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Fermi liquid theory forms the basis for our understanding of the majority of metals: their resistivity arises from the scattering of well defined quasiparticles at a rate where, in the low-temperature limit, the inverse of the characteristic time scale is proportional to the square of the temperature. However, various quantum materials1-15-notably high-temperature superconductors1-10-exhibit strange-metallic behaviour with a linear scattering rate in temperature, deviating from this central paradigm. Here we show the unexpected signatures of strange metallicity in a bosonic system for which the quasiparticle concept does not apply. Our nanopatterned YBa2Cu3O7-δ (YBCO) film arrays reveal linear-in-temperature and linear-in-magnetic field resistance over extended temperature and magnetic field ranges. Notably, below the onset temperature at which Cooper pairs form, the low-field magnetoresistance oscillates with a period dictated by the superconducting flux quantum, h/2e (e, electron charge; h, Planck's constant). Simultaneously, the Hall coefficient drops and vanishes within the measurement resolution with decreasing temperature, indicating that Cooper pairs instead of single electrons dominate the transport process. Moreover, the characteristic time scale τ in this bosonic system follows a scale-invariant relation without an intrinsic energy scale: h/τ ≈ a(kBT + γµBB), where h is the reduced Planck's constant, a is of order unity7,8,11,12, kB is Boltzmann's constant, T is temperature, µB is the Bohr magneton and γ ≈ 2. By extending the reach of strange-metal phenomenology to a bosonic system, our results suggest that there is a fundamental principle governing their transport that transcends particle statistics.
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Electrones , Superconductividad , Campos Magnéticos , Metales , TemperaturaRESUMEN
Recently, log-periodic quantum oscillations have been detected in the topological materials zirconium pentatelluride (ZrTe5) and hafnium pentatelluride (HfTe5), displaying an intriguing discrete scale invariance (DSI) characteristic. In condensed materials, the DSI is considered to be related to the quasi-bound states formed by massless Dirac fermions with strong Coulomb attraction, offering a feasible platform to study the long-pursued atomic-collapse phenomenon. Here, we demonstrate that a variety of atomic vacancies in the topological material HfTe5 can host the geometric quasi-bound states with a DSI feature, resembling an artificial supercritical atom collapse. The density of states of these quasi-bound states is enhanced, and the quasi-bound states are spatially distributed in the "orbitals" surrounding the vacancy sites, which are detected and visualized by low-temperature scanning tunneling microscope/spectroscopy. By applying the perpendicular magnetic fields, the quasi-bound states at lower energies become wider and eventually invisible; meanwhile, the energies of quasi-bound states move gradually toward the Fermi energy (EF). These features are consistent with the theoretical prediction of a magnetic field-induced transition from supercritical to subcritical states. The direct observation of geometric quasi-bound states sheds light on the deep understanding of the DSI in quantum materials.
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The nature of the anomalous metal state has been a major puzzle in condensed matter physics for more than three decades. Here, we report systematic investigation and modulation of the anomalous metal states in high-temperature interface superconductor FeSe films on SrTiO_{3} substrate. Remarkably, under zero magnetic field, the anomalous metal state persists up to 20 K in pristine FeSe films, an exceptionally high temperature standing out from previous observations. In stark contrast, for the FeSe films with nanohole arrays, the characteristic temperature of the anomalous metal state is considerably reduced. We demonstrate that the observed anomalous metal states originate from the quantum tunneling of vortices adjusted by the Ohmic dissipation. Our work offers a perspective for understanding the origin and modulation of the anomalous metal states in two-dimensional bosonic systems.
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Electrons residing in a flat-band system can play a vital role in triggering spectacular phenomenology due to relatively large interactions and spontaneous breaking of different degeneracies. In this work, we demonstrate chirally twisted triple bilayer graphene, a new moiré structure formed by three pieces of helically stacked Bernal bilayer graphene, as a highly tunable flat-band system. In addition to the correlated insulators showing at integer moiré fillings, commonly attributed to interaction induced symmetry broken isospin flavors in graphene, we observe abundant insulating states at half-integer moiré fillings, suggesting a longer-range interaction and the formation of charge density wave insulators which spontaneously break the moiré translation symmetry. With weak out-of-plane magnetic field applied, as observed half-integer filling states are enhanced and more quarter-integer filling states appear, pointing toward further quadrupling moiré unit cells. The insulating states at fractional fillings combined with Hartree-Fock calculations demonstrate the observation of a new type of correlated charge density wave insulators in graphene and points to a new accessible twist manner engineering correlated moiré electronics.
