Deep-learning assisted fast orbital angular momentum complex spectrum analysis.

Analyzing the orbital angular momentum (OAM) distribution of a vortex beam is critical for OAM-based applications. Here, we propose a deep residual network (DRN) to model the relationship between characteristics of the multiplexed OAM beam and their complex spectrum. The favorable experimental results show that our proposal can obtain both the intensity and phase terms of multiplexed OAM beams, dubbed complex spectrum, with a wide range of OAM modes, varying in intensity, phase ratio, and mode intervals at high accuracy and real-time speed. Specifically, the root mean square error (RMSE) of intensity and phase spectrum is evaluated as 0.002 and 0.016, respectively, with a response time of only 0.020 s. To the best of our knowledge, this work opens a new sight for fast OAM complex spectrum analysis and paves the way for numerous advanced domains that need real-time OAM complex spectrum diagnostic like ultrahigh-dimensional OAM tailoring.

Single-frequency orbital angular momentum switchable modes from a microchip laser.

We demonstrate the direct generation of single-frequency switchable orbital angular momentum (OAM) modes in a 1 µm wavelength range using a Nd:YVO4 microchip laser. The 808 nm laser diode pump beam is shaped into annular through an axicon associated with a lens. By adjusting the diameter and power of the annular pump beam, various OAM modes with different mode volumes can oscillate inside the Nd:YVO4 microchip. Moreover, a single-frequency output is also available due to the short cavity of the microchip. In the proof-of-principle experiment, single-frequency twofold multiplexed OAM modes | ± 1> and | ± 2> are generated, with experimentally measured fidelity higher than 96%. This work presents a compact and versatile single-frequency OAM source and will inspire multiple advanced scenarios ranging from classical to quantum photonics.

Thermally activated delayed fluorescence materials for organic light-emitting diodes.

Recently, the remarkable advances in thermally activated delayed fluorescence (TADF) materials have attracted much attention due to their 100% exciton utilization efficiency in organic light-emitting diodes (OLEDs). Although the commercialization of TADF materials is at an early stage, they exhibit enormous potential for next-generation OLEDs due to the comparable electroluminescence performance to metal of their phosphorescent complex counterparts, but without the presence of precious metal elements. This review summarizes the different types of TADF small molecules with various photophysical properties and the state-of-the-art molecular design strategies. Furthermore, the device engineering is discussed, and emerging optoelectronic applications, such as organic light-emitting electrochemical cells, organic lasing, and organic scintillators, are introduced. It is anticipated that this review can clarify the design of efficient TADF emitters and point out the direction of future development.

Power amplification for 1.6†µm high-order vortex modes.

1.6 µm high-order vortex modes carrying orbital angular momentums (OAMs) play significant roles in long-range Doppler lidars and other remote sensing. Amplification of 1.6 µm high-order vortex modes is an important way to provide high-power laser sources for such lidars and also enable the weak echo signal to be amplified so that it can be analyzed. In this work, we propose a four-pass Er:YAG vortex master-oscillator-power-amplification (MOPA) system to amplify 1.6 µm high-order vortex modes. In the proof-of-concept experiments, 1.6 µm single OAM mode (l = 3) is amplified successfully and the gain ranging from 1.88 to 2.36 is achieved. Multiplexed OAM mode (l=±3) is also amplified with favorable results. This work addresses the issue as the low gain of Er:YAG vortex MOPA, which provides a feasible path for 1.6 µm high-order vortex modes amplification.

1645-nm single-frequency vortex laser from an Er:YAG nonplanar ring oscillator.

A 1645-nm single-frequency vortex beam with narrow linewidth from an Er:YAG nonplanar ring oscillator (NPRO) using an annular pump beam is demonstrated. The pump beam from a 1532-nm fiber laser is shaped to an annular beam by an axicon. The Er:YAG NPRO generates a 1.96-W single-frequency vortex beam under a pump power of 13 W. The linewidth of the 1645-nm vortex laser is measured as 6 kHz. This work provides a convenient way of single-frequency vortex beam generation.

Multiplexed vortex state array toward high-dimensional data multicasting.

