Observation of Monoenergetic Electrons from Two-Pulse Ionization Injection in Quasilinear Laser Wakefields.

The generation of low emittance electron beams from laser-driven wakefields is crucial for the development of compact x-ray sources. Here, we show new results for the injection and acceleration of quasimonoenergetic electron beams in low amplitude wakefields experimentally and using simulations. This is achieved by using two laser pulses decoupling the wakefield generation from the electron trapping via ionization injection. The injection duration, which affects the beam charge and energy spread, is found to be tunable by adjusting the relative pulse delay. By changing the polarization of the injector pulse, reducing the ionization volume, the electron spectra of the accelerated electron bunches are improved.

Iterative wavefront optimization of ultrafast laser beams carrying orbital angular momentum.

Structured intense laser beams offer degrees of freedom that are highly attractive for high-field science applications. However, the performance of high-power laser beams in these applications is often hindered by deviations from the desired spatiotemporal profile. This study reports the wavefront optimization of ultrafast Laguerre-Gaussian beams through the synergy of adaptive optics and genetic algorithm-guided feedback. The results indicate that the intensity fluctuations along the perimeter of the target ring-shaped profile can be reduced up to ∼15%. Furthermore, the radius of the ring beam profile can be tailored to a certain extent by establishing threshold fitting criteria. The versatility of this approach is experimentally demonstrated in conjunction with different focusing geometries.

Ultra-broadband long-wave-infrared pulse production using a chirped-pulse difference-frequency generation.

We present a broadband light source based on near-infrared chirped-pulse difference-frequency mixing that is suitable for seeding long-wave-infrared (LWIR) optical parametric chirped-pulse amplification (OPCPA). A nitrocellulose pellicle is used in a Ti:sapphire regenerative amplifier to generate dual-frequency output pulses, which are subsequently mixed in a 0.4-mm thick AgGaS2 crystal. LWIR pulses with ∼1 µm full width at half maximum (FWHM) bandwidth centered at 10.5 µm are generated by mixing transform-limited pulses. Assisted by genetic algorithm optimization, the bandwidth is broadened to ∼3 µm FWHM within the 8-12 µm atmospheric transmission window. The seed source paves the path towards tabletop ultrafast terawatt-class passively carrier-envelope-phase stabilized OPCPA in the LWIR region.

Single-shot, double-pulse determination of the detonation energy in nanosecond-laser ablation using the blast model.

We demonstrate a novel single-shot method to determine the detonation energy of laser-induced plasma and investigate its performance. This approach can be used in cases where there are significant shot-to-shot variations in ablation conditions, such as laser fluctuations, target inhomogeneity, or multiple filamentation with ultrashort pulses. The Sedov blast model is used to fit two time-delayed shadowgrams measured with a double-pulse laser. We find that the reconstruction of detonation parameters is insensitive to the choice of interpulse delay in double-pulse shadowgraphy. In contrast, the initial assumption of expansion dimensionality has a large impact on the reconstructed detonation energy. The method allows for a reduction in the uncertainties of blast wave energy measurements as a diagnostic technique employed in various laser ablation applications.

High-energy nanosecond parametric source at 2.7 µm.

We report a high-energy nanosecond KTiOAsO4-based optical parametric oscillator and amplifier system driven by a 1064-nm, injection-seeded, Q-switched Nd:YAG laser to provide mid-infrared pumping for few-cycle optical parametric chirped-pulse amplification operating in the long-wave infrared spectral regime. An output energy of 10.5 mJ at 2726 nm was obtained from the final power amplifier with a spectral width of 2.8 nm, pulse duration of 1.2 ns, and M2 value of 2.4. The parametric source provides for the second mode of operation, where 10-ns pulses are produced by disabling the electro-optic slicing that enables the 1-ns mode. For 10-ns operation, the source produced energy of 25 mJ with a M2 value of 2.8.

Polarization-Dependent Self-Injection by Above Threshold Ionization Heating in a Laser Wakefield Accelerator.