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Axion field induced topological magnetoelectric response has attracted lots of attention since it was first proposed by Qi et al. [Phys. Rev. B 78, 195424 (2008).PRBMDO1098-012110.1103/PhysRevB.78.195424]. Here we find a new type of anticommutative magnetoelectric response ß^{ξ}(ω), which can induce a dynamical magnetoelectric current driven by a time-varying magnetic field. Unlike the Chern-Simons axion term, this magnetoelectric response term is gauge independent and nonquantized, and manifests in the systems breaking the symmetries of the time reversal, inversion, and mirror. In particular, we propose the antiferromagnetic material Mn_{2}Bi_{2}Te_{5} as a material candidate to observe dynamical magnetoelectric current, in which a large magnetoelectric response term ß^{ξ}(ω) originates from band inversion.
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Spin superconductor (SSC) is an exciton condensate state where the spin-triplet exciton superfluidity is charge neutral while spin 2(â/2). In analogy to the Majorana zero mode (MZM) in topological superconductors, the interplay between SSC and band topology will also give rise to a specific kind of topological bound state obeying non-Abelian braiding statistics. Remarkably, the non-Abelian geometric phase here originates from the Aharonov-Casher effect of the "half-charge" other than the Aharonov-Bohm effect. Such topological bound state of SSC is bound with the vortex of electric flux gradient and can be experimentally more distinct than the MZM for being electrically charged. This theoretical proposal provides a new avenue investigating the non-Abelian braiding physics without the assistance of MZM and charge superconductor.
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Recently, a half-quantized Hall conductance (HQHC) plateau was experimentally observed in a semimagnetic topological insulator heterostructure. However, the heterostructure was metallic with a nonzero longitudinal conductance, which contradicts the common belief that quantized Hall conductance is usually observed in insulators. In this work, we systematically study the surface transport of a semimagnetic topological insulator with both gapped and gapless Dirac surfaces in the presence of dephasing process. In particular, we reveal that the HQHC is directly related to the half-quantized chiral current along the edge of a strongly dephasing metal. The Hall conductance keeps a half-quantized value for large dephasing strengths, while the longitudinal conductance varies with Fermi energies and dephasing strengths. Furthermore, we evaluate both the conductance and resistance as a function of the temperature, which is consistent with the experimental results. Our results not only provide the microscopic transport mechanism of the HQHC, but also are instructive for the probe of the HQHC in future experiments.
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Recently, the search for an axion insulator state in the ferromagnetic-3D topological insulator (TI) heterostructure and MnBi_{2}Te_{4} has attracted intense interest. However, its detection remains difficult in experiments. We systematically investigate the disorder-induced phase transition of the axion insulator state in a 3D TI with antiparallel magnetization alignment surfaces. It is found that there exists a 2D disorder-induced phase transition on the surfaces of the 3D TI which shares the same universality class with the quantum Hall plateau to plateau transition. Then, we provide a phenomenological theory which maps the random mass Dirac Hamiltonian of the axion insulator state into the Chalker-Coddington network model. Therefore, we propose probing the axion insulator state by investigating the universal signature of such a phase transition in the ferromagnetic-3D TI heterostructure and MnBi_{2}Te_{4}. Our findings not only show a global phase diagram of the axion insulator state, but also stimulate further experiments to probe it.
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Metal-insulator transitions driven by magnetic fields have been extensively studied in 2D, but a 3D theory is still lacking. Motivated by recent experiments, we develop a scaling theory for the metal-insulator transitions in the strong-magnetic-field quantum limit of a 3D system. By using a renormalization-group calculation to treat electron-electron interactions, electron-phonon interactions, and disorder on the same footing, we obtain the critical exponent that characterizes the scaling relations of the resistivity to temperature and magnetic field. By comparing the critical exponent with those in a recent experiment [F. Tang et al., Nature (London) 569, 537 (2019)NATUAS0028-083610.1038/s41586-019-1180-9], we conclude that the insulating ground state was not only a charge-density wave driven by electron-phonon interactions but also coexisting with strong electron-electron interactions and backscattering disorder. We also propose a current-scaling experiment for further verification. Our theory will be helpful for exploring the emergent territory of 3D metal-insulator transitions under strong magnetic fields.
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In most cases, to observe quantized Hall plateaus, an external magnetic field is applied in intrinsic magnetic topological insulators MnBi_{2}Te_{4}. Nevertheless, whether the nonzero Chern number (C≠0) phase is a quantum anomalous Hall (QAH) state, or a quantum Hall (QH) state, or a mixing state of both is still a puzzle, especially for the recently observed C=2 phase [Deng et al., Science 367, 895 (2020)SCIEAS0036-807510.1126/science.aax8156]. In this Letter, we propose a physical picture based on the Anderson localization to understand the observed Hall plateaus in disordered MnBi_{2}Te_{4}. Rather good consistency between the experimental and numerical results confirms that the bulk states are localized in the absence of a magnetic field and a QAH edge state emerges with C=1. However, under a strong magnetic field, the lowest Landau band formed with the localized bulk states, survives disorder, together with the QAH edge state, leading to a C=2 phase. Eventually, we present a phase diagram of a disordered MnBi_{2}Te_{4} which indicates more coexistence states of QAH and QH to be verified by future experiments.