Optical vortex array has drawn widespread attention since the boom of special applications such as molecular selecting and optical communication. Here, we propose an integrated phase-only scheme to generate multiple multiplexed vortex beams simultaneously, constituting a multiplexed vortex state array, where the spatial position, as well as the corresponding orbital angular momentum (OAM) spectrum, can be manipulated flexibly as desired. Proof-of-concept experiments are carried out and show a few different multiplexed vortex state arrays that fit well with the simulation. Moreover, regarding the array as a data-carrier, a one-to-many multicasting link through multi-state OAM shift keying, a high-dimensional data coding, is also available in free space. In the experiment, four various OAM states are employed and achieve four bits binary symbols, and finally distribute three different images to three separate receivers independently from the same transmitter, showing great potential in the future high-dimensional optical networks.

Sorting orbital angular momentum of photons through a multi-ring azimuthal-quadratic phase.

Beams carrying orbital angular momentum (OAM) already play significant roles in many domains. Here we propose a practical design of an OAM beam splitter based on a single phase-only multi-ring azimuthal-quadratic diffraction optical element that can sort different OAM components into various spatial positions, and OAM state probing is also achieved. The performance is demonstrated through proof-of-principle experiments and shows favorable results. Furthermore, the intensity proportion of each OAM component, namely the OAM spectrum, is also diagnosed. This work offers high applicability and practicability for the recognition and separation of photon OAM, and thus paves the way for many advanced scenarios such as quantum communication, holographic encryption, and remote sensing.

Adjusted EfficientNet for the diagnostic of orbital angular momentum spectrum.

Orbital angular momentum (OAM) is one of multiple dimensions of beams. A beam can carry multiple OAM components, and their intensity weights form the OAM spectrum. The OAM spectrum determines complex amplitude distributions of a beam and features unique characteristics. Thus, measuring the OAM spectrum is of great significance, especially for OAM-based applications. Here we employ a deep neural network combined with a phase-only diffraction optical element to measure the OAM spectrum. The diffraction optical element is designed to diffract incident beams into distinct patterns corresponding to OAM distributions. Then, the EfficientNet, a kind of deep neural network, is adjusted to adapt and analyze the diffraction pattern to calculate the OAM spectrum. The favorable experimental results show that our proposal can reconstruct the OAM spectra with high precision and speed, works well for different numbers of OAM channels, and is also robust to Gaussian noise and random zooming. This work opens a new, to the best of our knowledge, ability for OAM spectrum recognition and will find applications in a number of advanced domains including large capacity optical communications, quantum key distribution, optical trapping, rotation detection, and so on.

Tailoring a complex perfect optical vortex array with multiple selective degrees of freedom.

Optical vortex arrays (OVAs) have successfully aroused substantial interest from researchers for their promising prospects ranging from classical to quantum physics. Previous reported OVAs still show a lack of controllable dimensions which may hamper their applications. Taking an isolated perfect optical vortex (POV) as an array element, whose diameter is independent of its topological charge (TC), this paper proposes combined phase-only holograms to produce sophisticated POV arrays. The contributed scheme enables dynamically controllable multi-ring, TC, eccentricity, size, and the number of optical vortices (OVs). Apart from traditional single ring POV element, we set up a ßg library to obtain optimized double ring POV element. With multiple selective degrees of freedom to be chosen, a series of POV arrays are generated which not only elucidate versatility of the method but also unravel analytical relationships between the set parameters and intensity patterns. More exotic structures are formed like the "Bear POV" to manifest the potential of this approach in tailoring customized structure beams. The experimental results show robust firmness with the theoretical simulations. As yet, these arrays make their public debut so far as we know, and will find miscellaneous applications especially in multi-microparticle trapping, large-capacity optical communications, novel pumping lasers and so on.

Turbulence aberration correction for vector vortex beams using deep neural networks on experimental data.