We report on the experimental observation of a decreased self-injection threshold by using laser pulses with circular polarization in laser wakefield acceleration experiments in a nonpreformed plasma, compared to the usually employed linear polarization. A significantly higher electron beam charge was also observed for circular polarization compared to linear polarization over a wide range of parameters. Theoretical analysis and quasi-3D particle-in-cell simulations reveal that the self-injection and hence the laser wakefield acceleration is polarization dependent and indicate a different injection mechanism for circularly polarized laser pulses, originating from larger momentum gain by electrons during above threshold ionization. This enables electrons to meet the trapping condition more easily, and the resulting higher plasma temperature was confirmed via spectroscopy of the XUV plasma emission.

Adaptive control of laser-wakefield accelerators driven by mid-IR laser pulses.

There has been growing interest both in studying high intensity ultrafast laser plasma interactions with adaptive control systems as well as using long wavelength driver beams. We demonstrate the coherent control of the dynamics of laser-wakefield acceleration driven by ultrashort (∼ 100 fs) mid-infrared (∼ 3.9 µm) laser pulses. The critical density at this wavelength is 7.3 × 1019 cm-3, which is achievable with an ordinary gas target system. Interactions between mid-infrared laser pulses and such near-critical-density plasma may be beneficial due to much higher absorption of laser energy. In addition, the normalized vector potential of the laser field a0 increases with longer laser wavelength, lowering the required peak laser intensity to drive non-linear laser-wakefield acceleration. Here, MeV level, collimated electron beams with non-thermal, peaked energy spectra are generated. Optimization of electron beam qualities are realized through adaptive control of the laser wavefront. A genetic algorithm controlling a deformable mirror improves the electron total charge, energy spectra, beam pointing and stability at various plasma density profiles. Particle-in-cell simulations reveal that the optimal wavefront causes an earlier injection on the density up-ramp and thus higher energy gain as well as less filamentation during the interaction, which leads to the improvement in electron beam collimation and energy spectra.

Optical emission from ultrafast laser filament-produced air plasmas in the multiple filament regime.

We perform optical emission spectroscopy of ultrafast laser filament-produced air plasmas in the multiple filament regime at driving wavelengths of 400 nm and 800 nm. The spatiotemporal structure of the emission from the plasmas are observed and the emission spectra are used to estimate plasma temperature and density for a range of laser parameters. Plasma temperatures are determined from the molecular nitrogen fluorescence, while the electron densities are estimated from Stark broadening of the oxygen-I 777.19-nm line. Electron temperatures are determined to be in the range of 5000-5200 K and they do not vary significantly along the length of the filament, nor are they sensitive to incident laser energy or wavelength. Electron densities are on order of 1016 cm-3 and show a greater variation with axial position, laser energy, and laser wavelength. We discuss mechanisms responsible for spatial localization of emitting species within the filament. Optical emission spectroscopy offers a simple, non-perturbing method to measure filament properties, that allows the information on the associated molecular transitions and excitation/ionization mechanisms to be extracted.

Intense laser filament-solid interactions from near-ultraviolet to mid-infrared.

Studies of high-power ultrashort laser pulse interaction with matter are not only of fundamental scientific interest, but are also highly relevant to applications in the domain of remote sensing. Here, we investigate the effect of laser wavelength on coupling of femtosecond laser filaments to solid targets. Three central wavelengths have been used to produce filaments: 0.4, 0.8, and 2.0 µm. We find that, unlike the case of conventional tight focusing, use of shorter wavelengths does not necessarily produce more efficient ablation. This is explained by increased multi-photon absorption arising in near-UV filamentation. Investigations of filament-induced plasma dynamics and its thermodynamic parameters provide the foundation for unveiling the interplay between wavelength-dependent filament ablation mechanisms. In this way, strategies to increase the sensitivity of material detection via this technique may be better understood, thereby improving the analytical performance in this class of applications.

Electrical conductance of near-infrared femtosecond air filaments in the multi-filament regime.

