Polarization-Dependent Interference of Coherent Scattering from Orthogonal Dipole Moments of a Resonantly Excited Quantum Dot.

Resonant photoluminescence excitation (RPLE) spectra of a neutral InGaAs quantum dot show unconventional line shapes that depend on the detection polarization. We characterize this phenomenon by performing polarization-dependent RPLE measurements and simulating the measured spectra with a three-level quantum model. The spectra are explained by interference between fields coherently scattered from the two fine structure split exciton states, and the measurements enable extraction of the steady-state coherence between the two exciton states.

Effects of photo-neutralization on the emission properties of quantum dots.

In this paper we investigate the coherence properties of a quantum dot used as photon pair source, under two-photon resonant excitation in combination with an additional photo-neutralization laser. The photo-neutralization increases the efficiency of the excitation process and thus, the brightness of the source, by a factor of approximately 1.5 for biexciton-exciton pairs. This enhancement does not degrade the relevant coherences in the system; neither the single photon coherence time, nor the coherence of the excitation process.

Toward optical quantum information processing with quantum dots coupled to microstructures [Invited].

Major improvements have been made on semiconductor quantum dot light sources recently and now they can be seen as a serious candidate for near-future scalable photonic quantum information processing experiments. The three key parameters of these photon sources for such applications have been pushed to extreme values: almost unity single-photon purity and photon indistinguishability, and high brightness. In this paper, we review the progress achieved recently on quantum-dot-based single-photon sources. We also review some quantum information experiments where entanglement processes are achieved using semiconductor quantum dots.

Statistically background-free, phase-preserving parametric up-conversion with faint light.

We demonstrate up-conversion with no statistically significant background photons and a dynamic range of 15 decades. Near-infrared 920 nm photons were converted into the visible at 577 nm using periodically poled lithium niobate waveguides pumped by a 1550 nm laser. In addition to achieving statistically noiseless frequency up-conversion, we report a high degree of phase preservation (with fringe visibilities ≥ 0.97) at the single-photon level using an up-converting Mach-Zehnder interferometer. This background-free process opens a path to single-photon detection with no intrinsic dark count. Combined with a demonstrated photon-number preserving property of an up-converter, this work demonstrates the feasibility of noiseless frequency up-conversion of entangled photon pairs.

Efficiency vs. multi-photon contribution test for quantum dots.

The development of linear quantum computing within integrated circuits demands high quality semiconductor single photon sources. In particular, for a reliable single photon source it is not sufficient to have a low multi-photon component, but also to possess high efficiency. We investigate the photon statistics of the emission from a single quantum dot with a method that is able to sensitively detect the trade-off between the efficiency and the multi-photon contribution. Our measurements show, that the light emitted from the quantum dot when it is resonantly excited possess a very low multi-photon content. Additionally, we demonstrated, for the first time, the non-Gaussian nature of the quantum state emitted from a single quantum dot.

Manipulation of high-order scattering processes in ultrasmall optical resonators to control far-field emission.

By imposing a set of harmonic perturbations to a microcavity boundary, we induce conversion and mixing of orbital angular momentum of light via surface scattering. Multiple scattering paths are available due to high-order scattering, which can be greatly enhanced by quasidegenerate resonances. By manipulating the relative strengths of these scattering processes, we theoretically synthesize the angular momentum spectra of individual modes so as to control their far-field patterns. We demonstrate experimentally that in wavelength-scale cavities of a fixed shape, the neighboring modes can have dramatically different emission directionality. This phenomenon is robust against slight shape deviation and surface roughness, and provides a general mechanism to control the emission direction of ultrasmall resonators.

Resonant interactions between a Mollow triplet sideband and a strongly coupled cavity.

We demonstrate resonant coupling of a Mollow triplet sideband to an optical cavity in the strong coupling regime. We show that, in this regime, the resonant sideband is strongly enhanced relative to the detuned sideband. Furthermore, the linewidth of the Mollow sidebands exhibits a highly nonlinear pump power dependence when tuned across the cavity resonance due to strong resonant interactions with the cavity mode. We compare our results to calculations using the effective phonon master equation and show that the nonlinear linewidth behavior is caused by strong coherent interaction with the cavity mode that exists only when the Mollow sideband is near cavity resonance.