The vector vortex beams (VVB) possessing non-separable states of light, in which polarization and orbital angular momentum (OAM) are coupled, have attracted more and more attentions in science and technology, due to the unique nature of the light field. However, atmospheric transmission distortion is a recurring challenge hampering the practical application, such as communication and imaging. In this work, we built a deep learning based adaptive optics system to compensate the turbulence aberrations of the vector vortex mode in terms of phase distribution and mode purity. A turbulence aberration correction convolutional neural network (TACCNN) model, which can learn the mapping relationship of intensity profile of the distorted vector vortex modes and the turbulence phase generated by first 20 Zernike modes, is well designed. After supervised learning plentiful experimental samples, the TACCNN model compensates turbulence aberration for VVB quickly and accurately. For the first time, experimental results show that through correction, the mode purity of the distorted VVB improves from 19% to 70% under the turbulence strength of D/r0 = 5.28 with correction time 100 ms. Furthermore, both spatial modes and the light intensity distribution can be well compensated in different atmospheric turbulence.

Generating a 64 × 64 beam lattice by geometric phase modulation from arbitrary incident polarizations.

A laser beam lattice from tailoring spatial dimensions of lights is a kind of structured optical field, which already have found many applications in lots of domains. Here we propose a geometric phase element made from polymerized liquid crystals to transform Gaussian beams into a 64×64 beam lattice with high performance. Different from other geometric phase elements, the proposed element can introduce identical phase modulations for any polarizations, indicating that the beam lattice could be well generated with arbitrary incident homogeneous polarizations but not limited to specific circular polarizations. In the experiment, a 64×64 beam lattice is well generated. It is estimated that the uniformity of the obtained lattice fluctuates about 60% among various incident polarizations, which is very close to the prediction. This work opens a new site for producing high-dimensional beam lattices and will inspire more advanced applications.

Resonantly pumped Er:YAG vector laser with selective polarization states at 1.6 µm.

A resonantly pumped Er:YAG vector laser emitting at 1645 nm with selective polarization states is demonstrated. A compact five-mirror resonator incorporated a pair of quarter-wave plates (QWPs), and a pair of q-plates (QPs) is employed. Cylindrical vector beams of all states on a single high-order Poincaré sphere could be obtained by rotating the QWPs and QPs relatively.

Detection of angular acceleration based on optical rotational Doppler effect.

The angular acceleration of a spinning object can be estimated by probing the object with Laguerre-Gauss (LG) beams and analyzing the rotational Doppler frequency shift of returned signals. The frequency shift is time dependent because of the change of the rotational angular velocity over time. The detection system is built to collect the beating signals of LG beams back-scattered from a non-uniform spinning body. Then a time-frequency analysis method is proposed to study the evolution of the angular velocity in time. The experimental results of different angular accelerations of the rotator are consistent with expectations. The measurement errors of different probe beams with various topological charges from l = ± 10 to l = ± 100 are also investigated.

Experimental demonstration of free-space multi-state orbital angular momentum shift keying.

Orbital angular momentum (OAM), a new dimension of photons, has potentials in lots of domains as high-dimensional data coding/decoding. Here we experimentally demonstrate a free-space data transmission system based on 8 bits multi-state OAM shift keying, where multiplexed optical vortices containing 8 various OAM states are employed to constitute 8 bits binary symbols. In the transmitter, the data coding of OAM shift keying is realized by switching a series of special-designed holograms. And in the receiver, the decoding is done by a single Dammann vortex grating along with image processing. We experimentally transmit data, including a gray-scale image, in free-space for 10 meters, showing zero bit-error-rate. The demonstrated results indicate a wide prospect for the future high-dimensional large data rate optical security communications.

Demonstration of free-space one-to-many multicasting link from orbital angular momentum encoding.

Multicasting is necessary when distributing signals between multiple users. In this Letter, we demonstrate an orbital angular momentum (OAM) encoding-based free-space one-to-many multicasting link, where digital signals are encoded into a series of time-varying OAM states and transmitted from one transmitter to multiple receivers with various locations. Moreover, encoding N various signals simultaneously in one transmitter and sending them at the same time to N various receivers separately, is also demonstrated. As a proof-of-concept, four different gray images are coded by one transmitter simultaneously and multicast to four various receivers separately. The favorable decoding results returned by the four receivers show good multicasting performance.