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Topological insulators (TIs) are an exciting discovery because of their robustness against disorder and interactions. Recently, second-order TIs have been attracting increasing attention, because they host topologically protected 1D hinge states in 3D or 0D corner states in 2D. A significantly critical issue is whether the second-order TIs also survive interactions, but it is still unexplored. We study the effects of weak Coulomb interactions on a 3D second-order TI, with the help of renormalization-group calculations. We find that the 3D second-order TIs are always unstable, suffering from two types of topological phase transitions. One is from second-order TI to TI, the other is to normal insulator. The first type is accompanied by emergent time-reversal and inversion symmetries and has a dynamical critical exponent κ=1. The second type does not have the emergent symmetries but has nonuniversal dynamical critical exponents κ<1. Our results may inspire more inspections on the stability of higher-order topological states of matter and related novel quantum criticalities.
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Recently, higher-order topological matter and 3D quantum Hall effects have attracted a great amount of attention. The Fermi-arc mechanism of the 3D quantum Hall effect proposed to exist in Weyl semimetals is characterized by the one-sided hinge states, which do not exist in all the previous quantum Hall systems, and more importantly, pose a realistic example of the higher-order topological matter. The experimental effort so far is in the Dirac semimetal Cd_{3}As_{2}, where, however, time-reversal symmetry leads to hinge states on both sides of the top and bottom surfaces, instead of the aspired one-sided hinge states. We propose that under a tilted magnetic field, the hinge states in Cd_{3}As_{2}-like Dirac semimetals can be one sided, highly tunable by field direction and Fermi energy, and robust against weak disorder. Furthermore, we propose a scanning tunneling Hall measurement to detect the one-sided hinge states. Our results will be insightful for exploring not only the quantum Hall effects beyond two dimensions, but also other higher-order topological insulators in the future.
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Quantum Griffiths singularity (QGS) reveals the profound influence of quenched disorder on the quantum phase transitions, characterized by the divergence of the dynamical critical exponent at the boundary of the vortex glasslike phase, named as quantum Griffiths phase. However, in the absence of vortices, whether the QGS can exist under a parallel magnetic field remains a puzzle. Here, we study the magnetic field induced superconductor-metal transition in ultrathin crystalline PdTe_{2} films grown by molecular beam epitaxy. Remarkably, the QGS emerges under both perpendicular and parallel magnetic field in four-monolayer PdTe_{2} films. The direct activated scaling analysis with a new irrelevant correction has been proposed, providing important evidence of QGS. With increasing film thickness to six monolayers, the QGS disappears under perpendicular field but persists under parallel field, and this discordance may originate from the differences in microscopic processes. Our work demonstrates the universality of parallel field induced QGS and can stimulate further investigations on novel quantum phase transitions under parallel magnetic field.
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We investigate the 3D quantum Hall effect in Weyl semimetals and elucidate a global picture of the edge states. The edge states hosting 3D quantum Hall effect are combinations of Fermi arcs and chiral Landau bands dispersing along the magnetic field direction. The Hall conductance, σ_{xz}^{H} [see Fig. 4], shows quantized plateaus with the variance of the magnetic field when the Fermi level is at the Weyl node. However, the chiral Landau bands can change the spatial distribution of the edge states, especially under a tilted magnetic field, and the resulting edge states lead to distinctive Hall transport phenomena. A tilted magnetic field contributes an intrinsic value to σ_{xz}^{H} and such an intrinsic value is determined by the tilting angle θ between the magnetic field and the y axis [see Fig. 1(c)]. Particularly, even if the perpendicular magnetic field is fixed, σ_{xz}^{H} will change its sign with an abrupt spatial shift of the edge states when θ exceeds a critical angle θ_{c}. Our work uncovers the novel edge-state nature of the 3D quantum Hall effect in Weyl semimetals.
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We numerically demonstrate that the topological corner states residing in the corners of higher-order topological insulator possess non-Abelian braiding properties. Such topological corner states are Dirac fermionic modes other than Majorana zero modes. We claim that Dirac fermionic modes protected by nontrivial topology also support non-Abelian braiding. An analytical description on such non-Abelian braiding is conducted based on the vortex-induced Dirac-type fermionic modes. Finally, the braiding operators for Dirac fermionic modes, especially their explicit matrix forms, are analytically derived and compared with the case of Majorana zero modes.
