Front propagation transition induced by diffraction in a liquid crystal light valve.

Driven optical systems can exhibit coexistence of equilibrium states. Traveling waves or fronts between different states present complex spatiotemporal dynamics. We investigate the mechanisms that govern the front spread. Based on a liquid crystal light valve experiment with optical feedback, we show that the front propagation does not pursue a minimization of free energy. Depending on the free propagation length in the optical feedback loop, the front speed exhibits a supercritical transition. Theoretically, from first principles, we use a model that takes it into account, characterizing the speed transition from a plateau to a growing regime. The theoretical and experimental results show quite fair agreement.

Optical textures: characterizing spatiotemporal chaos.

Macroscopic systems subjected to injection and dissipation of energy can exhibit complex spatiotemporal behaviors as result of dissipative self-organization. Here, we report a one- and two-dimensional pattern forming setup, which exhibits a transition from stationary patterns to spatiotemporal chaotic textures, based on a nematic liquid crystal layer with spatially modulated input beam and optical feedback. Using an adequate projection of spatiotemporal diagrams, we determine the largest Lyapunov exponent. Jointly, this exponent and Fourier transform allow us to distinguish between spatiotemporal chaos and amplitude turbulence concepts, which are usually merged.

Extreme events induced by spatiotemporal chaos in experimental optical patterns.

Extreme events such as rogue waves are often associated with the merging of coherent structures. We report on experimental results in the physics of extreme events emerging in a liquid-crystal light valve subjected to optical feedback, and we establish the relation of this phenomenon with the appearance of spatiotemporal chaos. This system, under particular conditions, exhibits stationary roll patterns that can be destabilized into quasi-periodic and chaotic textures when control parameters are properly modified. We have identified the parameter regions where extreme fluctuations of the amplitude can emerge and established their origin through its direct relation with the experimental largest Lyapunov exponents, the proportion of extreme events, and the normed kurtosis.

Finger front propagation in smectic-A Fréedericksz transition.

Systems with multistability are characterized by exhibiting complex nonlinear waves between equilibria. Experimentally, near the smectic-A to chiral nematic transition in a liquid crystal mixture cell with planar anchoring, we observe finger fronts emerge in the smectic-A phase when applying an electric field, a reorientation transition. Finger fronts propagate in the direction orthogonal to the anchoring. Colorimetry characterization allows us to describe the molecular reorientation transition and front dynamics. We reveal that the reorientation transition is of the first-order type and determine their critical points. The front speed is determined as a function of the applied voltage. Theoretically, based on a prototype model of liquid crystal transitions, we qualitatively describe the experimental observations. We have analytically determined the bifurcation diagram and the propagation speeds of finger fronts, finding a fair agreement with the experimental observations.

Extended stable equilibrium invaded by an unstable state.

Coexistence of states is an indispensable feature in the observation of domain walls, interfaces, shock waves or fronts in macroscopic systems. The propagation of these nonlinear waves depends on the relative stability of the connected equilibria. In particular, one expects a stable equilibrium to invade an unstable one, such as occur in combustion, in the spread of permanent contagious diseases, or in the freezing of supercooled water. Here, we show that an unstable state generically can invade a locally stable one in the context of the pattern forming systems. The origin of this phenomenon is related to the lower energy unstable state invading the locally stable but higher energy state. Based on a one-dimensional model we reveal the necessary features to observe this phenomenon. This scenario is fulfilled in the case of a first order spatial instability. A photo-isomerization experiment of a dye-dopant nematic liquid crystal, allow us to observe the front propagation from an unstable state.

Spontaneous light-induced Turing patterns in a dye-doped twisted nematic layer.

Optical pattern formation is usually due either to the combination of diffraction and nonlinearity in a Kerr medium or to the temporal modulation of light in a photosensitive chemical reaction. Here, we show a different mechanism by which light spontaneously induces stripe domains between nematic states in a twisted nematic liquid crystal layer doped with azo-dyes. Thanks to the photoisomerization process of the dopants, light in the absorption band of the dopants creates spontaneous patterns without the need of temporal modulation, diffraction, Kerr or other optical nonlinearity, but based on the different scales for dopant transport processes and nematic order parameter, which identifies a genuine Turing mechanism for this instability. Theoretically, the emergence of the stripe patterns is described on the basis of a model for the dopant concentration coupled with the nematic order parameter.