Novel Class of Ultrasound-Triggerable Drug Delivery Systems for the Improved Treatment of Tumors.

The controlled release of anticancer drugs at the tumor site is a central challenge in treating cancer. To achieve this goal, our strategy was based on tumor-specific targeting and ultrasound-triggered release of an anticancer agent from liposomal nanocarriers. To enhance the ultrasound-triggered drug release, we incorporated a lipophilic sonosensitizer, chlorin e6 (Ce6) ester, into the lipid bilayer of liposomes. Additionally, asparagine-glycine-arginine (NGR) that binds to CD13, which is overexpressed in tumor cells, was introduced into these liposomes. Under the navigation effects of the NGR, the novel ultrasound-triggerable NGR-modified liposomal nanocarrier (NGR/UT-L) accumulates in tumor sites. Once irradiated by ultrasound in tumor tissues, the sonodynamic effect produced by Ce6 could create more efficient disruptions of the lipid bilayer of the liposomal nanocarriers. After encapsulating doxorubicin (DOX) as the model drug, the ultrasound triggered lipid bilayer breakdown can spring the immediate release of DOX, making it possible for ultrasound-responsive chemotherapy with great selectivity. By combining tumor-specific targeting and stimuli-responsive controlled release into one system, NGR/UT-L demonstrated a perfect antitumor effect. Moreover, this report provides an example of controlled-release by means of a novel class of ultrasound triggering systems.

Orbital angular momentum channel monitoring of coaxially multiplexed vortices by diffraction pattern analysis.

We theoretically and experimentally demonstrate a scheme to monitor the weight of a single orbital angular momentum (OAM) channel for coaxial multiplexed optical vortices with large mode spacing. A specially designed holographic grating is illuminated by the incident multiplexed vortices first. Then the weight of each single OAM channel is obtained after analyzing the captured diffraction patterns. This work will find applications in domains where multiplexed optical vortices are of interest, such as the OAM-based data-transmission system, and so on.

Non-diffractive Bessel-Gauss beams for the detection of rotating object free of obstructions.

Bessel-Gauss beams carrying orbital angular momentum are widely known for their non-diffractive or self-reconstructing performance, and have been applied in lots of domains. Here we demonstrate that, by illuminating a rotating object with high-order Bessel-Gauss beams, a frequency shift proportional to the rotating speed and the topological charge is observed. Moreover, the frequency shift is still present once an obstacle exists in the path, in spite of the decreasing of received signals. Our work indicates the feasibility of detecting rotating objects free of obstructions, and has potential as obstruction-immune rotation sensors in engine monitoring, aerological sounding, and so on.

Generation of perfect polarization vortices using combined gratings in a single spatial light modulator.

Perfect polarization vortices (PPVs) are a type of vector beam with a diameter independent of the polarization order. In this paper, an experimental method is proposed to generate PPVs with an anisotropic polarization distribution. First, a specially designed hologram is generated on a liquid-crystal spatial light modulator (SLM) to obtain Bessel-Gaussian (BG) beams. Second, the BG beams are transformed into PPVs in the Bessel region by an interferometer, which includes a polarized beam splitter, two reflectors, and several lenses. In our experiment, PPVs with adjustable polarization orders and diameters are obtained by generating various combined holograms on the SLM.

Measurement of orbital angular momentum spectra of multiplexing optical vortices.

Optical vortex beams carrying orbital angular momentum (OAM) are widely investigated for their unique performance in recent years. They can be used to extend the capacity of optical communications system due to the orthogonality of different channels. In the receiver side of a multiplexing optical vortices system, verifying the OAM spectrum is of great importance. A new kind of diffraction element called Dammann vortex grating can distribute energies among different diffraction orders equally. Based on this unique characteristic, we reported a new algorithm to analyze the spot of each diffraction order. The OAM spectrum in the receiver side can then be obtained. In the experiment, the OAM spectrum measurement of at most six-channel multiplexing optical vortices is realized. The experimental results illustrate that the OAM spectrum gained by this approach is highly consistent with the theoretical value.