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The charge-density-wave (CDW) mechanism of the 3D quantum Hall effect has been observed recently in ZrTe_{5} [Tang et al., Nature 569, 537 (2019)10.1038/s41586-019-1180-9]. Different from previous cases, the CDW forms on a one-dimensional (1D) band of Landau levels, which strongly depends on the magnetic field. However, its theory is still lacking. We develop a theory for the CDW mechanism of 3D quantum Hall effect. The theory can capture the main features in the experiments. We find a magnetic field induced second-order phase transition to the CDW phase. We find that electron-phonon interactions, rather than electron-electron interactions, dominate the order parameter. We extract the electron-phonon coupling constant from the non-Ohmic I-V relation. We point out a commensurate-incommensurate CDW crossover in the experiment. More importantly, our theory explores a rare case, in which a magnetic field can induce an order-parameter phase transition in one direction but a topological phase transition in other two directions, both depend on one magnetic field.
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Recently, a zero Hall conductance plateau with random domains was experimentally observed in the quantum anomalous Hall (QAH) effect. We study the effects of random domains on the zero Hall plateau in QAH insulators. We find that the structure inversion symmetry determines the scaling property of the zero Hall plateau transition in the QAH systems. In the presence of structure inversion symmetry, the zero Hall plateau state shows a quantum-Hall-type critical point, originating from the two decoupled subsystems with opposite Chern numbers. However, the absence of structure inversion symmetry leads to a mixture between these two subsystems, gives rise to a line of critical points, and dramatically changes the scaling behavior. Hereinto, we predict a Berezinskii-Kosterlitz-Thouless-type transition during the Hall conductance plateau switching in the QAH insulators. Our results are instructive for both theoretic understanding of the zero Hall plateau transition and future transport experiments in the QAH insulators.
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The Majorana zero mode in the semiconductor-superconductor nanowire is one of the promising candidates for topological quantum computing. Recently, in islands of nanowires, subgap-state energies have been experimentally observed to oscillate as a function of the magnetic field, showing a signature of overlapped Majorana bound states. However, the oscillation amplitude either dies away after an overshoot or decays, sharply opposite to the theoretically predicted enhanced oscillations for Majorana bound states. We reveal that a steplike distribution of spin-orbit coupling in realistic devices can induce the decaying Majorana oscillations, resulting from the coupling-induced energy repulsion between the quasiparticle spectra on the two sides of the step. This steplike spin-orbit coupling can also lead to decaying oscillations in the spectrum of the Andreev bound states. For Coulomb-blockade peaks mediated by the Majorana bound states, the peak spacings have been predicted to correlate with peak heights by a π/2 phase shift, which was ambiguous in recent experiments and may be explained by the steplike spin-orbit coupling. Our work will inspire more works to reexamine effects of the nonuniform spin-orbit coupling, which is generally present in experimental devices.
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Identifying topological insulators and semimetals often focuses on their surface states, using spectroscopic methods such as angle-resolved photoemission spectroscopy or scanning tunneling microscopy. In contrast, studying the topological properties of topological insulators from their bulk-state transport is more accessible in most labs but seldom addressed. We show that, in the quantum limit of a topological insulator, the backscattering between the only two states on the Fermi surface of the lowest Landau band can be forbidden at a critical magnetic field. The conductivity is determined solely by the backscattering between the two states, leading to a resistance dip that may serve as a signature for topological insulator phases. More importantly, this forbidden backscattering mechanism for the resistance dip is irrelevant to details of disorder scattering. Our theory can be applied to revisit the experiments on Pb_{1-x}Sn_{x}Se, ZrTe_{5}, and Ag_{2}Te families, and will be particularly useful for controversial small-gap materials at the boundary between topological and normal insulators.
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Valley polarized topological kink states, existing broadly in the domain wall of hexagonal lattice systems, are identified in experiments. Unfortunately, only very limited physical properties are given. Using an Aharanov-Bohm interferometer composed of domain walls in graphene systems, we study the periodical modulation of a pure valley current in a large range by tuning the magnetic field or the Fermi level. For a monolayer graphene device, there exists one topological kink state, and the oscillation of the transmission coefficients has a single period. The π Berry phase and the linear dispersion relation of kink states can be extracted from the transmission data. For a bilayer graphene device, there are two topological kink states with two oscillation periods. Our proposal provides an experimentally feasible route to manipulate and characterize the valley-polarized topological kink states in classical wave and electronic graphene-type crystalline systems.