear Metasurfaces.

In terahertz (THz) technologies, generation and manipulation of THz waves are two key processes usually implemented by different device modules. Integrating THz generation and manipulation into a single compact device will advance the applications of THz technologies in various fields. Here, we demonstrate a hybrid nonlinear plasmonic metasurface incorporating an epsilon-near-zero (ENZ) indium tin oxide (ITO) layer to seamlessly combine efficient generation and manipulation of THz waves across a wide frequency band. The coupling between the plasmonic resonance of the metasurface and the ENZ mode of the ITO thin film enhances the THz conversion efficiency by more than 4 orders of magnitude. Meanwhile, such a hybrid device is capable of shaping the polarization and wavefront of the emitted THz beam via the engineered nonlinear Pancharatnam-Berry (PB) phases of the plasmonic meta-atoms. The presented hybrid nonlinear metasurface opens a new avenue toward miniaturized integrated THz devices and systems with advanced functionalities.

Multiplexing-oriented plasmon-MoS2 hybrid metasurfaces driven by nonlinear quasi bound states in the continuum.

Rapid progress in nonlinear plasmonic metasurfaces enabled many novel optical characteristics for metasurfaces, with potential applications in frequency metrology [Zimmermann et al. Opt. Lett. 29:310 (2004)], timing characterization [Singh et al. Laser Photonics Rev. 14:1 (2020)] and quantum information [Kues et al. Nature. 546:622 (2017)]. However, the spectrum of nonlinear optical response was typically determined from the linear optical resonance. In this work, a wavelength-multiplexed nonlinear plasmon-MoS2 hybrid metasurface with suppression phenomenon was proposed, where multiple nonlinear signals could to be simultaneously processed and optionally tuned. A clear physical picture to depict the nonlinear plasmonic bound states in the continuum (BICs) was presented, from the perspective of both classical and quantum approaches. Particularly, beyond the ordinary plasmon-polariton effect, we numerically demonstrated a giant BIC-inspired second-order nonlinear susceptibility 10-5m/V of MoS2 in the infrared band. The novelty in our study lies in the presence of a quantum oscillator that can be adopted to both suppress and enhance the nonlinear quasi BICs. This selectable nonlinear BIC-based suppression and enhancement effect can optionally block undesired modes, resulting in narrower linewidth as well as smaller quantum decay rates, which is also promising in slow-light-associated technologies.

Coupled cavity-waveguide based on topological corner state and edge state.

The topological corner state (TCS) and topological edge state (TES) have created new approaches to manipulate the propagation of light. The construction of a topological coupled cavity-waveguide (TCCW) based on the TCS and TES is worth looking forward to, due to its research prospects in realizing high-performance micro-nano integrated photonic devices. In this Letter, the TCCW is proposed in two-dimensional (2D) photonic crystal (PC), which possesses strong optical localization, high quality factor, and excellent robustness compared with the conventional coupled cavity-waveguide (CCCW). This work will pave the way toward designing high-performance logic gates, lasers, filters, and other micro-nano integrated photonics devices and expanding their applications.

Local orbital-angular-momentum dependent surface states with topological protection.

Chiral surface states along the zigzag edge of a valley photonic crystal in the honeycomb lattice are demonstrated. By decomposing the local fields into orbital angular momentum (OAM) modes, we find that the chiral surface states present OAM-dependent unidirectional propagation characteristics. Particularly, the propagation directivities of the surface states are quantified by the local OAM decomposition and are found to depend on the chiralities of both the source and surface states. These findings allow for the engineering control of the unidirectional propagation of electromagnetic energy without requiring an ancillary cladding layer. Furthermore, we examine the propagation of the chiral surface states against sharp bends. It turns out that although only certain states successfully pass through the bend, the unidirectional propagation is well maintained due to the topology of the structure.

Linear and nonlinear spin-orbital coupling in golden-angle spiral quasicrystals.

The appealing characteristics of quasi-crystalline nanostructure offer tremendous possibilities to tailor the transmission of the angular momenta. Moreover, the second harmonic generation existing in nonlinear nanostructures also exhibits remarkable potential in the fundamental and applied research areas of the angular momenta conversion. By systematically studying the general angular momenta conservation law, we show that the high-dimensional angular momenta transformation and spin-orbital coupling are realized by the nonlinear sunflower-type quasicrystals, which feature the high-fold rotational symmetry and possess an increasing degree of rotational symmetry in Fourier space. Interestingly, since the sequential Fibonacci numbers are essentially encoded in the distinctive nonlinear sunflower-type patterns, the high-fold angular momenta transformation regularly occurs at both linear and nonlinear wavelengths. The investigations of fundamental physics for the unique quasi-crystals reveal scientific importance for manipulating the angular momenta of nonlinear optical signals, which plays a key role in the promotion and development of modern physics.

First-principle calculation of Chern number in gyrotropic photonic crystals.

