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High-Efficiency Second-Harmonic Generation from Hybrid Light-Matter States.
Chervy, Thibault; Xu, Jialiang; Duan, Yulong; Wang, Chunliang; Mager, Loïc; Frerejean, Maurice; Münninghoff, Joris A W; Tinnemans, Paul; Hutchison, James A; Genet, Cyriaque; Rowan, Alan E; Rasing, Theo; Ebbesen, Thomas W.
Affiliation
  • Chervy T; ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg, France.
  • Xu J; School of Chemical Engineering and Technology, Tianjin University , Yaguan Road 135, 300350 Tianjin, People's Republic of China.
  • Duan Y; Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.
  • Wang C; Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.
  • Mager L; ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg, France.
  • Frerejean M; IPCMS, University of Strasbourg and CNRS , 23 rue du Loess, 67034 Strasbourg, France.
  • Münninghoff JA; Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.
  • Tinnemans P; Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.
  • Hutchison JA; Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.
  • Genet C; ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg, France.
  • Rowan AE; ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg, France.
  • Rasing T; Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.
  • Ebbesen TW; Australian Institute for Bioengineering and Nanotechnology (AIBN), The University of Queensland , Brisbane, Queensland 4072, Australia.
Nano Lett ; 16(12): 7352-7356, 2016 12 14.
Article in En | MEDLINE | ID: mdl-27960510
ABSTRACT
We report a novel approach to modify the second order nonlinear optical (NLO) susceptibility of organic nanofiber crystals by hybridization with the optical modes of microcavities in the strong coupling regime. The wavelength dependence of the SHG efficiency displays two intense peaks corresponding to the so-formed light-matter hybrid states. Our results demonstrate an enhancement of the resonant SHG efficiency of the lower polariton by 2 orders of magnitude for the collectively coupled molecules as compared to that of the same material outside the microcavity. This study is a proof of principle that opens a new direction for NLO of organic materials in subwavelength resonators.
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Collection: 01-internacional Database: MEDLINE Language: En Journal: Nano Lett Year: 2016 Type: Article Affiliation country: France
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PubMed Links

Collection: 01-internacional Database: MEDLINE Language: En Journal: Nano Lett Year: 2016 Type: Article Affiliation country: France