Linearly excited indium fluorescence imaging for temporally resolved high-precision flame thermometry.

Two-line atomic fluorescence (TLAF) is a promising technique for two-dimensional (2D) flame thermometry. However, it suffers either from a low signal-to-noise ratio (SNR) when excited in the linear regime or a quenching effect and nonlinear behavior in the nonlinear regime. This work aims to develop a new TLAF modality, which can overcome the aforementioned limitations based on a specifically designed laser source that can generate long pulses (∼400ns) with a moderate energy of ∼0.9µJ and operate at a repetition rate up to ∼22kHz. A proof-of-concept experiment was conducted and linearly excited fluorescence images with an SNR up to ∼14 were obtained within 1 ms acquisition time by synchronizing the laser with the microchannel plate (MCP) of a 10 Hz-rate intensified camera. The SNR achieved was comparable to that of a traditional nonlinear TLAF implementation and superior to a conventional linear TLAF approach. This approach offers a novel solution for recording linearly excited indium fluorescence images and is expected to make TLAF a temporally resolved and high-precision 2D thermometry for the first time.

Simple calibrated nonlinear excitation regime two-line atomic fluorescence thermometry.

Nonlinear excitation regime two-line atomic fluorescence (NTLAF) is a promising two-dimensional (2D) thermometry technique for turbulent sooty flames. However, the complexity of calibrating three system parameters and expensive instruments restricts the application of the current NTLAF technique. Here we propose a simple and cheap NTLAF measurement approach based on a one-parameter model and tunable diode laser absorption spectroscopy (TDLAS) calibration. Using this methodology, only one system parameter, instead of three as in traditional NTLAF, is to be calibrated by path-averaged temperature acquired by the TDLAS technique. As a demonstration, instantaneous 2D thermometry data of a homemade burner were acquired using this approach, with measurement uncertainty of ∼4.5% and deviation from both reference TDLAS results and Raleigh scattering measurement results less than 50 K, typically within 20 K. This approach offers a novel simplified NTLAF solution for noncontact, in-suit, high-resolution 2D temperature measurement and is expected to greatly improve the compatibility of the NTLAF technique in scientific research and engineering applications.