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Visible-Light-Induced and Iodoform-Promoted Functionalization of Ether with Secondary Sulfonyl Amides.
Zhang, Fengrong; Liu, Lanqin; Chen, Xiaoyun; Hou, Hong; Han, Ying; Yan, Chaoguo; Shi, Yaocheng; Zhu, Shaoqun.
Afiliação
  • Zhang F; School of Chemistry & Chemical Engineering, Yangzhou University, Yangzhou, 225009, China.
  • Liu L; School of Chemistry & Chemical Engineering, Yangzhou University, Yangzhou, 225009, China.
  • Chen X; School of Environmental and Chemical Engineering, Jiangsu University of Science and Technology, Zhenjiang 212005, China.
  • Hou H; School of Chemistry & Chemical Engineering, Yangzhou University, Yangzhou, 225009, China.
  • Han Y; School of Chemistry & Chemical Engineering, Yangzhou University, Yangzhou, 225009, China.
  • Yan C; School of Chemistry & Chemical Engineering, Yangzhou University, Yangzhou, 225009, China.
  • Shi Y; School of Chemistry & Chemical Engineering, Yangzhou University, Yangzhou, 225009, China.
  • Zhu S; School of Chemistry & Chemical Engineering, Yangzhou University, Yangzhou, 225009, China.
J Org Chem ; 89(1): 687-691, 2024 Jan 05.
Article em En | MEDLINE | ID: mdl-38101330
ABSTRACT
An iodoform-promoted functionalization of ether with secondary sulfonyl amides under visible-light irradiation was developed toward synthesis of hemiaminal skeleton with good to excellent isolated yields. The characterization of the isolated ether and iodoform complex revealed regioselective hydrogen atom transfer to initiate carbon radical formation and enabled the amination reaction with the sulfonamide.
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Texto completo: 1 Base de dados: MEDLINE Idioma: En Ano de publicação: 2024 Tipo de documento: Article País de afiliação: China
Texto completo
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Texto completo: 1 Base de dados: MEDLINE Idioma: En Ano de publicação: 2024 Tipo de documento: Article País de afiliação: China