Diffractive optical elements in single crystal diamond.

We demonstrate the design, fabrication, and experimental characterization of near-field binary phase transmission diffractive optical elements (DOEs) in single crystal diamond. Top-hat and arbitrary pattern DOE beam shapers were numerically optimized using an iterative Fourier transform algorithm (IFTA). Commercially available single crystal diamond plates (3mm×3mm×0.3mm) were patterned using hardmask deposition (α-Si), e-beam lithography, and O2 plasma-based diamond reactive ion etching. The resulting binary phase relief patterns were characterized using scanning electron microscopy (SEM) and atomic force microscopy (AFM). Experimental characterization of the single crystal diamond DOEs in transmission at λ=532nm confirms excellent uniformity of the resulting top-hat beam profile as required in copper welding applications.

AI-enabled real-time dual-comb molecular fingerprint imaging.

Hyperspectral imaging provides spatially resolved spectral information. Utilizing dual-frequency combs as active illumination sources, hyperspectral imaging with ultra-high spectral resolution can be implemented in a scan-free manner when a detector array is used for heterodyne detection. Here, we show that dual-comb hyperspectral imaging can be performed with an uncooled near-to-mid-infrared detector by exploiting the detector array's high frame rate, achieving 10 Hz acquisition in 30 spectral channels across 16,384 pixels. Artificial intelligence (AI) enables real-time data reduction and imaging of gas concentration based on characteristic molecular absorption signatures. Owing to the detector array's sensitivity from 1 to 5 µm wavelength, this demonstration lays the foundation for real-time versatile imaging of molecular fingerprint signatures across the infrared wavelength regime with high temporal resolution.

Thermally stable access to microresonator solitons via slow pump modulation.

Temporal dissipative Kerr solitons (DKSs) in microresonators provide ultra-short optical pulses and low-noise frequency combs with gigahertz to terahertz repetition rates. Owing to their unique properties, they have found application in fields, including optical communications, rapid laser ranging, and optical precision spectroscopy. However, due to the thermal instability encountered when entering the DKS regime, the stable generation of solitons remains challenging for many systems and usually requires rapid actuation of the pump laser detuning, pulsed driving, additional lasers, a particular mode structure and/or active feedback loops to stabilize the system. Here we show that slow pump modulation can remove the thermal instability and enable passively stable soliton states that can be readily accessed via arbitrarily slow laser tuning, thereby greatly reducing the technical complexity of stable DKS generation.

Phase-stabilised self-injection-locked microcomb.

Microresonator frequency combs (microcombs) hold great potential for precision metrology within a compact form factor, impacting a wide range of applications such as point-of-care diagnostics, environmental monitoring, time-keeping, navigation and astronomy. Through the principle of self-injection locking, electrically-driven chip-based microcombs with minimal complexity are now feasible. However, phase-stabilisation of such self-injection-locked microcombs-a prerequisite for metrological frequency combs-has not yet been attained. Here, we address this critical need by demonstrating full phase-stabilisation of a self-injection-locked microcomb. The microresonator is implemented in a silicon nitride photonic chip, and by controlling a pump laser diode and a microheater with low voltage signals (less than 1.57 V), we achieve independent control of the comb's offset and repetition rate frequencies. Both actuators reach a bandwidth of over 100 kHz, enabling phase-locking of the microcomb to external frequency references. These results establish photonic chip-based, self-injection-locked microcombs as low-complexity yet versatile sources for coherent precision metrology in emerging applications.

Femtosecond pulse amplification on a chip.

Femtosecond laser pulses enable the synthesis of light across the electromagnetic spectrum and provide access to ultrafast phenomena in physics, biology, and chemistry. Chip-integration of femtosecond technology could revolutionize applications such as point-of-care diagnostics, bio-medical imaging, portable chemical sensing, or autonomous navigation. However, current chip-integrated pulse sources lack the required peak power, and on-chip amplification of femtosecond pulses has been an unresolved challenge. Here, addressing this challenge, we report  >50-fold amplification of 1 GHz-repetition-rate chirped femtosecond pulses in a CMOS-compatible photonic chip to 800 W peak power with 116 fs pulse duration. This power level is 2-3 orders of magnitude higher compared to those in previously demonstrated on-chip pulse sources and can provide the power needed to address key applications. To achieve this, detrimental nonlinear effects are mitigated through all-normal dispersion, large mode-area and rare-earth-doped gain waveguides. These results offer a pathway to chip-integrated femtosecond technology with peak power levels characteristic of table-top sources.

Ultraviolet astronomical spectrograph calibration with laser frequency combs from nanophotonic lithium niobate waveguides.

Astronomical precision spectroscopy underpins searches for life beyond Earth, direct observation of the expanding Universe and constraining the potential variability of physical constants on cosmological scales. Laser frequency combs can provide the required accurate and precise calibration to the astronomical spectrographs. For cosmological studies, extending the calibration with such astrocombs to the ultraviolet spectral range is desirable, however, strong material dispersion and large spectral separation from the established infrared laser oscillators have made this challenging. Here, we demonstrate astronomical spectrograph calibration with an astrocomb in the ultraviolet spectral range below 400 nm. This is accomplished via chip-integrated highly nonlinear photonics in periodically-poled, nano-fabricated lithium niobate waveguides in conjunction with a robust infrared electro-optic comb generator, as well as a chip-integrated microresonator comb. These results demonstrate a viable route towards astronomical precision spectroscopy in the ultraviolet and could contribute to unlock the full potential of next-generation ground-based and future space-based instruments.

Dual-comb cavity ring-down spectroscopy.

Cavity ring-down spectroscopy is a ubiquitous optical method used to study light-matter interactions with high resolution, sensitivity and accuracy. However, it has never been performed with the multiplexing advantages of direct frequency comb spectroscopy without significantly compromising spectral resolution. We present dual-comb cavity ring-down spectroscopy (DC-CRDS) based on the parallel heterodyne detection of ring-down signals with a local oscillator comb to yield absorption and dispersion spectra. These spectra are obtained from widths and positions of cavity modes. We present two approaches which leverage the dynamic cavity response to coherently or randomly driven changes in the amplitude or frequency of the probe field. Both techniques yield accurate spectra of methane-an important greenhouse gas and breath biomarker. When combined with broadband frequency combs, the high sensitivity, spectral resolution and accuracy of our DC-CRDS technique shows promise for applications like studies of the structure and dynamics of large molecules, multispecies trace gas detection and isotopic composition.

Photo-acoustic dual-frequency comb spectroscopy.

Photo-acoustic spectroscopy (PAS) is one of the most sensitive non-destructive analysis techniques for gases, fluids and solids. It can operate background-free at any wavelength and is applicable to microscopic and even non-transparent samples. Extension of PAS to broadband wavelength coverage is a powerful tool, though challenging to implement without sacrifice of wavelength resolution and acquisition speed. Here we show that dual-frequency comb spectroscopy (DCS) and its potential for unmatched precision, speed and wavelength coverage can be combined with the advantages of photo-acoustic detection. Acoustic wave interferograms are generated in the sample by dual-comb absorption and detected by a microphone. As an example, weak gas absorption features are precisely and rapidly sampled; long-term coherent averaging further increases the sensitivity. This novel approach of dual-frequency comb photo-acoustic spectroscopy (DCPAS) generates unprecedented opportunities for rapid and sensitive multi-species molecular analysis across all wavelengths of light.