Motility-Induced Clustering of Active Particles under Soft Confinement.

We investigate the structural and dynamic properties of active Brownian particles (APs) confined within a soft annulus-shaped channel. Depending on the strength of the confinement and the Péclet number, we observe a novel reentrant behavior that is not present in unconfined systems. Our findings are substantiated by numerical simulations and analytical considerations, revealing that this behavior arises from the strong coupling between the Péclet number and the effective confining dimensionality of the APs. Our work highlights the peculiarities of soft boundaries for APs and how clogging can be avoided under such conditions.

Collective Hall current in chiral active fluids: Coupling of phase and mass transport through traveling bands.

Active fluids composed of constituents that are constantly driven away from thermal equilibrium can support spontaneous currents and can be engineered to have unconventional transport properties. Here, we report the emergence of (meta)stable traveling bands in computer simulations of aligning circle swimmers. These bands are different from polar flocks and, through coupling phase with mass transport, induce a bulk particle current with a component perpendicular to the propagation direction, thus giving rise to a collective Hall (or Magnus) effect. Traveling bands require sufficiently small orbits and undergo a discontinuous transition into a synchronized state with transient polar clusters for large orbital radii. Within a minimal hydrodynamic theory, we show that the bands can be understood as nondispersive soliton solutions fully accounting for the numerically observed properties.

Exploiting compositional disorder in collectives of light-driven circle walkers.

Emergent behavior in collectives of "robotic" units with limited capabilities that is robust and programmable is a promising route to perform tasks on the micro and nanoscale that are otherwise difficult to realize. However, a comprehensive theoretical understanding of the physical principles, in particular steric interactions in crowded environments, is still largely missing. Here, we study simple light-driven walkers propelled through internal vibrations. We demonstrate that their dynamics is well captured by the model of active Brownian particles, albeit with an angular speed that differs between individual units. Transferring to a numerical model, we show that this polydispersity of angular speeds gives rise to specific collective behavior: self-sorting under confinement and enhancement of translational diffusion. Our results show that, while naively perceived as imperfection, disorder of individual properties can provide another route to realize programmable active matter.

Force Generation in Confined Active Fluids: The Role of Microstructure.

We experimentally determine the force exerted by a bath of active particles onto a passive probe as a function of its distance to a wall and compare it to the measured averaged density distribution of active particles around the probe. Within the framework of an active stress, we demonstrate that both quantities are-up to a factor-directly related to each other. Our results are in excellent agreement with a minimal numerical model and confirm a general and system-independent relationship between the microstructure of active particles and transmitted forces.

Hunting active Brownian particles: Learning optimal behavior.

We numerically study active Brownian particles that can respond to environmental cues through a small set of actions (switching their motility and turning left or right with respect to some direction) which are motivated by recent experiments with colloidal self-propelled Janus particles. We employ reinforcement learning to find optimal mappings between the state of particles and these actions. Specifically, we first consider a predator-prey situation in which prey particles try to avoid a predator. Using as reward the squared distance from the predator, we discuss the merits of three state-action sets and show that turning away from the predator is the most successful strategy. We then remove the predator and employ as collective reward the local concentration of signaling molecules exuded by all particles and show that aligning with the concentration gradient leads to chemotactic collapse into a single cluster. Our results illustrate a promising route to obtain local interaction rules and design collective states in active matter.

Vorticity Determines the Force on Bodies Immersed in Active Fluids.

When immersed into a fluid of active Brownian particles, passive bodies might start to undergo linear or angular directed motion depending on their shape. Here we exploit the divergence theorem to relate the forces responsible for this motion to the density and current induced by-but far away from-the body. In general, the force is composed of two contributions: due to the strength of the dipolar field component and due to particles leaving the boundary, generating a nonvanishing vorticity of the polarization. We derive and numerically corroborate results for periodic systems, which are fundamentally different from unbounded systems with forces that scale with the area of the system. We demonstrate that vorticity is localized close to the body and to points at which the local curvature changes, enabling the rational design of particle shapes with desired propulsion properties.

From scalar to polar active matter: Connecting simulations with mean-field theory.

We study numerically the phase behavior of self-propelled elliptical particles interacting through the "hard" repulsive Gay-Berne potential at infinite Péclet number. Changing a single parameter, the aspect ratio, allows us to continuously go from discoid active Brownian particles to elongated polar rods. Discoids show phase separation, which changes to a cluster state of polar domains, which then form polar bands as the aspect ratio is increased. From the simulations, we identify and extract the two effective parameters entering the mean-field description: the force imbalance coefficient and the effective coupling to the local polarization. These two coefficients are sufficient to obtain a complete and consistent picture, unifying the paradigms of scalar and polar active matter.