Electrical conductive properties of femtosecond laser filaments are of significant interest for applications such as remote arc suppression and discharge guiding. We transmitted electrical current through a DC-biased air plasma channel formed in the wake of an energetic femtosecond laser pulse and observed an increased rate of change of the charge transmitted through the ionized channel with laser energy when crossing from the single- to multi-filament regimes. This behavior is attributed to the confluent effects of greater electron density and an increased cross-sectional area of the multi-filament plasma structures. As the laser energy is increased, the formation of additional conductive channels in the multi-filamentation regime becomes a significant contributor to the rapid increase of conductivity. These observations suggest a potential path to attractive applications such as efficient energy transfer in air mediated by femtosecond laser-produced filaments.

Enhancement of THz generation by feedback-optimized wavefront manipulation.

We apply active feedback optimization methods to pyroelectric measurements of a THz signal generated by four wave mixing in air using 1 mJ to 12 mJ, 35 fs laser pulses operating at 12 kHz repetition rate. A genetic algorithm, using the THz signal as a figure of merit, determines the voltage settings to a deformable mirror and results in up to a 6 fold improvement in the THz signal compared with settings optimized for the best focus. It is possible to optimize for different THz generation processes using this technique.

High-Flux Femtosecond X-Ray Emission from Controlled Generation of Annular Electron Beams in a Laser Wakefield Accelerator.

Annular quasimonoenergetic electron beams with a mean energy in the range 200-400 MeV and charge on the order of several picocoulombs were generated in a laser wakefield accelerator and subsequently accelerated using a plasma afterburner in a two-stage gas cell. Generation of these beams is associated with injection occurring on the density down ramp between the stages. This well-localized injection produces a bunch of electrons performing coherent betatron oscillations in the wakefield, resulting in a significant increase in the x-ray yield. Annular electron distributions are detected in 40% of shots under optimal conditions. Simultaneous control of the pulse duration and frequency chirp enables optimization of both the energy and the energy spread of the annular beam and boosts the radiant energy per unit charge by almost an order of magnitude. These well-defined annular distributions of electrons are a promising source of high-brightness laser plasma-based x rays.

Ionization-induced self-compression of tightly focused femtosecond laser pulses.

As lasers become progressively higher in power, optical damage thresholds will become a limiting factor. Using the nonlinear optics of plasma may be a way to circumvent these limits. Here, we present a new self-compression mechanism for high-power, femtosecond laser pulses based on geometrical focusing and three dimensional spatiotemporal reshaping in an ionizing plasma. By propagating tightly focused, 10-mJ femtosecond laser pulses through a 100-µm gas jet, the interplay between ionization gradients, focusing, and diffraction of the light pulse leads to stable and uniform self-compression of the pulse, while maintaining a high-energy throughput and excellent refocusability. Self-compression down to 16 fs from an original 36-fs pulse is measured using second-harmonic-generation frequency-resolved optical gating. Using this mechanism, we are able to maintain a high transmission (>88%) such that the pulse peak power is doubled. Three-dimensional numerical simulations are performed to support our interpretation of the experimental observations.

Table-top laser-based source of femtosecond, collimated, ultrarelativistic positron beams.

The generation of ultrarelativistic positron beams with short duration (τ(e+) ≃ 30 fs), small divergence (θ(e+) ≃ 3 mrad), and high density (n(e+) ≃ 10(14)-10(15) cm(-3)) from a fully optical setup is reported. The detected positron beam propagates with a high-density electron beam and γ rays of similar spectral shape and peak energy, thus closely resembling the structure of an astrophysical leptonic jet. It is envisaged that this experimental evidence, besides the intrinsic relevance to laser-driven particle acceleration, may open the pathway for the small-scale study of astrophysical leptonic jets in the laboratory.

Compressor optimization with compressor-based multiphoton intrapulse interference phase scan (MIIPS).

