Zeeman optical pumping of 87Rb atoms in a hollow-core photonic crystal fiber.

Preparation of an atomic ensemble in a particular Zeeman state is a critical step of many protocols for implementing quantum sensors and quantum memories. These devices can also benefit from optical fiber integration. In this work we describe experimental results supported by a theoretical model of single-beam optical pumping of 87Rb atoms within a hollow-core photonic crystal fiber. The observed 50% population increase in the pumped F = 2, mF = 2 Zeeman substate along with the depopulation of remaining Zeeman substates enabled us to achieve a threefold improvement in the relative population of the mF = 2 substate within the F = 2 manifold, with 60% of the F = 2 population residing in the mF = 2 dark sublevel. Based on theoretical model, we propose methods to further improve the pumping efficiency in alkali-filled hollow-core fibers.

Magnetic induction tomography of structural defects with alkali-metal spin maser.

Implementation of an alkali-metal spin maser in magnetic induction tomography is explored. While the spin maser vastly improves the detection speed and solves the problem of imperfect bias magnetic field stabilization in non-destructive testing, it provides only partial information about the spatial extent of the defect. We demonstrate two ways in which the whole image of the defect can be reconstructed and experimentally demonstrate that the amplitude of the spin maser signal can be used as an indicator of defect depth. Additionally, the spatial extent of the imaging of the defect is increased by the application of a spin maser operating at two frequencies. A significant benefit of operating in the spin maser mode is that the system follows any fluctuations in the Larmor frequency due to changes in the bias magnetic field strength. This removes the need for active stabilization of the bias magnetic field, greatly reducing the complexity of the system.

Role of the probe beam in a radio-frequency atomic magnetometer.

We explore the role of the linearly polarized probe beam in the radio-frequency atomic magnetometer. Two regimes of coupling of the linearly polarized light to the atomic ensemble, near and off-resonant, are demonstrated and discussed. Our studies cover three types of interaction between the atomic spin system and the linearly polarized beam, i.e., absorptive production of spin polarization, dispersive spin state readout, and nonlinear spin couplings. The work is performed with the outlook of optimization and simplification of magnetometer operation. Operation of a magnetometer with a single beam, generating and probing the atomic orientation, is presented. This single-beam configuration, which combines optical pumping, nonlinear spin couplings, and spin-exchange collisions, creates the option for a portable device with simple instrumentation.

Absolute frequency measurement of rubidium 5S-7S two-photon transitions.

We report the absolute frequency measurements of rubidium 5S-7S two-photon transitions with a cw laser digitally locked to an atomic transition and referenced to an optical frequency comb. The narrow, two-photon transition, 5S-7S (760 nm), insensitive to first-order in a magnetic field, is a promising candidate for frequency reference. The performed tests yielded more accurate transition frequencies than previously reported.