Ground state of the easy-axis rare-earth kagome langasite Pr3Ga5SiO14.
Phys Rev Lett
; 104(5): 057202, 2010 Feb 05.
Article
em En
| MEDLINE
| ID: mdl-20366794
We report muon spin relaxation and {69,71}Ga nuclear quadrupolar resonance local-probe investigations of the kagome compound Pr3Ga5SiO14. Small quasistatic random internal fields develop below 40 K and persist down to our base temperature of 21 mK. They originate from hyperfine-enhanced 141Pr nuclear magnetism which requires a nonmagnetic Pr3+ crystal-field (CF) ground state. In addition, we observe a broad maximum of the relaxation rate at approximately 10 K which we attribute to the population of the first excited magnetic CF level. Our results yield a Van Vleck paramagnet picture, at variance with the formerly proposed spin-liquid ground state.
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Phys Rev Lett
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2010
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Article
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