The multiphoton intrapulse interference phase scan (MIIPS) technique is modified to optimize the compressor settings of a chirped pulse amplification (CPA) laser system. Here, we use the compressor itself to perform the phase scan inherent in MIIPS measurement . A frequency-resolved optical gating measurement shows that the pulse duration of the compressor optimized using the modified MIIPS technique is 33.8 fs with a 2.24 rad temporal phase variation above 2% intensity. The measured time-bandwidth product is 0.60, which is close to that of transform-limited Gaussian pulse (0.44).

Optimization of the electron beam dump for a GeV-class laser electron accelerator.

The advances of laser-driven electron acceleration offer the promise of great reductions in the size of high-energy electron accelerator facilities. Accordingly, it is desirable to design compact radiation shielding for such facilities. A key component of radiation shielding is the high-energy electron beam dump. In an effort to optimize the electron beam dump design, different material combinations have been simulated with the FLUKA Monte Carlo code in the range of 1-40 GeV. The studied beam dump configurations consist of alternating layers of high-Z material (lead or iron) and low-Z material (high-density concrete or borated polyethylene) in either three-layer or five-layer structures. The designs of various beam dump configuration have been compared and it has been found that the iron and concrete stacking in a three-layer structure with a thick iron layer results in the lowest dose at 1, 10, and 40 GeV. The performance of the beam dump exhibits a strong dependence on the selected materials, the stacking method, the beam dump thickness, as well as the electron energy. This parametric study provides general insights that can be used for compact shielding design of future electron accelerator facilities.

Multiple colliding electromagnetic pulses: a way to lower the threshold of e+ e- pair production from vacuum.

The scheme of a simultaneous multiple pulse focusing on one spot naturally arises from the structural features of projected new laser systems, such as the Extreme Light Infrastructure (ELI) and High Power laser Energy Research (HiPER). It is shown that the multiple pulse configuration is beneficial for observing e+ e- pair production from a vacuum under the action of sufficiently strong electromagnetic fields. The field of focused pulses is described using a realistic three-dimensional model based on an exact solution of the Maxwell equations. The e+ e- pair production threshold in terms of electromagnetic field energy can be substantially lowered if, instead of one or even two colliding pulses, multiple pulses are focused on one spot. The multiple pulse interaction geometry gives rise to subwavelength field features in the focal region. These features result in the production of extremely short e+ e- bunches.

Ultra-high intensity- 300-TW laser at 0.1 Hz repetition rate.

We demonstrate the highest intensity - 300 TW laser by developing booster amplifying stage to the 50-TW-Ti:sapphire laser (HERCULES). To our knowledge this is the first multi-100TW-scale laser at 0.1 Hz repetition rate.

Ultrafast Laser Filament-induced Fluorescence Spectroscopy of Uranyl Fluoride.

Uranyl fluoride (UO2F2) is a compound which forms in the reaction between water and uranium hexafluoride, a uranium containing gas widely used for uranium enrichment. Uranyl fluoride exhibits negligible natural background in atmosphere; as a result, its observation implies the presence and active operation of nearby enrichment facilities and could be used as a tracer for treaty verification technologies. Additionally, detection of UO2F2 has a potential application in guiding remediation efforts around enrichment facilities. Laser-induced fluorescence (LIF) has been proposed in the past as a viable technique for the detection and tracking of UO2F2. We demonstrate that ultrafast laser filamentation coupled with LIF extends the capabilities of standard LIF to enable remote detection of UO2F2. An intense femtosecond laser pulse propagated in air collapses into a plasma channel, referred to as a laser filament, allowing for the extended delivery of laser energy. We first investigate the luminescence of UO2F2 excited by the second harmonic of an ultrafast Ti:sapphire laser and subsequently excite it using the conical emission that accompanies ultrafast laser filamentation in air. We measure the decay rates spanning 4.3-5.6 × 104 s-1 and discuss the characteristics of the luminescence for both ultrafast- and filament-excitation. Larger decay rates than those observed using standard LIF are caused by a saturated component of prompt decay from annihilation of dense excited states upon excitation with an ultrafast source. The reproducibility of such decay rates for the given range of incident laser intensities 1.0-1.6 × 1011 W cm-2 is promising for the application of this technique in remote sensing.