Quantum non-Gaussian Depth of Single-Photon States.

We introduce and experimentally explore the concept of the non-Gaussian depth of single-photon states with a positive Wigner function. The depth measures the robustness of a single-photon state against optical losses. The directly witnessed quantum non-Gaussianity withstands significant attenuation, exhibiting a depth of 18 dB, while the nonclassicality remains unchanged. Quantum non-Gaussian depth is an experimentally approachable quantity that is much more robust than the negativity of the Wigner function. Furthermore, we use it to reveal significant differences between otherwise strongly nonclassical single-photon sources.

Measurement and modification of biexciton-exciton time correlations.

Photons which are generated in a two-photon cascade process have an underlying time correlation since the spontaneous emission of the upper level populates the intermediate state. This correlation leads to a reduction of the purity of the photon emitted from the intermediate state. Here we characterize this time correlation for the biexciton-exciton cascade of an InAs/GaAs quantum dot. We show that the correlation can be reduced by tuning the biexciton transition in resonance to a planar distributed Bragg reflector cavity. The enhanced and inhibited emission into the cavity accelerates the biexciton emission and slows down the exciton emission thus reduces the correlation and increases the purity of the exciton photon. This is essential for schemes like creating time-bin entangled photon pairs from quantum dot systems.

Deterministic photon pairs and coherent optical control of a single quantum dot.

The strong confinement of semiconductor excitons in a quantum dot gives rise to atomlike behavior. The full benefit of such a structure is best observed in resonant excitation where the excited state can be deterministically populated and coherently manipulated. Because of the large refractive index and device geometry it remains challenging to observe resonantly excited emission that is free from laser scattering in III/V self-assembled quantum dots. Here we exploit the biexciton binding energy to create an extremely clean single photon source via two-photon resonant excitation of an InAs/GaAs quantum dot. We observe complete suppression of the excitation laser and multiphoton emissions. Additionally, we perform full coherent control of the ground-biexciton state qubit and observe an extended coherence time using an all-optical echo technique. The deterministic coherent photon pair creation makes this system suitable for the generation of time-bin entanglement and experiments on the interaction of photons from dissimilar sources.

Dynamics of nonclassical light from a single solid-state quantum emitter.

We measure the dynamics of a nonclassical optical field using two-time second-order correlations in conjunction with pulsed excitation. The technique quantifies single-photon purity and coherence during the excitation-decay cycle of an emitter, illustrated here using a quantum dot. We observe that for certain pump wavelengths, photons detected early in the cycle have reduced single-photon purity and coherence compared to those detected later. A model indicates that the single-photon purity dynamics are due to exciton recapture after initial emission and within the same pulse cycle.

Low-photon-number optical switching with a single quantum dot coupled to a photonic crystal cavity.

We demonstrate fast nonlinear optical switching between two laser pulses with as few as 140 photons of pulse energy by utilizing strong coupling between a single quantum dot (QD) and a photonic crystal cavity. The cavity-QD coupling is modified by a detuned pump pulse, resulting in a modulation of the scattered and transmitted amplitude of a time synchronized probe pulse that is resonant with the QD. The temporal switching response is measured to be as fast as 120 ps, demonstrating the ability to perform optical switching on picosecond timescales.

Local chirality of optical resonances in ultrasmall resonators.

In wavelength-scale cavities with chiral-symmetric geometry, wave optical effects can introduce local chirality, that is, a spatial separation of the clockwise and counterclockwise propagating resonant modes. We show that this local chirality results in unidirectional lasing emission in the far field. In the presence of a waveguide, the local chirality also allows for directional evanescent coupling of the lasing modes, and the output direction can be varied by selecting the coupling position along the cavity boundary. Our results demonstrate that the local chirality of optical resonances can be utilized to control the output directionality and enhance the collection efficiency of emission from ultrasmall resonators.

Chiral Transport of Hot Carriers in Graphene in the Quantum Hall Regime.

