ABSTRACT
We demonstrate experimentally that by engineering the structural asymmetry of the primary unit cell of a symmetrically nanopatterned metallic film the optical transmission becomes strongly dependent on the polarization of the incident wave. By considering a specific plasmonic structure consisting of square arrays of nanoscale asymmetric cruciform apertures we show that the enhanced optical anisotropy is induced by the excitation inside the apertures of localized surface plasmon resonances. The measured transmission spectra of these plasmonic arrays show a transmission maximum whose spectral location can be tuned by almost 50% by simply varying the in-plane polarization of the incident photons. Comprehensive numerical simulations further prove that the maximum of the transmission spectra corresponds to polarization-dependent surface plasmon resonances tightly confined in the two arms of the cruciform aperture. Despite this, there are isosbestic points where the transmission, reflection, and absorption spectra are polarization-independent, regardless of the degree of asymmetry of the apertures.
Subject(s)
Computer-Aided Design , Models, Theoretical , Optical Devices , Refractometry/instrumentation , Surface Plasmon Resonance/instrumentation , Computer Simulation , Equipment Design , Equipment Failure Analysis , Light , Scattering, RadiationABSTRACT
In response to the incident light's electric field, the electron density oscillates in the plasmonic hotspots producing an electric current. Associated Ohmic losses raise the temperature of the material within the plasmonic hotspot above the melting point. A nanojet and nanosphere ejection can then be observed precisely from the plasmonic hotspots.