As an important figure of merit for characterizing the quantized collective behaviors of the wavefunction, Chern number is the topological invariant of quantum Hall insulators. Chern number also identifies the topological properties of the photonic topological insulators (PTIs), thus it is of crucial importance in PTI design. In this paper, we develop a first principle computatioal method for the Chern number of 2D gyrotropic photonic crystals (PCs), starting from the Maxwell's equations. Firstly, we solve the Hermitian generalized eigenvalue equation reformulated from the Maxwell's equations by using the full-wave finite-difference frequency-domain (FDFD) method. Then the Chern number is obtained by calculating the integral of Berry curvature over the first Brillouin zone. Numerical examples of both transverse-electric (TE) and transverse-magnetic (TM) modes are demonstrated, where convergent Chern numbers can be obtained using rather coarse grids, thus validating the efficiency and accuracy of the proposed method.

Nonlinearity in the Dark: Broadband Terahertz Generation with Extremely High Efficiency.

Plasmonic metamaterials and metasurfaces offer new opportunities in developing high performance terahertz emitters and detectors beyond the limitations of conventional nonlinear materials. However, simple meta-atoms for second-order nonlinear applications encounter fundamental trade-offs in the necessary symmetry breaking and local-field enhancement due to radiation damping that is inherent to the operating resonant mode and cannot be controlled separately. Here we present a novel concept that eliminates this restriction obstructing the improvement of terahertz generation efficiency in nonlinear metasurfaces based on metallic nanoresonators. This is achieved by combining a resonant dark-state metasurface, which locally drives nonlinear nanoresonators in the near field, with a specific spatial symmetry that enables destructive interference of the radiating linear moments of the nanoresonators, and perfect absorption via simultaneous electric and magnetic critical coupling of the pump radiation to the dark mode. Our proposal allows eliminating linear radiation damping, while maintaining constructive interference and effective radiation of the nonlinear components. We numerically demonstrate a giant second-order nonlinear susceptibility ∼10^{-11} m/V, a one order improvement compared with the previously reported split-ring-resonator metasurface, and correspondingly, a 2 orders of magnitude enhanced terahertz energy extraction should be expected with our configuration under the same conditions. Our study offers a paradigm of high efficiency tunable nonlinear metadevices and paves the way to revolutionary terahertz technologies and optoelectronic nanocircuitry.

Efficient volumetric method of moments for modeling plasmonic thin-film solar cells with periodic structures.

Metallic nanoparticles (NPs) support localized surface plasmon resonances (LSPRs), which enable to concentrate sunlight at the active layer of solar cells. However, full-wave modeling of the plasmonic solar cells faces great challenges in terms of huge computational workload and bad matrix condition. It is tremendously difficult to accurately and efficiently simulate near-field multiple scattering effects from plasmonic NPs embedded into solar cells. In this work, a preconditioned volume integral equation (VIE) is proposed to model plasmonic organic solar cells (OSCs). The diagonal block preconditioner is applied to different material domains of the device structure. As a result, better convergence and higher computing efficiency are achieved. Moreover, the calculation is further accelerated by two-dimensional periodic Green's functions. Using the proposed method, the dependences of optical absorption on the wavelengths and incident angles are investigated. Angular responses of the plasmonic OSCs show the super-Lambertian absorption on the plasmon resonance but near-Lambertian absorption off the plasmon resonance. The volumetric method of moments and explored physical understanding are of great help to investigate the optical responses of OSCs.

Investigation of broadband terahertz generation from metasurface.

The nonlinear metamaterials have been shown to provide nonlinear properties with high nonlinear conversion efficiency and in a myriad of light manipulation. Here we study terahertz generation from nonlinear metasurface consisting of single layer nanoscale split-ring resonator array. The terahertz generation due to optical rectification by the second-order nonlinearity of the split-ring resonator is investigated by a time-domain implementation of the hydrodynamic model for electron dynamics in metal. The results show that the nonlinear metasurface enables us to generate broadband terahertz radiation and free from quasi-phase-matching conditions. The proposed scheme provides a new concept of broadband THz source and designing nonlinear plasmonic metamaterials.

Graphene plasmonics for tuning photon decay rate near metallic split-ring resonator in a multilayered substrate.

Study of photon decay rate is essential to various optical devices, where graphene is an emerging building block due to its electrical tunability. In this paper, we study photon decay rate of a quantum emitter near a metallic split-ring resonator, which is embedded in a multilayered substrate incorporating a graphene layer. Analyzing photon decay rate in such a complex multilayered system is not only computationally challenging but also highly important to experimentally realizable devices. First, the dispersion relation of graphene plasmonics supported at a dieletric/graphene/dielectric structure is investigated systematically. Meanwhile, the dispersion relation of metallic plasmonics supported at a dielectric/metal structure is studied comparatively. According to our investigation, graphene offers several flexible tuning routes for manipulating photon decay rate, including tunable chemical potential and the emitter's position and polarization. Next, considering plasmonic waves in a graphene sheet occur in the infrared regime, we carefully design a metallic split ring resonating around the same frequency range. Consequently, this design enables a mutual interaction between graphene plasmonics and metallic plasmonics. The boundary element method with a multilayered medium Green's function is adopted in the numerical simulation. Blue-shifted and splitting resonance peaks are theoretically observed, which suggests a strong mode coupling. Moreover, the mode coupling has a switch on-off feature via electrostatically doping the graphene sheet. This work is helpful to dynamically manipulate photon decay rate in complex optical devices.