Photocurrent (PC) measurements can reveal the relaxation dynamics of photoexcited hot carriers beyond the linear response of conventional transport experiments, a regime important for carrier multiplication. Here, we study the relaxation of carriers in graphene in the quantum Hall regime by accurately measuring the PC signal and modeling the data using optical Bloch equations. Our results lead to a unified understanding of the relaxation processes in graphene over different magnetic field strength regimes, which is governed by the interplay of Coulomb interactions and interactions with acoustic and optical phonons. Our data provide clear indications of a sizable carrier multiplication. Moreover, the oscillation pattern and the saturation behavior of PC are manifestations of not only the chiral transport properties of carriers in the quantum Hall regime but also the chirality change at the Dirac point, a characteristic feature of a relativistic quantum Hall effect.

On- and off-resonance second-harmonic generation in GaAs microdisks.

We present a theoretical description of on- and off-resonance, 4¯-quasi-phasematched, second-harmonic generation (SHG) in microdisks made of GaAs or other materials possessing 4¯ symmetry, such as GaP or ZnSe. The theory describes the interplay between quasi-phasematching (QPM) and the cavity-resonance conditions. For optimal conversion, all waves should be resonant with the microdisk and should satisfy the 4¯-QPM condition. We explore χ(2) nonlinear mixing if one of the waves is not resonant with the microdisk cavity and calculate the second-harmonic conversion spectrum. We also describe perfectly destructive 4¯-QPM where both the fundamental and second-harmonic are on-resonance with the cavity but SHG is suppressed.

A reversibly tunable photonic crystal nanocavity laser using photochromic thin film.

We demonstrate a reversibly tunable photonic crystal quantum dot laser using a photochromic thin film. The laser is composed of a photonic crystal cavity with a bare cavity Q as high as 4500 coupled to a high density ensemble of indium arsenide quantum dots. By depositing a thin layer of photochromic material on the photonic crystal cavities, the laser can be optically tuned smoothly and reversibly over a wavelength range of 2.68 nm. Lasing is observed at temperatures as high as 80 K in the 900-1000 nm near-infrared wavelength range. The spontaneous emission coupling factor is measured to be as high as ß=0.41, indicating that the laser operates in the high-ß regime.

Strong coupling between two quantum dots and a photonic crystal cavity using magnetic field tuning.

We demonstrate strong coupling between two indium arsenide (InAs) quantum dots (QDs) and a photonic crystal cavity by using a magnetic field as a frequency tuning method. The magnetic field causes a red shift of an exciton spin state in one QD and a blue shift in the opposite exciton spin state of the second QD, enabling them to be simultaneously tuned to the same cavity resonance. This method can match the emission frequency of two QDs separated by detunings as large as 1.35 meV using a magnetic field of up to 7 T. By controlling the detuning between the two QDs we measure the vacuum Rabi splitting (VRS) both when the QDs are individually coupled to the cavity, as well as when they are coupled to the cavity simultaneously. In the latter case the oscillator strength of two QDs shows a collective behavior, resulting in enhancement of the VRS as compared to the individual cases. Experimental results are compared to theoretical calculations based on the solution to the full master equation and found to be in excellent agreement.

Photonic network laser.

We demonstrated lasing in two-dimensional trivalent network structures with short-range order. Despite the lack of translational and rotational symmetries, such structures possess a large isotropic photonic bandgap. Different from those of a photonic crystal, the band-edge modes are spatially localized and have high quality factor.

Control of lasing in biomimetic structures with short-range order.

We demonstrate lasing in photonic amorphous structures that mimic the isotropic nanostructures which produce noniridescent color in nature. Our experimental and numerical studies reveal that lasing becomes most efficient at certain frequencies, due to enhanced optical confinement by short-range order. The optimal lasing frequency can be tuned by adjusting the structure factor. This work shows that lasing in nanostructures may be effectively improved and manipulated by short-range order.

Coalescence of single photons emitted by disparate single-photon sources: the example of InAs quantum dots and parametric down-conversion sources.

Single photons produced by fundamentally dissimilar physical processes will in general not be indistinguishable. We show how photons produced from a quantum dot and by parametric down-conversion in a nonlinear crystal can be manipulated to be indistinguishable. The measured two-photon coalescence probability is 16%, and is limited by quantum-dot decoherence. Temporal filtering to the quantum-dot coherence time and accounting for detector time response increases this to 61% while retaining 25% of the events. This technique can connect different elements in a scalable quantum network.