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1.
Phys Rev Lett ; 128(11): 112002, 2022 Mar 18.
Artigo em Inglês | MEDLINE | ID: mdl-35362997

RESUMO

Higher-order hadronic corrections to the anomalous magnetic moment of the muon have been evaluated including next-to-next-to-leading-order insertions of hadronic vacuum polarization and next-to-leading-order corrections to hadronic light-by-light scattering. This leaves a set of mixed leptonic and hadronic corrections in the form of double-bubble topologies as the only remaining hadronic effect at O(α^{4}). Here, we estimate these contributions by analyzing the respective cuts of the diagrams, suggesting that the impact is limited to ≲1×10^{-11} and thus negligible at the level of the final precision of the Fermilab g-2 experiment.

2.
Langmuir ; 38(2): 762-768, 2022 Jan 18.
Artigo em Inglês | MEDLINE | ID: mdl-34985893

RESUMO

Electrical and optical applications based on micro- and nanoparticles have specific demands on their interfacial properties. These properties are strongly related to atmospheric conditions to which the particles were exposed during their formation. In this study, metallic In microparticles are synthesized by solidification of In droplets on an amorphous Mo substrate at normal pressure and under vacuum conditions. The influence of ambient pressure on the interface and surface shape is investigated. While solidification at atmospheric pressure leads to collapsed particles with undisturbed contact to the substrate, low pressures result in smooth spherical particles but with cavities inside. Numerical simulations with COMSOL Multiphysics reveal different temperature profiles and heat flux in particles during solidification for both cases. This indicates different starting conditions of the solidification, which leads to the described phenomenon eventually. The investigation of the varying process conditions on the particle shape in combination with the calculated and measured temperature curves over time gives valuable insights into new approaches to synthesize micro- and nanoparticles with defined interfacial properties. Both ambient pressure and cooling rate provide well-controllable and reliable parameters for the realization of different interfacial shapes.

3.
Beilstein J Nanotechnol ; 11: 1371-1380, 2020.
Artigo em Inglês | MEDLINE | ID: mdl-32974115

RESUMO

The dewetting process is crucial for several applications in nanotechnology. Even though not all dewetting phenomena are fully understood yet, especially regarding metallic fluids, it is clear that the formation of nanometre-sized particles, droplets, and clusters as well as their movement are strongly linked to their wetting behaviour. For this reason, the thermodynamic stability of thin metal layers (0.1-100 nm) with respect to their free energy is examined here. The decisive factor for the theoretical considerations is the interfacial energy. In order to achieve a better understanding of the interfacial interactions, three different models for estimating the interfacial energy are presented here: (i) fully theoretical, (ii) empirical, and (iii) semi-empirical models. The formation of nanometre-sized gold particles on silicon and silicon oxide substrates is investigated in detail. In addition, the strengths and weaknesses of the three models are elucidated, the different substrates used are compared, and the possibility to further process the obtained particles as nanocatalysts is verified. The importance of a persistent thin communication wetting layer between the particles and its effects on particle size and number is also clarified here. In particular, the intrinsic reduction of the Laplace pressure of the system due to material re-evaporation and Ostwald ripening describes the theoretically predicted and experimentally obtained results. Thus, dewetting phenomena of thin metal layers can be used to manufacture nanostructured devices. From this point of view, the application of gold droplets as catalysts to grow germanium nanowires on different substrates is described.

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