Observing abnormally large group velocity at the plasmonic band edge via a universal eigenvalue analysis.

We developed a novel universal eigenvalue analysis for 2D arbitrary nanostructures comprising dispersive and lossy materials. The complex dispersion relation (or complex Bloch band structure) of a metallic grating is rigorously calculated by the proposed algorithm with the finite-difference implementation. The abnormally large group velocity is observed at a plasmonic band edge with a large attenuation constant. Interestingly, we found the abnormal group velocity is caused by the leaky (radiation) loss, not by metallic absorption (ohmic) loss. The periodically modulated surface of the grating significantly modifies the original dispersion relation of the semi-infinite dielectric-metal structure and induces the extraordinarily large group velocity, which is different from the near-zero group velocity at photonic band edge. The work is fundamentally important to the design of plasmonic nanostructures.

Wavelength-tunable high-fidelity entangled photon sources enabled by dual Stark effects.

The construction of a large-scale quantum internet requires quantum repeaters containing multiple entangled photon sources with identical wavelengths. Semiconductor quantum dots can generate entangled photon pairs deterministically with high fidelity. However, realizing wavelength-matched quantum-dot entangled photon sources faces two difficulties: the non-uniformity of emission wavelength and exciton fine-structure splitting induced fidelity reduction. Typically, these two factors are not independently tunable, making it challenging to achieve simultaneous improvement. In this work, we demonstrate wavelength-tunable entangled photon sources based on droplet-etched GaAs quantum dots through the combined use of AC and quantum-confined Stark effects. The emission wavelength can be tuned by ~1 meV while preserving an entanglement fidelity f exceeding 0.955(1) in the entire tuning range. Based on this hybrid tuning scheme, we finally demonstrate multiple wavelength-matched entangled photon sources with f > 0.919(3), paving the way towards robust and scalable on-demand entangled photon sources for quantum internet and integrated quantum optical circuits.

Tuning optical responses of metallic dipole nanoantenna using graphene.

Nanoantennas play a fundamental role in the nanotechnology due to their capabilities to confine and enhance the light through converting the localized fields to propagating ones, and vice versa. Here, we theoretically propose a novel nanoantenna with the metal-insulator-graphene configuration where a graphene sheet dynamically controls the characteristics of a metallic dipole antenna in terms of near-field distribution, resonance frequency, bandwidth, radiation pattern, etc. Our results show that by modifying dispersion relation of the graphene sheet attached to the insulator through tuning chemical potentials, we can achieve strong mode couplings between the graphene sheet and the metallic nanoantenna on the top of the insulator. Interestingly, the in-phase and out-of-phase couplings between metallic plasmonics and graphene plasmonics not only split the single resonance frequency of the conventional metallic dipole antenna but also modify the near-field and far-field responses of the metal-graphene nanoantenna. This work is of a great help to design high-performance electrically-tunable nanoantennas applicable both in nano-optics and nano-electronics fields.

Light harvesting improvement of organic solar cells with self-enhanced active layer designs.

We present designs of organic solar cells (OSCs) incorporating periodically arranged gradient type active layer. The designs can enhance light harvesting with patterned organic materials themselves (i.e. self-enhanced active layer design) to avoid degrading electrical performances of OSCs in contrast to introducing inorganic concentrators into OSC active layers such as silicon and metallic nanostructures. Geometry of the OSC is fully optimized by rigorously solving Maxwell's equations with fast and efficient scattering matrix method. Optical absorption is accessed by a volume integral of the active layer excluding the metallic absorption. Our numerical results show that the OSC with a self-enhanced active layer, compared with the conventional planar active layer configuration, has broadband and wide-angle range absorption enhancement due to better geometric impedance matching and prolonged optical path. This work provides a theoretical foundation and engineering reference for high performance OSC designs.

Optical and electrical study of organic solar cells with a 2D grating anode.

We investigate both optical and electrical properties of organic solar cells (OSCs) incorporating 2D periodic metallic back grating as an anode. Using a unified finite-difference approach, the multiphysics modeling framework for plasmonic OSCs is established to seamlessly connect the photon absorption with carrier transport and collection by solving the Maxwell's equations and semiconductor equations (Poisson, continuity, and drift-diffusion equations). Due to the excited surface plasmon resonance, the significantly nonuniform and extremely high exciton generation rate near the metallic grating are strongly confirmed by our theoretical model. Remarkably, the nonuniform exciton generation indeed does not induce more recombination loss or smaller open-circuit voltage compared to 1D multilayer standard OSC device. The increased open-circuit voltage and reduced recombination loss by the plasmonic OSC are attributed to direct hole collections at the metallic grating anode with a short transport path. The work provides an important multiphysics understanding for plasmonic organic photovoltaics.